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Tuning magnetic ground states of RMn6Sn6 (R = Lu, Mg) kagome metals by dimensionality reduction: Route to ferromagnetism and large anomalous Hall effect

Rajdeep Biswas1,*,†, Jyoti Sharma2,*,‡, Aftab Alam2,§, and Tanusri Saha Dasgupta1,∥

  • *These authors contributed equally to this work.
  • †Contact author: biswasprabal49@gmail.com
  • ‡Contact author: jsharma628@gmail.com
  • §Contact author: aftab@phy.iitb.ac.in
  • ∥Contact author: t.sahadasgupta@gmail.com

Phys. Rev. Materials 9, 104205 – Published 30 October, 2025

DOI: https://doi.org/10.1103/h9ym-4cp2

Abstract

The ternary intermetallic compounds, RMn6Sn6 (R = rare-earth or alkali or alkaline-earth metal) hosting Kagome bilayer of Mn, present a class of systems that naturally allows for the interplay of magnetism and topology. In search of ferromagnetic members in these systems, we show that dimensional reduction can be an effective means to achieve ferromagnetism and large anomalous Hall conductivity. Focusing on two specific members with R = Lu and Mg, our first-principles calculations show that dimensional confinement through the construction of experimentally relevant atomistically thin single bilayer kagome geometry of Mn atoms gives rise to a ferromagnetic metal with multiple Weyl points along with spin-orbit-coupling induced gapped bands. The calculated anomalous Hall conductivity in the thin film geometry turns out to be 287 and 178Ω−1cm−1, comparable to that found for bulk RMn6Sn6 with alkali or alkaline-earth metal at R site. This is of interest as thin-film geometry can be efficiently integrated to devices.

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