Export citation

Export citation

Choose format for download:

Download Citation
  • Letter

Persistence of charge density wave fluctuations in the absence of long-range order in a hole-doped kagome metal

Terawit Kongruengkit1, Andrea N. Capa Salinas1, Ganesh Pokharel1, Brenden R. Ortiz2, Stephen D. Wilson1, and John W. Harter1,*

  • *Contact author: harter@ucsb.edu

Phys. Rev. Materials 10, L022001 – Published 5 February, 2026

DOI: https://doi.org/10.1103/fzx6-hd1b

Abstract

The kagome metals AV3Sb5 (A=K, Rb, Cs) exhibit a complex interplay between charge density wave (CDW) order and superconductivity. In this study, we use ultrafast coherent phonon spectroscopy to probe the evolution of CDW order in hole-doped CsV3Sb5−xSnx across a broad range of compositions (0≤x≤0.68). While thermodynamic and diffraction measurements show long-range CDW order vanishes above x≈0.05, we observe persistent signatures of CDW fluctuations up to the highest doping levels, with correlation times on the order of several picoseconds. These results indicate the presence of a robust fluctuating charge order that survives well beyond the established CDW phase boundary. Furthermore, these fluctuations are enhanced near a doping-tuned quantum phase transition at x*≈0.15, which coincides with a local minimum in the superconducting Tc double-dome. Additional measurements on Ti- and K-substituted samples confirm that this behavior is intrinsic to hole doping and not tied to disorder. Overall, our findings suggest that CDW fluctuations play a central role in the electronic phase diagram of AV3Sb5 and may mediate or compete with superconductivity.

Physics Subject Headings (PhySH)

Collections

This article appears in the following collection:

Quantum Phenomena in Kagome Materials

The Editors of Physical Review Materials are pleased to present the Collection on Quantum Phenomena in Kagome Materials, highlighting cutting-edge advances in theory, synthesis, properties and applications of kagome materials. The Collection is being guest-edited by Mingda Li (MIT), Xiangang Wan (Nanjing University) and Linda Ye (Caltech). Every article published in this collection underwent a rigorous peer review process, adhering to the same high standards applied to all papers. The Physical Review Materials editorial team managed the peer review and made all editorial decisions.

Authorization Required

We need you to provide your credentials before accessing this content.

Supplemental Material (Subscription Required)

References (Subscription Required)

Outline

Information

Sign In to Your Journals Account

Filter

Filter

Article Lookup

Enter a citation