We report high-fidelity state readout of a trapped ion qubit using a trap-integrated photon detector. We determine the hyperfine qubit state of a single ${}^9{\mathrm{Be}}^{+}$ ion held in a surface-electrode rf ion trap by counting state-dependent ion fluorescence photons with a superconducting nanowire single-photon detector fabricated into the trap structure. The average readout fidelity is 0.9991(1), with a mean readout duration of $46\mu \mathrm{s}$, and is limited by the polarization impurity of the readout laser beam and by off-resonant optical pumping. Because there are no intervening optical elements between the ion and the detector, we can use the ion fluorescence as a self-calibrated photon source to determine the detector quantum efficiency and its dependence on photon incidence angle and polarization.

Quantum criticality, as a fascinating quantum phenomenon, may provide significant advantages for quantum sensing. Here we propose a dynamic framework for quantum sensing with a family of Hamiltonians that undergo quantum phase transitions (QPTs). By giving the formalism of the quantum Fisher information (QFI) for quantum sensing based on critical quantum dynamics, we demonstrate its divergent feature when approaching the critical point. We illustrate the basic principle and the details of experimental implementation using quantum Rabi model. The framework is applicable to a variety of examples and does not rely on the stringent requirement for particular state preparation or adiabatic evolution. It is expected to provide a route towards the implementation of criticality-enhanced quantum sensing.

We derive a thermodynamic uncertainty relation for general open quantum dynamics, described by a joint unitary evolution on a composite system comprising a system and an environment. By measuring the environmental state after the system-environment interaction, we bound the counting observables in the environment by the survival activity, which reduces to the dynamical activity in classical Markov processes. Remarkably, the relation derived herein holds for general open quantum systems with any counting observable and any initial state. Therefore, our relation is satisfied for classical Markov processes with arbitrary time-dependent transition rates and initial states. We apply our relation to continuous measurement and the quantum walk to find that the quantum nature of the system can enhance the precision. Moreover, we can make the lower bound arbitrarily small by employing appropriate continuous measurement.

We derive geometrical bounds on the irreversibility in both quantum and classical Markovian open systems that satisfy the detailed balance condition. Using information geometry, we prove that irreversible entropy production is bounded from below by a modified Wasserstein distance between the initial and final states, thus strengthening the Clausius inequality in the reversible-Markov case. The modified metric can be regarded as a discrete-state generalization of the Wasserstein metric, which has been used to bound dissipation in continuous-state Langevin systems. Notably, the derived bounds can be interpreted as the quantum and classical speed limits, implying that the associated entropy production constrains the minimum time of transforming a system state. We illustrate the results on several systems and show that a tighter bound than the Carnot bound for the efficiency of quantum heat engines can be obtained.

Spin-orbital-angular-momentum (SOAM) coupling has been realized in recent experiments of Bose-Einstein condensates [Chen et al., Phys. Rev. Lett. 121, 113204 (2018) and Zhang et al., Phys. Rev. Lett. 122, 110402 (2019)], where the orbital angular momentum imprinted upon bosons leads to quantized vortices. For fermions, such an exotic synthetic gauge field can provide fertile ground for fascinating pairing schemes and rich superfluid phases, which are yet to be explored. Here we demonstrate how SOAM coupling stabilizes vortices in Fermi superfluids through a unique mechanism that can be viewed as the angular analog to that of the spin-orbit-coupling-induced Fulde-Ferrell state under a Fermi surface deformation. Remarkably, the vortex size is comparable with the beam waist of Raman lasers generating the SOAM coupling, which is typically much larger than previously observed vortices in Fermi superfluids. With tunable size and core structure, these giant vortex states provide unprecedented experimental access to topological defects in Fermi superfluids.

Optical approaches to quantum computation require the creation of multimode photonic quantum states in a controlled fashion. Here we experimentally demonstrate phase locking of two all-optical quantum memories, based on a concatenated cavity system with phase reference beams, for the time-controlled release of two-mode entangled single-photon states. The release time for each mode can be independently determined. The generated states are characterized by two-mode optical homodyne tomography. Entanglement and nonclassicality are preserved for release-time differences up to 400 ns, confirmed by logarithmic negativities and Wigner-function negativities, respectively.

