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    Metamagnetic transitions in Ba2LnFeO5 (Ln = Tb, Dy, Ho, Yb): Spin-flip processes in single or dual easy-axis systems

    V. Hardy, F. Guillou, V. Caignaert, F. Veillon, Y. Bréard, and B. Raveau

    F. Wilhelm and A. Rogalev

    B. Gonano

    • Center for Materials Science and Nanotechnology, Department of Chemistry, University of Oslo, PO Box 1033 Blindern, N-0315 Oslo, Norway

    Phys. Rev. Materials 10, 054409 – Published 8 May, 2026

    DOI: https://doi.org/10.1103/8fcn-lq24

    Abstract

    We report on the metamagnetic transition observed in oxides Ba2LnFeO5 (Ln = Tb, Dy, Ho, Er, Yb), which contain two magnetic sublattices: Fe3+ and Ln3+. The magnetic ordering in these materials results from a competition between several types of interaction (Fe-Fe, Fe-Ln, and Ln−Ln), combined in most cases with a strong easy-axis anisotropy of the Ln3+ magnetic moments induced by the crystal electric field (CEF). A specific mechanism is proposed to account for the peculiar metamagnetism in this class of materials, and its variation along the Ln series. This study is based on a set of results including magnetization, x-ray magnetic circular dichroism, neutron powder diffraction, and calculations of the CEF.

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