We establish the fluctuation theorem in the presence of information exchange between a nonequilibrium system and other degrees of freedom such as an observer and a feedback controller, where the amount of information exchange is added to the entropy production. The resulting generalized second law sets the fundamental limit of energy dissipation and energy cost during the information exchange. Our results apply not only to feedback-controlled processes but also to a much broader class of information exchanges, and provide a unified framework of nonequilibrium thermodynamics of measurement and feedback control.

In this Letter, we compute an analogue of Tsirelson’s bound for Hardy’s test of nonlocality, that is, the maximum violation of locality constraints allowed by the quantum formalism, irrespective of the dimension of the system. The value is found to be the same as the one achievable already with two-qubit systems, and we show that only a very specific class of states can lead to such maximal value, thus highlighting Hardy’s test as a device-independent self-test protocol for such states. By considering realistic constraints in Hardy’s test, we also compute device-independent upper bounds on this violation and show that these bounds are saturated by two-qubit systems, thus showing that there is no advantage in using higher-dimensional systems in experimental implementations of such a test.

Recent progress on micro- and nanometer-scale manipulation has opened the possibility to probe systems small enough that thermal fluctuations of energy and coordinate variables can be significant compared with their mean behavior. We present an experimental study of nonequilibrium thermodynamics in a classical two-state system, namely, a metallic single-electron box. We have measured with high statistical accuracy the distribution of dissipated energy as single electrons are transferred between the box electrodes. The obtained distributions obey Jarzynski and Crooks fluctuation relations. A comprehensive microscopic theory exists for the system, enabling the experimental distributions to be reproduced without fitting parameters.

We propose a novel class of atomic clocks based on highly charged ions. We consider highly forbidden laser-accessible transitions within the $4f^{12}$ ground-state configurations of highly charged ions. Our evaluation of systematic effects demonstrates that these transitions may be used for building exceptionally accurate atomic clocks which may compete in accuracy with recently proposed nuclear clocks.

We present a general theory of non-Markovian dynamics for open systems of noninteracting fermions (bosons) linearly coupled to thermal environments of noninteracting fermions (bosons). We explore the non-Markovian dynamics by connecting the exact master equations with the nonequilibirum Green’s functions. Environmental backactions are fully taken into account. The non-Markovian dynamics consists of nonexponential decays and dissipationless oscillations. Nonexponential decays are induced by the discontinuity in the imaginary part of the self-energy corrections. Dissipationless oscillations arise from band gaps or the finite band structure of spectral densities. The exact analytic solutions for various non-Markovian thermal environments show that non-Markovian dynamics can be largely understood from the environmental-modified spectra of open systems.

We study nonequilibrium phase transitions in the presence of disorder that locally breaks the symmetry between two equivalent macroscopic states. In low-dimensional equilibrium systems, such random-field disorder is known to have dramatic effects: it prevents spontaneous symmetry breaking and completely destroys the phase transition. In contrast, we show that the phase transition of the one-dimensional generalized contact process persists in the presence of random-field disorder. The ultraslow dynamics in the symmetry-broken phase is described by a Sinai walk of the domain walls between two different absorbing states. We discuss the generality and limitations of our theory, and we illustrate our results by large-scale Monte Carlo simulations.

We study quantum states produced by optimal phase covariant quantum cloners. We argue that cloned quantum superpositions are not macroscopic superpositions in the spirit of Schrödinger’s cat, despite their large particle number. This is indicated by calculating several measures for macroscopic superpositions from the literature, as well as by investigating the distinguishability of the two superposed cloned states. The latter rapidly diminishes when considering imperfect detectors or noisy states and does not increase with the system size. In contrast, we find that cloned quantum states themselves are macroscopic, in the sense of both proposed measures and their usefulness in quantum metrology with an optimal scaling in system size. We investigate the applicability of cloned states for parameter estimation in the presence of different kinds of noise.

Quantum computation that combines the coherence stabilization virtues of decoherence-free subspaces and the fault tolerance of geometric holonomic control is of great practical importance. Some schemes of adiabatic holonomic quantum computation in decoherence-free subspaces have been proposed in the past few years. However, nonadiabatic holonomic quantum computation in decoherence-free subspaces, which avoids a long run-time requirement but with all the robust advantages, remains an open problem. Here, we demonstrate how to realize nonadiabatic holonomic quantum computation in decoherence-free subspaces. By using only three neighboring physical qubits undergoing collective dephasing to encode one logical qubit, we realize a universal set of quantum gates.

We examine numerically the zero-temperature ($2+1$)-dimensional directed polymer in a random medium, along with several of its brethren via the Kardar-Parisi-Zhang (KPZ) equation. Using finite-size and KPZ scaling Ansätze, we extract the universal distributions controlling fluctuation phenomena in this canonical model of nonequilibrium statistical mechanics. Specifically, we study point-point, point-line, and point-plane directed polymer geometries, scenarios which yield higher-dimensional analogs of the Tracy-Widom distributions of random matrix theory. Our analysis represents a robust, multifaceted numerical characterization of the $2+1$ KPZ universality class and its limit distributions.

Nonequilibrium systems are often characterized by the transport of some quantity at a macroscopic scale, such as, for instance, a current of particles through a wire. The asymmetric simple exclusion process (ASEP) is a paradigm for nonequilibrium transport that is amenable to exact analytical solution. In the present work, we determine the full statistics of the current in the finite size open ASEP for all values of the parameters. Our exact analytical results are checked against numerical calculations using density matrix renormalization group techniques.

In nonrelativistic quantum mechanics, measurements performed by separate observers are modeled via tensor products. In algebraic quantum field theory, though, local observables corresponding to spacelike separated parties are just required to commute. The problem of determining whether these two definitions of separation lead to the same set of bipartite correlations is known in nonlocality as Tsirelson’s problem. In this article, we prove that the analog of Tsirelson’s problem in steering scenarios is false. That is, there exists a steering inequality that can or cannot be violated depending on how we define spacelike separation at the operator level.

