It is well known that the ground state energy of many-particle Hamiltonians involving only 2-body interactions can be obtained using constrained optimizations over density matrices which arise from reducing an $N$-particle state. While determining which 2-particle density matrices are “$N$-representable” is a computationally hard problem, all known extreme $N$-representable 2-particle reduced density matrices arise from a unique $N$-particle preimage, satisfying a conjecture established in 1972. We present explicit counterexamples to this conjecture through giving Hamiltonians with 2-body interactions which have degenerate ground states that cannot be distinguished by any 2-body operator. We relate the existence of such counterexamples to quantum error correction codes and topologically ordered spin systems.

We continuously measure the state of a superconducting quantum bit coupled to a microwave readout cavity by using a fast, ultralow-noise parametric amplifier. This arrangement allows us to observe quantum jumps between the qubit states in real time, and should enable quantum error correction and feedback—essential components of quantum information processing.

We propose and demonstrate a scheme for boosting the efficiency of entanglement distribution based on a decoherence-free subspace over lossy quantum channels. By using backward propagation of a coherent light, our scheme achieves an entanglement-sharing rate that is proportional to the transmittance $T$ of the quantum channel in spite of encoding qubits in multipartite systems for the decoherence-free subspace. We experimentally show that highly entangled states, which can violate the Clauser-Horne-Shimony-Holt inequality, are distributed at a rate proportional to $T$.

Electron spin qubits in molecular systems offer high reproducibility and the ability to self-assemble into larger architectures. However, interactions between neighboring qubits are “always on,” and although the electron spin coherence times can be several hundred microseconds, these are still much shorter than typical times for nuclear spins. Here we implement an electron-nuclear hybrid scheme which uses coherent transfer between electron and nuclear spin degrees of freedom in order to both effectively turn on or off interqubit coupling mediated by dipolar interactions and benefit from the long nuclear spin decoherence times ($T_{2n}$). We transfer qubit states between the electron and ${}^{15}\mathrm{N}$ nuclear spin in ${}^{15}\mathrm{N}@{\mathrm{C}}_{60}$ with a two-way process fidelity of 88%, using a series of tuned microwave and radio frequency pulses and measure a nuclear spin coherence lifetime of over 100 ms.

We present and experimentally demonstrate a communication protocol that employs shared entanglement to reduce errors when sending a bit over a particular noisy classical channel. Specifically, it is shown that given a single use of this channel, one can transmit a bit with higher success probability when the sender and receiver share entanglement compared to the best possible strategy when they do not. The experiment is realized using polarization-entangled photon pairs, whose quantum correlations play a critical role in both the encoding and decoding of the classical message. Experimentally, we find that a bit can be successfully transmitted with probability $0.891\pm 0.002$, which is close to the theoretical maximum of $(2+2^{-1/2})/3\approx 0.902$ and is significantly above the optimal classical strategy, which yields $5/6\approx 0.833$.

Optical vortices are lines of phase singularity which percolate through all optical fields. We report the entanglement of linked optical vortex loops in the light produced by spontaneous parametric down-conversion. As measured by using a Bell inequality, this entanglement between topological features extends over macroscopic and finite volumes. The entanglement of photons in complex three-dimensional topological states suggests the possibility of entanglement of similar features in other quantum systems describable by complex scalar functions, such as superconductors, superfluids, and Bose-Einstein condensates.

The 6.7 and 12.2 GHz masers, corresponding to the $5_1\to 6_0{A}^{+}$ and $2_0\to 3_{-1}E$ transitions in methanol (${\mathrm{CH}}_3\mathrm{OH}$), respectively, are among the brightest radio objects in the sky. We present calculations for the sensitivity of these and other transitions in the ground state of methanol to a variation of the proton-to-electron mass ratio. We show that the sensitivity is greatly enhanced due to a cancellation of energies associated with the hindered internal rotation and the overall rotation of the molecule. We find sensitivities of $K_{\mu }=-42$ and $K_{\mu }=-33$, for the $5_1\to 6_0{A}^{+}$ and $2_0\to 3_{-1}E$ transitions, respectively. The sensitivities of other transitions in the different isotopologues of methanol range from $-88$ to 330. This makes methanol a sensitive probe for spatial and temporal variations of the proton-to-electron mass ratio.

If nonlocality is to be inferred from a violation of Bell’s inequality, an important assumption is that the measurement settings are freely chosen by the observers, or alternatively, that they are random and uncorrelated with the hypothetical local variables. We demonstrate a connection between models that weaken this assumption, allowing partial correlation, and (i) models that allow classical communication between the distant parties, (ii) models that exploit the detection loophole. Even if Bob’s choices are completely independent, all correlations from projective measurements on a singlet can be reproduced, with mutual information between Alice’s choice and local variables less than or equal to one bit.

Magnetic fields as weak as Earth’s may affect the outcome of certain photochemical reactions that go through a radical pair intermediate. When the reaction environment is anisotropic, this phenomenon can form the basis of a chemical compass and has been proposed as a mechanism for animal magnetoreception. Here, we demonstrate how to optimize the design of a chemical compass with a much better directional sensitivity simply by a gradient field, e.g., from a magnetic nanostructure. We propose an experimental test of these predictions, and suggest design principles for a hybrid metallic-organic chemical compass. In addition to the practical interest in designing a biomimetic weak magnetic field sensor, our result shows that gradient fields can serve as powerful tools to probe spin correlations in radical pair reactions.