We introduce a new approach to Gottesman-Kitaev-Preskill (GKP) states that treats their finite-energy version in an exact manner. Based on this analysis, we develop new qubit-oscillator circuits that autonomously stabilize a GKP manifold, correcting errors without relying on qubit measurements. Finally, we show numerically that logical information encoded in GKP states is very robust against typical oscillator noise sources when stabilized by these new circuits.

The performance of quantum key distribution (QKD) is severely limited by multiphoton pulses emitted by laser sources due to the photon-number splitting attack. Coherent-one-way (COW) QKD has been introduced as a promising solution to overcome this limitation, and thus extend the achievable distance of practical QKD. Indeed, thanks to its experimental simplicity, the COW protocol is already used in commercial applications. Here, we derive simple upper security bounds on its secret key rate, which demonstrate that it scales at most quadratically with the system’s transmittance, thus solving a long-standing problem. That is, in contrast to what has been claimed, this approach is inappropriate for long-distance QKD transmission. Remarkably, our findings imply that all implementations of the COW protocol performed so far are insecure.

The theoretical investigation of nonadiabatic processes is hampered by the complexity of the coupled electron-nuclear dynamics beyond the Born-Oppenheimer approximation. Classically, the simulation of such reactions is limited by the unfavorable scaling of the computational resources as a function of the system size. While quantum computing exhibits proven quantum advantage for the simulation of real-time dynamics, the study of quantum algorithms for the description of nonadiabatic phenomena is still unexplored. In this Letter, we propose a quantum algorithm for the simulation of fast nonadiabatic chemical processes together with an initialization scheme for quantum hardware calculations. In particular, we introduce a first-quantization method for the time evolution of a wave packet on two coupled harmonic potential energy surfaces (Marcus model). In our approach, the computational resources scale polynomially in the system dimensions, opening up new avenues for the study of photophysical processes that are classically intractable.

As two valuable quantum resources, Einstein-Podolsky-Rosen entanglement and steering play important roles in quantum-enhanced communication protocols. Distributing such quantum resources among multiple remote users in a network is a crucial precondition underlying various quantum tasks. We experimentally demonstrate the deterministic distribution of two- and three-mode Gaussian entanglement and steering by transmitting separable states in a network consisting of a quantum server and multiple users. In our experiment, entangled states are not prepared solely by the quantum server, but are created among independent users during the distribution process. More specifically, the quantum server prepares separable squeezed states and applies classical displacements on them before spreading out, and users simply perform local beam-splitter operations and homodyne measurements after they receive separable states. We show that the distributed Gaussian entanglement and steerability are robust against channel loss. Furthermore, one-way Gaussian steering is achieved among users that is useful for further directional or highly asymmetric quantum information processing.

Self-testing is a procedure for characterizing quantum resources with the minimal level of trust. Up to now it has been used as a device-independent certification tool for particular quantum measurements, channels, and pure entangled states. In this work we introduce the concept of self-testing more general entanglement structures. More precisely, we present the first self-tests of an entangled subspace—the five-qubit code and the toric code. We show that all quantum states maximally violating a suitably chosen Bell inequality must belong to the corresponding code subspace, which remarkably includes also mixed states.

Thermodynamic uncertainty relations yield a lower bound on entropy production in terms of the mean and fluctuations of a current. We derive their general form for systems under arbitrary time-dependent driving from arbitrary initial states and extend these relations beyond currents to state variables. The quality of the bound is discussed for various types of observables for an interacting pair of colloidal particles in a moving laser trap and for the dynamical unfolding of a small protein. Since the input for evaluating these bounds does not require specific knowledge of the system or its coupling to the time-dependent control, they should become widely applicable tools for thermodynamic inference in time-dependently driven systems.

