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    Quantum anomalous Hall effect of Mo-doped LiMgAs monolayer with high transmittance

    Zhen Wang1, Xianglin Liu1, Yuxin Li1, Yuli Xiong1, Jie Zhang1, Yifu Luo1, Shoubing Ding1,*, Tie Yang2,†, Zhenxiang Cheng3 et al.

    Zhimin Wu1,‡

    • *Contact author: shoubingding@cqnu.edu.cn
    • †Contact author: yangtie@swu.edu.cn
    • ‡Contact author: zmwu@cqnu.edu.cn

    Phys. Rev. Materials 9, 104202 – Published 6 October, 2025

    DOI: https://doi.org/10.1103/6vyb-888l

    Abstract

    Two-dimensional (2D) ferromagnetic topological materials (FMTMs), capable of integrating spin-polarized conduction and nontrivial quantum states, are pivotal for advancing spintronic and topological microelectronics. However, existing 2D FMTMs face a critical trade-off between robust quantum phenomena (e.g., quantum anomalous Hall effect, QAHE) and optical transparency. Here, we demonstrate through first-principles calculations that a Mo-doped LiMgAs monolayer (Li12Mg10Mo2As12) breaks this limitation by synergizing the groundbreaking features: (1) strain-robust Weyl half-semimetallicity with fully spin-polarized Weyl points near the Fermi level, stable under −5%–5% biaxial strain; (2) topological phase transition to QAHE via spin-orbit coupling (SOC), yielding a Chern number C = +1 and quantum anomalous Hall effect; and (3) unprecedented optical transparency (without SOC) exceeding 90% in the visible spectrum, outperforming conventional 2D magnetic systems. Remarkably, the Li12Mg10Mo2As12 monolayer maintains room-temperature-compatible thermal stability (300 K ab initio molecular dynamics simulations) and a much higher Curie temperature (TC=178 K). This multifunctional integration of half-metallic ferromagnetism, topology-switching capability, and ultrahigh transparency positions Li12Mg10Mo2As12 as a promising material for designing transparent quantum Hall sensors, low-power spin filters, and wearable optoelectronic devices, thereby bridging quantum topology with photonic technology.

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