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    Quenching the noncollinear spin order in high-Tc layered ferromagnet Fe5GeTe2

    Rabindra Basnet and Ramesh C. Budhani*

    • *Contact author: ramesh.budhani@morgan.edu

    Phys. Rev. Materials 9, 124412 – Published 18 December, 2025

    DOI: https://doi.org/10.1103/28qv-6dh3

    Abstract

    The realization of long-range spin order in two dimensions (2D) has catapulted the search for layered materials with magnetic ordering above room temperature. These efforts aim to understand and enhance the spin–spin interactions in 2D. An emergent class of such magnets is the layered FeNGeTe2 (N =3, 4, and 5). Here, we investigate the magnetic states over a wide field–temperature phase space in the high-Tc ferromagnet Fe5GeTe2 using magnetization, ferromagnetic resonance (FMR), and magnetotransport measurements. Our findings reveal a magnetic phase transition from a collinear to a complex noncollinear magnetic order near the temperature T*≈160 K, below which magnetic susceptibility is reduced, FMR linewidth broadened, and anomalous Hall resistivity suppressed. Such noncollinearity results from the competition between magnetocrystalline anisotropy and Dzyaloshinskii–Moriya interaction arising from the unusual Fe1 ordering in two possible split sites. Our study focuses on the strategy to quench the noncollinear spin order. Substituting 40% Ni in Fe5GeTe2 is found to be one such quenching strategy. This provides deeper insights into the magnetism of a high-Tc layered ferromagnet, offering opportunities to develop 2D magnet-based devices.

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