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    Intrinsic even-odd thickness-driven anomalous Hall effect in epitaxial MnBi2Te4 thin films

    Debarghya Mallick1, Simon Kim1, An-Hsi Chen1, Gabriel A. Vázquez-Lizardi2, Alessandro R. Mazza3, T. Zac Ward4, Gyula Eres1, Yue Cao5, Debangshu Mukherjee6 et al.

    Hu Miao1, Liang Wu7, Christopher Nelson4, Danielle Reifsnyder Hickey2,8,9, Robert G. Moore1, and Matthew Brahlek1,*

    • *Contact author: brahlekm@ornl.gov

    Phys. Rev. Materials 10, 044203 – Published 21 April, 2026

    DOI: https://doi.org/10.1103/pqj7-prc1

    Abstract

    We demonstrate precise control of magnetism in MnBi2Te4 thin films through careful synthesis by molecular beam epitaxy, achieving minimal defects and accurate layer thickness control. By optimizing Mn-Bi-Te ratios and growth temperatures, we minimize detrimental self-doping effects and accurately target integer-layer films. X-ray diffraction and reflectivity provide quantitative measures of film quality and thickness. When these macroscale probes of structure and thickness are integrated with magnetotransport measurements, a striking even-odd layer dependence of the anomalous Hall effect is revealed. Odd-layer films exhibit a large hysteresis up to the Néel temperature (∼25K), consistent with noncompensated antiferromagnetism, while even-layer films show minimal response, as expected for an antiferromagnet. The sign of the anomalous Hall effect exhibits a sign reversal for intrinsic magnetism versus magnetism associated with defects. This work identifies critical factors for inducing pure, noncompensated ferromagnetism and reveals the characteristics of the intrinsic anomalous Hall effect in MnBi2Te4, which together is a step toward realizing the zero-field quantum anomalous Hall effect in topological materials.

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