Reuse & Permissions

It is not necessary to obtain permission to reuse this article or its components as it is available under the terms of the Creative Commons Attribution 4.0 International license. This license permits unrestricted use, distribution, and reproduction in any medium, provided attribution to the author(s) and the published article's title, journal citation, and DOI are maintained. Please note that some figures may have been included with permission from other third parties. It is your responsibility to obtain the proper permission from the rights holder directly for these figures.

Export citation

Export citation

Choose format for download:

Download Citation
  • Editors' Suggestion
  • Open Access

Orthogonality point and intersublattice exchange in Dy2Fe17 determined in strong magnetic fields

Y. Skourski1,*, M. D. Kuz'min2, K. P. Skokov3, N. Shayanfar3, A. V. Andreev4, S. Zherlitsyn1, S. Yasin1,†, L. Zvyagina1, O. Drachenko5 et al.

O. Portugall5 and J. Wosnitza1,6

  • *Contact author: skourski@hzdr.de
  • †Present address: College of Integrative Studies, Abdullah Al Salem University, Khaldiya, Kuwait.

Phys. Rev. Materials 9, 064404 – Published 10 June, 2025

DOI: https://doi.org/10.1103/scy5-m3j8

Abstract

We report on magnetization measurements of single crystalline Dy2Fe17 in pulsed magnetic fields up to ∼127T. To produce the fields, we used (i) a single- and (ii) a double-coil magnet generating pulses in the 10 ms range, as well as (iii) semidestructive single-turn coils creating pulses of much shorter duration, ∼5µs. We observed steplike transitions at 64.3 and 77.7 T, for fields applied along [100] and [120], respectively. We confirmed the latter transition by ultrasound-velocity measurements using the double-coil magnet. Our data allowed us to locate the orthogonality point of Dy2Fe17 at (μ0H⊥=90T, M⊥=31μB/f.u.) and determine the intersublattice exchange field, μ0Hex=215T.

View figure in article

Physics Subject Headings (PhySH)

Article Text

References (35)

