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    Epitaxial stabilization of magnetic GdAuSb/LaAuSb superlattices

    Patrick J. Strohbeen1, Soohyun Im2, Tamalika Samanta1, Zachary LaDuca1, Dongxue Du1, Estiaque H. Shourov1, Jessica L. McChesney3, Fanny Rodolakis3, Paul M. Voyles1 et al.

    Jason K. Kawasaki1,*

    • *Contact author: jkawasaki@wisc.edu

    Phys. Rev. Materials 10, 074421 – Published 19 August, 2026

    DOI: https://doi.org/10.1103/18lw-9dl1

    Abstract

    We report the epitaxial stabilization of GdAuSb films and GdAuSb/LaAuSb superlattices via molecular beam epitaxy on (0001)-oriented Al2O3 substrates. GdAuSb crystallizes in the Au-Au dimerized YPtAs structure type (space group P63/mmc), the same structure as the Dirac semimetal LaAuSb. Angle-resolved photoemission spectroscopy (ARPES) measurements show similar near EF bandstructures for GdAuSb and LaAuSb, plus a rigid band shift for GdAuSb toward more holelike behavior and corelike Gd 4f states ∼9eV below the Fermi energy. LaAuSb/GdAuSb superlattices exhibit sharp superlattice fringes by x-ray diffraction and atomically precise interfaces by scanning transmission electron microscopy. Superlattices display two transitions in temperature-dependent resistvity, compared to a single Néel temperature for thick GdAuSb films. Superlattices of LnAuSb materials (Ln= rare earth) with atomically abrupt interfaces offer an epitaxial platform for control of magnetic and topological order via tunable intralayer exchange and reduced dimensionality.

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