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Reemergence of superconductivity in pressurized quasi-one-dimensional superconductor K2Mo3As3

Cheng Huang1,2,*, Jing Guo1,4,*, Kang Zhao1,2,*, Fan Cui1,2, Shengshan Qin1,2, Qingge Mu1, Yazhou Zhou1, Shu Cai1,2, Chongli Yang1 et al.

Sijin Long1,2, Ke Yang3, Aiguo Li3, Qi Wu1, Zhian Ren1,2, Jiangping Hu1,2, and Liling Sun1,2,4,†

  • 1Institute of Physics and Beijing National Laboratory for Condensed Matter Physics, Chinese Academy of Sciences, Beijing 100190, China
  • 2University of Chinese Academy of Sciences, Beijing 100190, China
  • 3Shanghai Synchrotron Radiation Facilities, Shanghai Institute of Applied Physics, Chinese Academy of Sciences, Shanghai 201204, China
  • 4Songshan Lake Materials Laboratory, Dongguan, Guangdong 523808, China

  • *These authors contributed equally to this work.
  • †Author to whom correspondence may be addressed: llsun@iphy.ac.cn

Phys. Rev. Materials 5, L021801 – Published 1 February, 2021

DOI: https://doi.org/10.1103/PhysRevMaterials.5.L021801

Abstract

Here we report a pressure-induced reemergence of superconductivity in a recently discovered superconductor K2Mo3As3, which is an experimental case observed in quasi-one-dimensional superconductors. We find that, after full suppression of the ambient-pressure superconducting (SC-I) state at 8.7 GPa, an intermediary nonsuperconducting state sets in and prevails to the pressure up to 18.2 GPa, however, above this pressure a different superconducting (SC-II) state appears unexpectedly. High pressure x-ray diffraction measurements demonstrate that the pressure-induced dramatic change of the lattice parameter c contributes mainly to the emergence of the SC-II state. Combined with the theoretical calculations on band structure, our results suggest that the reemergence of superconductivity is associated with the change of the complicated interplay among different orbital electrons, driven by the pressure-induced anisotropic change of the lattice.

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