  1. J. M. D. Coey, Hard magnetic materials: A perspective, IEEE Trans. Magn. 47, 4671 (2011).
  2. K.-H. Müller, S. Sawatzki, R. Gauß, and O. Gutfleisch, in Handbook of Magnetism and Magnetic Materials, edited by J. M. D. Coey and S. S. P. Parkin (Springer, Cham, 2018), p. 1369.
  3. J. M. D. Coey, Perspective and prospects for rare earth permanent magnets, Engineering 6, 119 (2020).
  4. D. Gignoux and D. Schmitt, in Handbook on the Physics and Chemistry of Rare Earths, edited by K. A. Gschneidner, Jr. and L. Eyring (Elsevier Science, Amsterdam, 1995), Vol. 20, p. 293.
  5. W. F. Li, H. Sepehri-Amin, T. Ohkubo, N. Hase, and K. Hono, Distribution of Dy in high-coercivity (Nd, Dy)–Fe–B sintered magnet, Acta Mater. 59, 3061 (2011).
  6. V. P. Menushenkov and A. G. Savchenko, Heat treatment, microstructure and coercivity of (Nd, Dy)-Fe-B based permanent magnets, J. Magn. Magn. Mater. 272–276, E1891 (2004).
  7. K. Clausen and B. Lebech, Magnetic excitations in Ho2Co17 and Ho2Fe17, J. Phys. C: Solid State Phys. 15, 5095 (1982).
  8. S. Sinnema, Magnetic interactions in R2T17 and R2T17B intermetallic compounds, Ph.D. thesis, University of Amsterdam, 1988.
  9. R. Verhoef, P. H. Quang, R. J. Radwanski, C. Marquina, and J. J. M. Franse, Magnetisation curves of single-crystalline Tb2Fe17, J. Magn. Magn. Mater. 104–107, 1473 (1992).
  10. R. Verhoef, F. R. de Boer, S. Sinnema, J. J. M. Franse, F. Tomiyama, M. Ono, M. Date, and A. Yamagishi, Multiple field-induced transitions in Er2Fe17 in fields up to 50 T, Phys. B: Condens. Matter 177, 223 (1992).
  11. Y. Skourski, M. D. Kuz'min, K. P. Skokov, A. V. Andreev, and J. Wosnitza, High-field magnetization of Ho2Fe17, Phys. Rev. B 83, 214420 (2011).
  12. M. D. Kuz'min, Y. Skourski, K. P. Skokov, and K. H. Müller, High-field magnetization measurements on Er2Fe17 single crystals, Phys. Rev. B 75, 184439 (2007).
  13. O. Isnard, A. V. Andreev, M. D. Kuz'min, Y. Skourski, D. I. Gorbunov, J. Wosnitza, N. V. Kudrevatykh, A. Iwasa, A. Kondo, A. Matsuo, and K. Kindo, High magnetic field study of the Tm2Fe17 and Tm2Fe17D3.2 compounds, Phys. Rev. B 88, 174406 (2013).
  14. R. Gersdorf, P. H. Frings, J. J. M. Franse, and F. R. de Boer, The Amsterdam high-field facility, Phys. B: Condens. Matter 201, 530 (1994).
  15. J. P. Liu, F. R. de Boer, P. F. de Châtel, R. Coehoorn, and K. H. J. Buschow, On the 4f−3d exchange interaction in intermetallic compounds, J. Magn. Magn. Mater. 132, 159 (1994).
  16. T. Asano, Y. Sakai, M. Oshikiri, K. Inoue, H. Maeda, G. Heremans, L. Van Bockstal, Li Liang, and F. Herlach, Copper-silver wire coils for pulsed magnet, Phys. B: Condens. Matter 201, 556 (1994).
  17. G. S. Boebinger, A. H. Lacerda, H. J. Schneider-Muntau, and N. Sullivan, The national high magnetic field laboratory's pulsed magnetic field facility in los alamos, Phys. B: Condens. Matter 294–295, 512 (2001).
  18. S. Zherlitsyn, A. D. Bianchi, T. Herrmannsdoerfer, F. Pobell, Y. Skourski, A. Sytcheva, S. Zvyagin, and J. Wosnitza, Coil design for non-destructive pulsed-field magnets targeting 100 T, IEEE Trans. Appl. Supercond. 16, 1660 (2006).
  19. K. Kindo, 100 T magnet developed in Osaka, Phys. B: Condens. Matter 294–295, 585 (2001).
  20. S. Zherlitsyn, B. Wustmann, T. Herrmannsdörfer, and J. Wosnitza, Status of the pulsed-magnet-development program at the dresden high magnetic field laboratory, IEEE Trans. Appl. Supercond. 22, 4300603 (2012).
  21. H. Jones, P. H. Frings, M. von Ortenberg, A. Lagutin, L. van Bockstal, O. Portugall, and F. Herlach, First experiments in fields above 75 T in the European “coilin-coilex” magnet, Phys. B: Condens. Matter 346–347, 553 (2004).
  22. O. Portugall, P. Y. Solane, P. Plochocka, D. K. Maude, and R. J. Nicholas, Beyond 100 Tesla: Scientific experiments using single-turn coils, C. R. Phys. 14, 115 (2013).
  23. O. Portugall, N. Puhlmann, H. U. Müller, M. Barczewski, I. Stolpe, and M. von Ortenberg, Megagauss magnetic field generation in single-turn coils: New frontiers for scientific experiments, J. Phys. D 32, 2354 (1999).
  24. S. Zherlitsyn, S. Yasin, J. Wosnitza, A. A. Zvyagin, A. V. Andreev, and V. Tsurkan, Spin-lattice effects in selected antiferromagnetic materials, Low Temp. Phys. 40, 123 (2014).
  25. O. Isnard, S. Miraglia, J. L. Soubeyroux, D. Fruchart, and P. l'Héritier, A structural analysis and some magnetic properties of the R2Fe17Hx series, J. Magn. Magn. Mater. 137, 151 (1994).
  26. K. H. J. Buschow, Intermetallic compounds of rare-earth and 3d transition metals, Rep. Prog. Phys. 40, 1179 (1977).
  27. A. V. Andreev, Y. Skourski, M. D. Kuz'min, S. Yasin, S. Zherlitsyn, R. Daou, J. Wosnitza, A. Iwasa, A. Kondo, A. Matsuo, and K. Kindo, Magnetic and magnetoelastic anomalies of an Er2Co17 single crystal in high magnetic fields, Phys. Rev. B 83, 184422 (2011).
  28. M. D. Kuz'min, Deducing model parameters of ferrimagnets from high-field magnetization curves, Phys. Rev. B 79, 212405 (2009).
  29. B. Lüthi, Physical Acoustics in the Solid State (Springer, Berlin, Heidelberg, 2005).
  30. M. D. Kuz'min and M. Richter, Lanthanide exchange fields and intermultiplet transitions in permanent-magnet materials, Eur. Phys. J. Plus 138, 1068 (2023).
  31. M. Loewenhaupt, P. Tils, D. P. Middleton, K. H. J. Buschow, and R. Eccleston, Nitrogen-induced reduction of the Gd-Fe exchange coupling in Gd2Fe17Nx, J. Magn. Magn. Mater. 129, L151 (1994).
  32. T. Goto, T. Sakakibara, K. Murata, H. Komatsu, and K. Fukamichi, Itinerant electron metamagnetism in YCo2 and LuCo2, J. Magn. Magn. Mater. 90–91, 700 (1990).
  33. T. Goto, H. Aruga Katori, T. Sakakibara, and M. Yamaguchi, Successive phase transitions in ferromagnetic YCo3, Phys. B: Condens. Matter 177, 255 (1992).
  34. T. T. Terashima, A. Ikeda, Y. H. Matsuda, A. Kondo, K. Kindo, and F. Iga, Magnetization process of the kondo insulator YbB in ultrahigh magnetic fields, J. Phys. Soc. Jpn. 86, 054710 (2017).
  35. https://mgml.eu

Outline

Information

Sign In to Your Journals Account

Filter

Filter

Article Lookup

Enter a citation