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    Magnetic topological textures in BiFeO3 with ferroelectric domain walls

    Tiziana Musso*

    Bin Xu

    Yousra Nahas and Sergei Prokhorenko

    Daniel Sando†

    Nagarajan Valanoor

    • Jiangsu Key Laboratory of Frontier Material Physics and Devices, School of Physical Science and Technology, Soochow University, Suzhou 215006, China

    • Smart Ferroic Materials Center, Physics Department and Institute for Nanoscience and Engineering, University of Arkansas, Fayetteville, Arkansas, USA

    • MacDiarmid Institute for Advanced Materials and Nanotechnology, School of Physical and Chemical Sciences, University of Canterbury, Christchurch 8042, New Zealand

    • *Contact author: t.musso@unsw.edu.au
    • †Contact author: daniel.sando@canterbury.ac.nz

    Phys. Rev. Materials 9, 114410 – Published 13 November, 2025

    DOI: https://doi.org/10.1103/kptk-8dzc

    Abstract

    Topological defects in ferroic materials are attracting significant attention due to their role as a platform for distinctive physical phenomena and their potential applications in electronic devices. Bismuth ferrite stands out as a well-known multiferroic material, exhibiting both ferroelectric and antiferromagnetic properties at room temperature. While magnetic topological defects in bismuth ferrite begin to be well documented, the influence of cycloids with different propagation directions on the magnetic structure at ferroelectric domain walls remains relatively unexplored. In this study, we employ a first-principles-based effective Hamiltonian method in conjunction with Monte Carlo simulations to predict the formation of distinct magnetic textures at ferroelectric domain walls. An analysis of the Pontryagin charge density reveals them to be localized Bloch points, merons, and homogeneous Pontryagin charge-density tubes, which hold promise for future usage in electronic devices.

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