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    Switchable anomalous valley Hall effect in 2D antiferromagnetic system

    Jiaxuan Hui, Yandong Ma*, Ying Dai, Baibiao Huang, and Xinru Li†

    • School of Physics, State Key Laboratory of Crystal Materials, Shandong University, Shandanan Str. 27, Jinan 250100, China

    • *Contact author: yandong.ma@sdu.edu.cn
    • †Contact author: lixr@sdu.edu.cn

    Phys. Rev. Materials 10, 024402 – Published 6 February, 2026

    DOI: https://doi.org/10.1103/bdfy-8ff7

    Abstract

    Currently, the realization and control of anomalous valley Hall effect (AVHE) in two-dimensional antiferromagnetic (AFM) systems are predominantly achieved through optical excitation, which hinders its practical applications. Here, we propose a strategy to overcome this limitation by inserting a valley-active AFM layer between two ferromagnetic (FM) semiconductor layers. Using CrCl3−VSiS3−CrCl3 heterotrilayer as a model system, our first-principles calculations reveal that interfacial proximity coupling can introduce intrinsic sublattice-asymmetric exchange field. This field can break the PT symmetry and lift the spin degeneracy of valleys in the AFM layer while preserving its intrinsic valley polarization, thereby inducing a pronounced AVHE. Crucially, the sublattice-asymmetric exchange field can be reversed through flipping the magnetization orientation of the FM layers, resulting in reversible static control of AVHE without altering the AFM Néel order. These findings establish an alternative paradigm for controlling AVHE in AFM materials and advance the field of antiferromagnet-based valleytronics.

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