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Tuning the magnetic anisotropy in artificially layered Mn3GaN/Mn3Ga superlattices

Lu Guo1,*, Neil Campbell2,*, Alexander J. Grutter3, Gahee Noh5, Tianxiang Nan1, Paige Quarterman3, Si-Young Choi5,6, Thomas Tybell4, Mark S. Rzchowski2 et al.

Chang-Beom Eom1,†

  • 1Department of Materials Science and Engineering, University of Wisconsin-Madison, Madison, Wisconsin 53706, USA
  • 2Department of Physics, University of Wisconsin-Madison, Madison, Wisconsin 53706, USA
  • 3NIST Center for Neutron Research, National Institute of Standards and Technology, Gaithersburg, Maryland 20899, USA
  • 4Department of Electronic Systems, Norwegian University of Science and Technology, Trondheim 7491, Norway
  • 5Department of Materials Science and Engineering, Pohang University of Science and Technology, Pohang 37673, Republic of Korea
  • 6Center for Van der Waals Quantum Solids, Institute for Basic Science, Pohang 37673, Republic of Korea

  • *These authors contributed equally to this work.
  • †Corresponding author: eom@engr.wisc.edu

Phys. Rev. Materials 8, L011401 – Published 31 January, 2024

DOI: https://doi.org/10.1103/PhysRevMaterials.8.L011401

Abstract

Artificially layered superlattices with two distinct spin structures offer new opportunities for manipulation of magnetic properties and interfacial spin configurations. We have grown epitaxial, coherent superlattices of ferrimagnetic Mn3Ga and noncollinear antiferromagnetic Mn3GaN. The out-of-plane ferrimagnetism of the Mn3Ga layer, and the Berry-phase charge to spin current generation by the noncollinear antiferromagnetic Mn3GaN layer, provide a unique combination for spintronic applications. Reactive magnetron sputtering growth resulted in abrupt transitions between the two layers through controlling the N2 flow. X-ray diffraction and cross-sectional scanning transmission electron microscopy images demonstrate clean layering and consistent modulation wavelengths, with interfacial roughness less than one unit cell. This allows investigation of the interfacial magnetic interactions. Through a combination of superconducting quantum interference device magnetometry and polarized neutron reflectometry we show that Mn3Ga/Mn3GaN superlattice structures have the out-of-plane magnetic anisotropy decreased compared to Mn3Ga single-layer films. This softening is primarily a result of reduced anisotropy energy at the interface and is linked to the Mn3GaN layer. This superlattice structure provides a platform for devices that use out-of-plane spin torques generated from an antiferromagnetic material to switch the net magnetic moment of a ferrimagnetic material. Our results demonstrate the tunability of magnetic anisotropy to allow for optimal balancing of the switching power and thermal stability in spintronic heterostructures.

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