We demonstrate fully phase-matched high harmonic emission spanning the water window spectral region important for nano- and bioimaging and a breadth of materials and molecular dynamics studies. We also generate the broadest bright coherent bandwidth ($\approx 300\mathrm{eV}$) to date from any light source, small or large, that is consistent with a single subfemtosecond burst. The harmonic photon flux at 0.5 keV is ${10}^3$ higher than demonstrated previously. This work extends bright, spatially coherent, attosecond pulses into the soft x-ray region for the first time.

This Letter reports physical realization of acoustic metamaterials with anisotropic mass density. These metamaterials consist of a superlattice of two fluidlike components radially periodic. Several structures are spectroscopically characterized at large wavelengths (homogenization limit) by studying the acoustic resonances existing in the circular cavity where they are embedded. This characterization method allows us to extract the diagonal components of the sound speed tensor. Analytical expressions describing the anisotropic behavior as a function of the corrugation parameter are also developed and their predictions are in agreement with measurements.

In this Letter, we propose a composite nanochannel system, where half of the channel is of low surface energy, while the other half has a relatively high surface energy. Molecular dynamics simulations show that fluids in such channels can be continuously driven by a symmetric temperature gradient. In the low surface energy part, the fluid moves from high to low temperature, while the fluid migrates from low to high temperature in the high surface energy part. The mechanisms that govern the flow are explained and the conditions required to guarantee the flow and the possible applications are discussed.

We demonstrate, theoretically and experimentally, self-trapping of optical beams in nanoparticle suspensions by virtue of thermophoresis. We use light to control the local concentration of nanoparticles, and increase their density at the center of the optical beam, thereby increasing the effective refractive index in the beam vicinity, causing the beam to self-trap.

Superfluidity, the ability of a fluid to move without dissipation, is one of the most spectacular manifestations of the quantum nature of matter. We explore here the possibility of superfluid motion of light. Controlling the speed of a light packet with respect to a defect, we demonstrate the presence of superfluidity and, above a critical velocity, its breakdown through the onset of a dissipative phase. We describe a possible experimental realization based on the transverse motion through an array of waveguides. These results open new perspectives in transport optimization.

We predict quantum correlations between noninteracting particles evolving simultaneously in a disordered medium. While the particle density follows the single-particle dynamics and exhibits Anderson localization, the two-particle correlation develops unique features that depend on the quantum statistics of the particles and their initial separation. On short time scales, the localization of one particle becomes dependent on whether or not the other particle is localized. On long time scales, the localized particles show oscillatory correlations within the localization length. These effects can be observed in Anderson localization of nonclassical light and ultracold atoms.

We consider how all-angle negative refraction may be induced in anisotropic crystals by making use of the phonon response. We investigate the example of crystal quartz at far-infrared wavelengths. Reflection and transmission measurements confirm the expected behavior, and show relatively high transmission efficiency at frequencies at which negative refraction occurs.

We introduce a class of optical media based on adiabatically modulated, dielectric-only, and potentially extremely low-loss, photonic crystals (PC). The media we describe represent a generalization of the eikonal limit of transformation optics (TO). The basis of the concept is the possibility to fit some equal frequency surfaces of certain PCs with elliptic surfaces, allowing them to mimic the dispersion relation of light in anisotropic effective media. PC cloaks and other TO devices operating at visible wavelengths can be constructed from optically transparent substances such as glasses, whose attenuation coefficient can be as small as 10 dB/km, suggesting the TO design methodology can be applied to the development of optical devices not limited by the losses inherent to metal-based, passive metamaterials.

Light transport in superdiffusive media of finite size is studied theoretically. The intensity Green’s function for a slab geometry is found by discretizing the fractional diffusion equation and employing the eigenfunction expansion method. Truncated step length distributions and complex boundary conditions are considered. The profile of a coherent backscattering cone is calculated in the superdiffusion approximation.

We report on the formation and sustainment of liquid columns with aspect ratios much larger than the value at the onset of the Rayleigh-Plateau instability. This is achieved by using the passive feedback of the radiation pressure applied on the column surface by an acoustic beam injected at the upper end of the column and guided along it. We develop an analytical model that describes the coupling between the acoustic wave guiding and the balance between acoustic and capillary surface forces exerted on the column surface and find a satisfactory agreement with the experiment.

Colloidal thin films of varying rigidity detaching from a substrate under an electric field induced stress are studied by video microscopy. For soft films, the process of detachment shows single-particle dynamics, analogous to desorption. For rigid films, a collective delamination spanning hundreds of particles occurs. A competition among the rigidity of the film, the interaction with the substrate, and the external stress leads to a correlation length over which the film delaminates at a critical stress. The phenomenon is described as a dynamical transition in a disordered elastic medium.

