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    Giant topological Hall effect in epitaxial Ni80Fe20/La0.65Sr0.35MnO3 thin film heterostructures

    Kusampal Yadav1, Dilruba Hasina1, Nasiruddin Mondal1, Sayantika Bhowal2,*, and Devajyoti Mukherjee1,†

    • *Contact author: sbhowal@iitb.ac.in
    • †Contact author: sspdm@iacs.res.in

    Phys. Rev. Materials 9, 105003 – Published 30 October, 2025

    DOI: https://doi.org/10.1103/5qr7-s1h8

    Abstract

    The emergence of new physical properties at the interfaces between complex oxides has always been of both fundamental and practical importance. Here, we report the observation of a giant topological Hall resistivity of ∼2.8µΩcm at room temperature in an epitaxial thin-film heterostructure of permalloy (Py, Ni80Fe20) and the half-metallic ferromagnet La0.65Sr0.35MnO3 (LSMO). This large magnitude of the topological Hall effect in the Py/LSMO heterostructure, compared to single-layer Py and LSMO thin films, is attributed to the optimized combination of ferromagnetism in LSMO and the strong spin-orbit-coupling-driven Rashba interaction at the interface. The introduction of a ferroelectric BaTiO3 sandwich layer in the Py/LSMO heterostructure also leads to an enhanced topological Hall resistivity compared to the single-layer Py thin film. Interestingly, magnetic force microscopy measurements reveal skyrmionlike features, suggesting the origin of the topological Hall effect. Our theoretical model calculations for the skyrmion lattice further indicate that the Rashba interaction, driven by the broken inversion symmetry in the Py/LSMO films, can account for the observed changes in the topological Hall effect at the interface. Our work opens the door for the potential use of Py/LSMO thin films in spintronic applications.

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    This article appears in the following collection:

    Magnetic Phenomena at Oxide Interfaces: Fundamentals to Devices

    The Editors of Physical Review Materials are pleased to present the Collection on Magnetic Phenomena at Oxide Interfaces, highlighting cutting-edge advances in oxide interface magnetism and its applications. The Collection is being guest-edited by Lucas Caretta from Brown University (USA) and Jacobo Santamaria from Universidad Complutense de Madrid (Spain). Every article published in this collection underwent a rigorous peer review process, adhering to the same high standards applied to all papers. The Physical Review Materials editorial team managed the peer review and made all editorial decisions.

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