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Emergence of partially disordered antiferromagnetism and isothermal magnetization plateau due to geometrical frustration in a metallic compound, Er2RhSi3

Kartik K. Iyer1,2,*, Kalobaran Maiti1, Sudhindra Rayaprol3, Ram Kumar4, S. Mattepanavar5, S. Dodamani2, and E. V. Sampathkumaran6,†

  • 1Tata Institute of Fundamental Research, Homi Bhabha Road, Colaba, Mumbai 400005, India
  • 2KLE Society's Dr. Prabhakar Kore Basic Science Research Centre, KLE Academy of Higher Education and Research, Belagavi 590010, India
  • 3UGC-DAE Consortium for Scientific Research, Mumbai Centre, BARC Campus, Trombay, Mumbai 400085, India
  • 4Maryland Quantum Materials Center, University of Maryland, College Park, Maryland 20742, USA
  • 5KLE Society's Basavaprabhu Kore Arts, Science and Commerce College, Chikodi 591201, India
  • 6Homi Bhabha Centre for Science Education, TIFR, V. N. Purav Marg, Mankhurd, Mumbai 400088, India

  • *Iyerkk@gmail.com
  • †sampathev@gmail.com

Phys. Rev. Materials 7, L101401 – Published 10 October, 2023

DOI: https://doi.org/10.1103/PhysRevMaterials.7.L101401

Abstract

Partially disordered antiferromagnetism (PDA) (in which one of the three magnetic ions in a triangular network remains magnetically disordered) has been known commonly among geometrically frustrated insulating materials. The 1/3 plateau in isothermal magnetization M of such materials has been of great theoretical interest. Here we report these properties in an AlB2-structure-derived metallic material, Er2RhSi3, in which the Er sublattice has triangular networks. The presence of a well-defined λ anomaly in the temperature T dependence of heat capacity and its magnetic-field H dependence and the loss of spin-disorder contribution to electrical resistivity ρ confirm antiferromagnetic order below TN=5K. On the other hand, the separation of zero-field-cooled and field-cooled dc magnetic susceptibility χ curves, the decay of isothermal remnant magnetization, and the frequency dependence of real and imaginary components of ac χ suggest the onset of spin-glass freezing concomitant with the antiferromagnetic order. In addition, interestingly, we observe the 1/3 plateau in M(H) below 20 kOe for T<TN. The change in ρ as a function of H at a given temperature well below TN is also revealing, with this compound exhibiting a plateau below 20 kOe, with complexities at higher fields. Therefore, this compound serves as a prototype for theoretical understanding of transport behavior across the 1/3 plateau due to PDA magnetism in a metal without any interference from the 4f delocalization phenomenon.

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