Study of the anisotropic hidden order and antiferromagnetic phases of by thermal expansion and magnetoresistance measurements
Phys. Rev. Materials 9, 075001 – Published 8 July, 2025
DOI: https://doi.org/10.1103/d4d2-pn8c
Abstract
Thermal expansion and magnetoresistance measurements as a function of temperature (T) and magnetic field (B), respectively, were carried out on Os-substituted single crystals with to 0.28. Mean-field-like peaks at temperature in the linear thermal expansion coefficient vs T curves in both the hidden order (HO) phase and the large-moment antiferromagnetic (LMAFM) phase of exhibit a striking resemblance and a discontinuity in at delineating the boundary between the two phases. Anomalies at were also seen in both the calculated effective Grüneisen parameter and the energy gap associated with the HO or LMAFM phase. The hydrostatic pressure derivative of calculated from thermal expansion and specific heat [D. L. Kunwar et al., Phys. Rev. B 105, L041106 (2022)] data agree with the experimental results [C. T. Wolowiec, Proc. Natl Acad. Sci. USA 118, e2026591118 (2021)], whereas the calculated uniaxial pressure derivatives in different crystallographic directions are anisotropic, as shown in the anisotropic linear thermal expansion. This anisotropy was further reflected in the radically different responses of to B applied in different directions: a few percent change in is induced for B parallel to the axis, whereas barely changes for B applied in the of the single crystals, regardless of whether the crystals are in the HO or LMAFM phase.