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Scaling behavior and giant field enhancement of the thermal conductivity in the honeycomb antiferromagnet BaCo2(AsO4)2

Jiayi Hu1,*, Ruidan Zhong2,†, Peter Czajka1, Tong Gao1,‡, R. J. Cava2, and N. P. Ong1,§

  • *Contact author: jihcindy@gmail.com
  • †Present address: Tsung-Dao Lee Institute and School of Physics and Astronomy, Shanghai Jiao Tong University, Shanghai 201210, China.
  • ‡Present address: Building 3, West Area, Xibeiwang East Street, Haidian District, Beijing 100193, China.
  • §Contact author: npo@princeton.edu

Phys. Rev. Materials 9, L061401 – Published 10 June, 2025

DOI: https://doi.org/10.1103/6gbq-d7jk

Abstract

The layered honeycomb material BaCo2(AsO4)2 is of topical interest because its magnetic state is related to that of the Kitaev magnet α−RuCl3. Using thermal transport to probe how magnetic excitations interact with phonons in the magnetically disordered regime, we have uncovered an unusually large enhancement of the thermal conductivity κxx in an in-plane magnetic field H. Just above the Néel temperature TN, a field of 13 T increases κxx by a factor of ∼211, which is very large compared to other magnetic insulators. Interestingly, κxx(H,T) exhibits a scaling behavior in the entire magnetically disordered region that surrounds the ordered zigzag state. The ratio Δκxx(H,T)/κxx(13,T), measured throughout the disordered region, collapses to a one-parameter scaling function exp(−1/gx) (where x=μBB/kBT and g is a constant).

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