We propose a kind of plasmonic whispering-gallery mode highly localized on the exterior surface of a metal-coated microresonator. This exterior (EX) surface mode possesses high quality factors at room temperature, and can be efficiently excited by a tapered fiber. The EX mode can couple to an interior (IN) mode and this coupling produces a strong anticrossing behavior, which not only allows conversion of IN to EX modes, but also forms a long-lived antisymmetric mode. As a potential application, the EX mode could be used for a biosensor with a sensitivity high of up to 500 nm per refraction index unit, a large figure of merit, and a wide detection range.

We use a glass-based microfluidic device to study the electric current behavior of an electrospray process in the presence of a coflowing liquid. The current shows strong voltage dependence and weak flow rate dependence, in stark contrast to classical electrospray. By considering that the current is dominated by convection near the apex of the conical meniscus and driven by tangential electric stresses, we quantitatively capture the voltage and flow rate dependence of the current. Our results elucidate the influence of external field strength and open the way to achieve robust electric control of the current and of the drop size in microfluidics.

We report the observation of a novel nonlinear optoacoustic phenomenon, that we name forward stimulated interpolarization scattering. When two frequency-offset laser signals are colaunched into orthogonally polarized guided modes of a birefringent small-core ($1.8\mu \mathrm{m}$ diameter) photonic crystal fiber, a pattern of axially moving polarization fringes is produced, with a velocity and spacing that depends on the frequency offset. At values of frequency offset in the few-GHz range, the pattern of moving fringes can perfectly match the phase velocity and axial wavelength (3.9 mm) of the torsional-radial acoustic mode tightly guided in the core. An intense optoacoustic interaction ensues, leading to efficient nonlinear exchange of power from the higher frequency (pump) mode to the orthogonally polarized lower frequency (Stokes) mode. A full-vectorial theory is developed to explain the observations.

The binary path selection of droplets reaching a $T$ junction is regulated by time-delayed feedback and nonlinear couplings. Such mechanisms result in complex dynamics of droplet partitioning: numerous discrete bifurcations between periodic regimes are observed. We introduce a model based on an approximation that makes this problem tractable. This allows us to derive analytical formulae that predict the occurrence of the bifurcations between consecutive regimes, establish selection rules for the period of a regime, and describe the evolutions of the period and complexity of droplet pattern in a cycle with the key parameters of the system. We discuss the validity and limitations of our model which describes semiquantitatively both numerical simulations and microfluidic experiments.

Linear transient growth analysis is commonly used to suggest the structure of disturbances which are particularly efficient in triggering transition to turbulence in shear flows. We demonstrate that the addition of nonlinearity to the analysis can substantially change the prediction made in pipe flow from simple two-dimensional streamwise rolls to a spanwise and cross-stream localized three-dimensional state. This new nonlinear optimal is demonstrably more efficient in triggering turbulence than the linear optimal indicating that there are better ways to design perturbations to achieve transition.

The phase description is a powerful tool for analyzing noisy limit-cycle oscillators. The method, however, has found only limited applications so far, because the present theory is applicable only to Gaussian noise while noise in the real world often has non-Gaussian statistics. Here, we provide the phase reduction method for limit-cycle oscillators subject to general, colored and non-Gaussian, noise including a heavy-tailed one. We derive quantifiers like mean frequency, diffusion constant, and the Lyapunov exponent to confirm consistency of the results. Applying our results, we additionally study a resonance between the phase and noise.

The ability to determine static and (hydro)dynamic properties of carbon nanotubes (CNTs) is crucial for many applications. While their static properties (e.g., solubility and wettability) are fairly well understood, their mechanical responses (e.g., deflection under shear) to ambient fluid flow are to a large extent unknown. We analyze the elastic response of single-walled CNT forests, attached to the bottom wall of a channel, to the aerodynamic loading exerted by both laminar and turbulent flows. Our analysis yields analytical expressions for velocity distributions, the drag coefficient, and bending profiles of individual CNTs. This enables us to determine flexural rigidity of CNTs in wind-tunnel experiments. The model predictions agree with laboratory experiments for a large range of channel velocities.

We report on the observation of a mode-locked laser generated with a crystalline whispering gallery mode resonator pumped with a continuous wave laser. Optical pumping of the resonator generates an optical frequency comb with phase locked components at the Raman offset of the resonator host material. Phase locking of the modes is confirmed via measurement of the radio-frequency beat note produced by the comb on a fast photodiode. Neither the conventional Kerr comb nor hyperparametric oscillation is observed when the comb is present. We present a theoretical explanation of the effect.

We study high-order harmonic generation in aligned molecules close to the ionization threshold. Two distinct contributions to the harmonic signal are observed, which show very different responses to molecular alignment and ellipticity of the driving field. We perform a classical electron trajectory analysis, taking into account the significant influence of the Coulomb potential on the strong-field-driven electron dynamics. The two contributions are related to primary ionization and excitation processes, offering a deeper understanding of the origin of high harmonics near the ionization threshold. This Letter shows that high-harmonic spectroscopy can be extended to the near-threshold spectral range, which is in general spectroscopically rich.