We describe a simple entangling principle based on the scattering of photons off single emitters in one-dimensional waveguides (or extremely lossy cavities). The scheme can be applied to polarization- or time bin-encoded photonic qubits, and features a filtering mechanism that works effectively as a built-in error-correction directive. This automatically maps imperfections from the dominant sources of errors into heralded losses instead of infidelities, something highly advantageous, for instance, in quantum information applications. The scheme is thus adequate for high-fidelity maximally entangling gates even in the weak-coupling regime. These, in turn, can be directly used to store and retrieve photonic-qubit states, thereby completing an atom-photon interface toolbox, or applied to sequential measurement-based quantum computations with atomic memories.

With the advent of quantum information, the violation of a Bell inequality is used to witness the absence of an eavesdropper in cryptographic scenarios such as key distribution and randomness expansion. One of the key assumptions of Bell’s theorem is the existence of experimental “free will,” meaning that measurement settings can be chosen at random and independently by each party. The relaxation of this assumption potentially shifts the balance of power towards an eavesdropper. We consider a no-signaling model with reduced “free will” and bound the adversary’s capabilities in the task of randomness expansion.

An algorithm is presented for error correction in the surface code quantum memory. This is shown to correct depolarizing noise up to a threshold error rate of 18.5%, exceeding previous results and coming close to the upper bound of 18.9%. The time complexity of the algorithm is found to be polynomial with error suppression, allowing efficient error correction for codes of realistic sizes.

We study the statistics of the work done, fluctuation relations, and irreversible entropy production in a quantum many-body system subject to the sudden quench of a control parameter. By treating the quench as a thermodynamic transformation we show that the emergence of irreversibility in the nonequilibrium dynamics of closed many-body quantum systems can be accurately characterized. We demonstrate our ideas by considering a transverse quantum Ising model that is taken out of equilibrium by an instantaneous change of the transverse field.

The hair bundle of sensory cells in the vertebrate ear provides an example of a noisy oscillator close to a Hopf bifurcation. The analysis of the data from both spontaneous and forced oscillations shows a strong violation of the fluctuation-dissipation theorem, revealing the presence of an underlying active process that keeps the system out of equilibrium. Nevertheless, we show that a generalized fluctuation-dissipation theorem, valid for nonequilibrium steady states, is fulfilled within the limits of our experimental accuracy and computational approximations, when the adequate conjugate degrees of freedom are chosen.

The ${}^{229}\mathrm{Th}$ nucleus possesses the lowest-energy nuclear isomeric state. Two widely accepted indirect measurements of the transition energy place it within reach of existing laser capabilities. Direct searches for the isomer deexcitation have proven elusive despite extensive effort over the past couple of decades. There is now a growing interest in finding this unique transition because of its potential applications in nuclear, atomic, condensed matter, and optical physics, quantum information, metrology, and cosmology, including the development of a new type of clock based on this nuclear transition. In this Letter we report the first direct observation of the deexcitation of the lowest-lying isomeric state in ${}^{229}\mathrm{Th}$. By collecting ${}^{229}\mathrm{Th}$ recoils following the alpha decay of ${}^{233}\mathrm{U}$ into ${\mathrm{MgF}}_2$ plates and measuring the subsequent light emission, we have isolated the isomer deexcitation and measured the transition’s half-life to be $6\pm 1\mathrm{h}$. Through comparison measurements with ${}^{235\mathrm{m}}\mathrm{U}$ isomer, we found that the observed ${}^{229\mathrm{m}}\mathrm{Th}$ deexcitation signal originates from photon emission rather than internal conversion electron emission. This discovery lays the groundwork for optical and laser spectroscopy of ${}^{229\mathrm{m}}\mathrm{Th}$ nuclear isomer and the development of a ${}^{229}\mathrm{Th}$ nuclear clock.

A fundamental task in modern cryptography is the joint computation of a function which has two inputs, one from Alice and one from Bob, such that neither of the two can learn more about the other’s input than what is implied by the value of the function. In this Letter, we show that any quantum protocol for the computation of a classical deterministic function that outputs the result to both parties (two-sided computation) and that is secure against a cheating Bob can be completely broken by a cheating Alice. Whereas it is known that quantum protocols for this task cannot be completely secure, our result implies that security for one party implies complete insecurity for the other. Our findings stand in stark contrast to recent protocols for weak coin tossing and highlight the limits of cryptography within quantum mechanics. We remark that our conclusions remain valid, even if security is only required to be approximate and if the function that is computed for Bob is different from that of Alice.

We provide quantitative bounds on the characterization of multiparticle separable states by states that have locally symmetric extensions. The bounds are derived from two-particle bounds and relate to recent studies on quantum versions of de Finetti’s theorem. We discuss algorithmic applications of our results, in particular a quasipolynomial-time algorithm to decide whether a multiparticle quantum state is separable or entangled (for constant number of particles and constant error in the norm induced by one-way local operations and classical communication, or in the Frobenius norm). Our results provide a theoretical justification for the use of the search for symmetric extensions as a test for multiparticle entanglement.

Analytic expressions that describe Casimir interactions over the entire range of separations have been limited to planar surfaces. Here we derive analytic expressions for the classical or high-temperature limit of Casimir interactions between two spheres (interior and exterior configurations), including the sphere-plane geometry as a special case, using bispherical coordinates. We consider both Dirichlet boundary conditions and metallic boundary conditions described by the Drude model. At short distances, closed-form expansions are derived from the exact result, displaying an intricate structure of deviations from the commonly employed proximity force approximation.