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    Epitaxial growth and superconductivity of optimally doped Sr1−xEuxCuO2 cuprate films

    Hang Yan1, Ze-Xian Deng1, Jia-Qi Fan1, Xue-Qing Yu1, Xiao-Peng Hu1, Can-Li Song1,2,*, Xu-Cun Ma1,2,†, and Qi-Kun Xue1,2,3,4

    • 1State Key Laboratory of Low-Dimensional Quantum Physics, Department of Physics, Tsinghua University, Beijing 100084, China
    • 2Frontier Science Center for Quantum Information, Beijing 100084, China
    • 3Beijing Academy of Quantum Information Sciences, Beijing 100193, China
    • 4Southern University of Science and Technology, Shenzhen 518055, China

    • *Corresponding author: clsong07@mail.tsinghua.edu.cn
    • †Corresponding author: xucunma@mail.tsinghua.edu.cn

    Phys. Rev. Materials 7, 074802 – Published 6 July, 2023

    DOI: https://doi.org/10.1103/PhysRevMaterials.7.074802

    Abstract

    Superconducting infinite-layer Sr1−xEuxCuO2 films at optimal doping (x∼0.15) have been epitaxially grown on SrTiO3(001) substrates with oxide molecular beam epitaxy. By combining x-ray diffraction and transport measurements, we have established a narrow window of growth conditions [i.e., ozone pressure, substrate temperature, (Sr+Eu)/Cu flux ratio, and postannealing] in which the superconducting infinite-layer structure can be readily achieved while eliminating any unwanted competing phases. A smaller out-of-plane lattice constant (c<3.42Å) is found to be crucial to prompt superconductivity in the Sr1−xEuxCuO2 films. Thickness-dependent electrical resistivity measurements reveal superconductivity even when the film thickness is thinned down to 5 nm. Furthermore, the superconducting state of the epitaxial infinite-layer films remains remarkably stable against air exposure, providing an ideal platform to explore the high-temperature superconductivity and unusual properties in cuprates.

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