Spin glasses and many-body localization (MBL) are prime examples of ergodicity breaking, yet their physical origin is quite different: the former phase arises due to rugged classical energy landscape, while the latter is a quantum-interference effect. Here, we study quantum dynamics of an isolated 1D spin glass under application of a transverse field. At high energy densities, the system is ergodic, relaxing via a resonance avalanche mechanism, that is also responsible for the destruction of MBL in nonglassy systems with power-law interactions. At low energy densities, the interaction-induced fields obtain a power-law soft gap, making the resonance avalanche mechanism inefficient. This leads to the persistence of the spin-glass order, as demonstrated by resonance analysis and by numerical studies. A small fraction of resonant spins forms a thermalizing system with long-range entanglement, making this regime distinct from the conventional MBL. The model considered can be realized in systems of trapped ions, opening the door to investigating slow quantum dynamics induced by glassiness.

Photonic quantum memory is the core element in quantum information processing (QIP). For the scalable and convenient practical applications, great efforts have been devoted to the integrated quantum memory based on various waveguides fabricated in solids. However, on-demand storage of qubits, which is an essential requirement for QIP, is still challenging to be implemented using such integrated quantum memory. Here we report the on-demand storage of time-bin qubits in an on-chip waveguide memory fabricated on the surface of a ${{}^{151}\mathrm{Eu}}^{3+}:{\mathrm{Y}}_2\mathrm{Si}{\mathrm{O}}_5$ crystal, utilizing the Stark-modulated atomic frequency comb protocol. A qubit storage fidelity of $99.3\%\pm 0.2\%$ is obtained with single-photon-level coherent pulses, far beyond the highest fidelity achievable using the classical measure-and-prepare strategy. The developed integrated quantum memory with the on-demand retrieval capability represents an important step toward practical applications of integrated quantum nodes in quantum networks.

The famous Kibble-Zurek mechanism offers us a significant clue to study quantum phase transitions out of equilibrium. Here, we investigate an intriguing phenomenon of a spin-orbit coupled Bose-Einstein condensate by quenching the Raman coupling strength from a high-symmetry phase (nonmagnetic phase) to a low-symmetry phase (magnetic phase). When crossing the critical point, the fluctuation of momentum distribution leads to delayed bifurcation structures. Simultaneously, the domain information emerges in momentum space. Moreover, the universal scalings of spatiotemporal dynamics are extracted from the fluctuations and domains, which manifests homogeneous and inhomogeneous Kibble-Zurek power laws at different timescales. Our work demonstrates a paradigmatic study on the inhomogeneous Kibble-Zurek mechanism.

The quantum approximate optimization algorithm (QAOA) employs variational states generated by a parameterized quantum circuit to maximize the expected value of a Hamiltonian encoding a classical cost function. Whether or not the QAOA can outperform classical algorithms in some tasks is an actively debated question. Our work exposes fundamental limitations of the QAOA resulting from the symmetry and the locality of variational states. A surprising consequence of our results is that the classical Goemans-Williamson algorithm outperforms the QAOA for certain instances of MaxCut, at any constant level. To overcome these limitations, we propose a nonlocal version of the QAOA and give numerical evidence that it significantly outperforms the standard QAOA for frustrated Ising models.

The Nambu-Goldstone (NG) modes in a nonrelativistic system can be classified into two types from their characteristic features: being of either an odd (type I) or an even (type II) power energy-momentum dispersion. Conventionally, the type-II NG modes may universally arise from spontaneous breaking of noncommutative symmetry pairs. Here, we predict a novel type of quadratically dispersed NG modes that emerges in mixed $s$ and $p$ band Bose superfluids in an optical lattice and, unlike the conventional type-II NG modes, cannot be solely interpreted with the celebrated symmetry-based argument. Instead, we show that the existence of such modes has a profound connection to the topological transition on projective complex order-parameter space. The detection scheme is also proposed. Our Letter reveals a new universal mechanism for emergence of type-II NG modes, which bridges intrinsically the Landau symmetry-breaking and topological theories.

Effective and efficient forecasting relies on identification of the relevant information contained in past observations—the predictive features—and isolating it from the rest. When the future of a process bears a strong dependence on its behavior far into the past, there are many such features to store, necessitating complex models with extensive memories. Here, we highlight a family of stochastic processes whose minimal classical models must devote unboundedly many bits to tracking the past. For this family, we identify quantum models of equal accuracy that can store all relevant information within a single two-dimensional quantum system (qubit). This represents the ultimate limit of quantum compression and highlights an immense practical advantage of quantum technologies for the forecasting and simulation of complex systems.