We propose an experiment to directly probe the non-Abelian statistics of Majorana fermions by braiding them in an $s$-wave superfluid of ultracold atoms. We show that different orders of braiding operations give orthogonal output states that can be distinguished through Raman spectroscopy. Realization of Majorana states in an $s$-wave superfluid requires strong spin-orbital coupling and a controllable Zeeman field in the perpendicular direction. We present a simple laser configuration to generate the artificial spin-orbital coupling and the required Zeeman field in the dark-state subspace.

We extend the concept of an entanglement spectrum from the geometrical to the particle bipartite partition. We apply this to several fractional quantum Hall wave functions on both sphere and torus geometries to show that this new type of entanglement spectra completely reveals the physics of bulk quasihole excitations. While this is easily understood when a local Hamiltonian for the model state exists, we show that the quasihole wave functions are encoded within the model state even when such a Hamiltonian is not known. As a nontrivial example, we look at Jain’s composite fermion states and obtain their quasiholes directly from the model state wave function. We reach similar conclusions for wave functions described by Jack polynomials.

The resources required to characterize the dynamics of engineered quantum systems—such as quantum computers and quantum sensors—grow exponentially with system size. Here we adapt techniques from compressive sensing to exponentially reduce the experimental configurations required for quantum process tomography. Our method is applicable to processes that are nearly sparse in a certain basis and can be implemented using only single-body preparations and measurements. We perform efficient, high-fidelity estimation of process matrices of a photonic two-qubit logic gate. The database is obtained under various decoherence strengths. Our technique is both accurate and noise robust, thus removing a key roadblock to the development and scaling of quantum technologies.

We address the question of whether superfluidity can survive in the case of fermion pairing between different species with mismatched Fermi surfaces using as an example a population-imbalanced mixture of ${}^6\mathrm{Li}$ atomic Fermi gas loaded in a two-dimensional optical lattice at nonzero temperatures. The collective mode is calculated from the Bethe-Salpeter equations in the general random phase approximation assuming a Fulde-Ferrell order parameter. The numerical solution shows that, in addition to low-energy (Goldstone) mode, two rotonlike minima exist, and therefore, the superfluidity can survive in this imbalanced system.

We consider the Kane-Mele model supplemented by a Hubbard $U$ term. The phase diagram is mapped out using projective auxiliary field quantum Monte Carlo simulations. The quantum spin liquid of the Hubbard model is robust against weak spin-orbit interaction, and is not adiabatically connected to the spin-Hall insulating state. Beyond a critical value of $U>U_c$ both states are unstable toward magnetic ordering. In the quantum spin-Hall state we study the spin, charge, and single-particle dynamics of the helical Luttinger liquid by retaining the Hubbard interaction only on a ribbon edge. The Hubbard interaction greatly suppresses charge currents along the edge and promotes edge magnetism but leaves the single-particle signatures of the helical liquid intact.

We derive a quantum Cramér-Rao bound (QCRB) on the error of estimating a time-changing signal. The QCRB provides a fundamental limit to the performance of general quantum sensors, such as gravitational-wave detectors, force sensors, and atomic magnetometers. We apply the QCRB to the problem of force estimation via continuous monitoring of the position of a harmonic oscillator, in which case the QCRB takes the form of a spectral uncertainty principle. The bound on the force-estimation error can be achieved by implementing quantum noise cancellation in the experimental setup and applying smoothing to the observations.

We demonstrate that non-Abelian rotations within the degenerate ground-state manifold of a set of Majorana fermions can be realized by the addition or removal of single electrons, and propose an implementation using Coulomb blockaded quantum dots. The exchange of electrons generates rotations similar to braiding, though not in real space. Unlike braiding operations, rotations by a continuum of angles are possible, while still being partially robust against perturbations. The quantum dots can also be used for readout of the state of the Majorana system via a charge measurement.

We consider a basic model of digital memory where each cell is composed of a reflecting medium with two possible reflectivities. By fixing the mean number of photons irradiated over each memory cell, we show that a nonclassical source of light can retrieve more information than any classical source. This improvement is shown in the regime of few photons and high reflectivities, where the gain of information can be surprising. As a result, the use of quantum light can have nontrivial applications in the technology of digital memories, such as optical disks and barcodes.

We introduce a procedure to infer the interactions among a set of binary variables, based on their sampled frequencies and pairwise correlations. The algorithm builds the clusters of variables contributing most to the entropy of the inferred Ising model and rejects the small contributions due to the sampling noise. Our procedure successfully recovers benchmark Ising models even at criticality and in the low temperature phase, and is applied to neurobiological data.

We carry out a detailed study of the motion of particles driven by a constant external force over a landscape consisting of a periodic potential corrugated by a small amount of spatial disorder. We observe anomalous behavior in the form of subdiffusion and superdiffusion and even subtransport over very long time scales. Recent studies of transport over slightly random landscapes have focused only on parameters leading to normal behavior, and while enhanced diffusion has been identified when the external force approaches the critical value associated with the transition from locked to running solutions, the regime of anomalous behavior had not been recognized. We provide a qualitative explanation for the origin of these anomalies, and make connections with a continuous time random walk approach.

We introduce a family of Hamiltonian systems for measurement-based quantum computation with continuous variables. The Hamiltonians (i) are quadratic, and therefore two body, (ii) are of short range, (iii) are frustration-free, and (iv) possess a constant energy gap proportional to the squared inverse of the squeezing. Their ground states are the celebrated Gaussian graph states, which are universal resources for quantum computation in the limit of infinite squeezing. These Hamiltonians constitute the basic ingredient for the adiabatic preparation of graph states and thus open new venues for the physical realization of continuous-variable quantum computing beyond the standard optical approaches. We characterize the correlations in these systems at thermal equilibrium. In particular, we prove that the correlations across any multipartition are contained exactly in its boundary, automatically yielding a correlation area law.