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Interfacial potential gradient modulates Dzyaloshinskii-Moriya interaction in Pt/Co/metal multilayers

Fernando Ajejas1,*, Yanis Sassi1, William Legrand1, Sophie Collin1, Jose Peña Garcia2, André Thiaville3, Stefania Pizzini2, Nicolas Reyren1, Vincent Cros1,† et al.

Albert Fert1

  • 1Unité Mixte de Physique, CNRS, Thales, Université Paris-Saclay, 91767, Palaiseau, France
  • 2Université Grenoble Alpes, CNRS, Institut Néel, F-38000 Grenoble, France
  • 3Laboratoire de Physique des Solides, Université Paris-Saclay, CNRS UMR 8502, 91405, Orsay Cedex, France

  • *Present address: Department of Physics and Center for Advanced Nanoscience, University of California, San Diego, La Jolla, California 92093, USA; fajejas@physics.ucsd.edu
  • †vincent.cros@cnrs-thales.fr.

Phys. Rev. Materials 6, L071401 – Published 5 July, 2022

DOI: https://doi.org/10.1103/PhysRevMaterials.6.L071401

Abstract

The actual mechanisms occurring at interfaces underlying the Dzyaloshinskii-Moriya interaction (DMI) remain a question in nanomagnetism. In this study, we investigate the origin of the interfacial DMI, aiming at estimating how independent the DMI contributions of the two interfaces of a FM layer are and what their relative weight in the effective DMI amplitude is. To this aim, we explore the correlation between the effective interfacial DMI and the metal properties, namely, atomic number, electronegativity, and the work function of the metal M. A clear linear relationship is found between the interfacial DMI and the work function difference at the Co/M interface. This result is strong evidence of the independent DMI contributions of the two interfaces for the chosen Co thickness(1 nm). It also suggests that the Co/Cu interface bears no interfacial DMI. These findings can guide the optimization of the magnetic properties of future devices.

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