Hydrated granular packings often crack into discrete clusters of grains when dried. Despite its ubiquity, an accurate prediction of cracking remains elusive. Here, we elucidate the previously overlooked role of individual grain shrinkage—a feature common to many materials—in determining crack patterning using both experiments and simulations. By extending classical Griffith crack theory, we obtain a scaling law that quantifies how cluster size depends on the interplay between grain shrinkage, stiffness, and size—applicable to a diverse array of shrinkable granular packings.

We present local direct imaging of the progressive adsorption of colloidal particles inside a 3D model porous medium. By varying the interparticle electrostatic interactions, we observe a large range of particle deposition regimes, from a single layer of particles at the surface of the medium to multiple layers and eventually clogging of the system. We derive the complete deposition dynamics and show that colloid accumulation is a self-limited mechanism towards a deposited fraction associated with a balance between the particle interactions and the imposed flow rate. These trends are explained and predicted using a simple probability model considering the particle adsorption energy and the variation of the drag energy with evolving porosity. This constitutes a direct validation of speculated particle transport mechanisms, and a further understanding of accumulation mechanisms.

We propose and experimentally realize a technique to measure the transfer function of a control line in the frequency domain using a qubit as a vector network analyzer. Our method requires coupling the line under test to the longitudinal component of the Hamiltonian of the qubit and the ability to induce Rabi oscillations through simultaneous driving of the transverse component. The method can be used to increase the fidelity of entangling gates in a quantum processor. We have demonstrated that by characterizing the “flux” control line of a superconducting transmon qubit in the range from 1 to 450 MHz and using this characterization to improve the fidelity of an entangling cphase gate between two transmon qubits.

The anomaly cancellation equations for the U(1) gauge group can be written as a cubic equation in $n-1$ integer variables, where $n$ is the number of Weyl fermions carrying the U(1) charge. We solve this Diophantine cubic equation by providing a parametrization of the charges in terms of $n-2$ integers, and prove that this is the most general solution.

We demonstrate various regimes of synchronization in systems of two coupled cavity soliton-based Kerr frequency combs. We show subharmonic, harmonic, and harmonic-ratio synchronization of coupled microresonators, and reveal their dynamics in the form of Arnold tongues, structures that are ubiquitous in nonlinear dynamical systems. Our experimental results are well corroborated by numerical simulations based on coupled Lugiato-Lefever equations. This Letter illustrates the newfound degree of flexibility in synchronizing Kerr combs across a wide range of comb spacings and could find applications in time and frequency metrology, spectroscopy, microwave photonics, optical communications, and astronomy.

A new type of dynamics called laminar chaos was recently discovered through a theoretical analysis of a scalar delay differential equation with time-varying delay. Laminar chaos is a low-dimensional dynamics characterized by laminar phases of nearly constant intensity with periodic durations and a chaotic variation of the intensity from one laminar phase to the next laminar phase. This is in stark contrast to the typically observed higher-dimensional turbulent chaos, which is characterized by strong fluctuations. In this Letter we provide the first experimental observation of laminar chaos by studying an optoelectronic feedback loop with time-varying delay. The noise inherent in the experiment requires the development of a nonlinear Langevin equation with variable delay. The results show that laminar chaos can be observed in higher-order systems, and that the phenomenon is robust to noise and a digital implementation of the variable time delay.

A transition from a $d^2$ to a $d$ law is observed in molecular dynamics (MD) simulations when the diameter ($d$) of an evaporating droplet reduces to the order of the vapor’s mean free path; this cannot be explained by classical theory. This Letter shows that the $d$ law can be predicted within the Navier-Stokes-Fourier (NSF) paradigm if a temperature-jump boundary condition derived from kinetic theory is utilized. The results from this model agree with those from MD in terms of the total lifetime, droplet radius, and temperature, while the classical $d^2$ law underpredicts the lifetime of the droplet by a factor of 2. Theories beyond NSF are also employed in order to investigate vapor rarefaction effects within the Knudsen layer adjacent to the interface.

Fixed-node diffusion Monte Carlo (FNDMC) method is a stochastic quantum many-body approach that has a great potential in electronic structure theory. We examine how FNDMC total energy $E(N)$ satisfies exact constraints, linearity and derivative discontinuity, versus fractional electron number $N$, if combined with mean-field trial wave functions that miss such features. H and Cl atoms with fractional charge reveal that FNDMC method is well able to restore the piecewise linearity of $E(N)$. The method uses ensemble and projector ingredients to achieve the correct charge localization. A water-solvated ${\mathrm{Cl}}^{-}$ complex illustrates superior performance of FNDMC method for charged noncovalent systems.

Electric resistivity, magnetic susceptibility, and x-ray diffraction measurements under high pressure are performed in both $\alpha$-${\mathrm{Sr}}_2{\mathrm{VO}}_4$ and $\alpha$-${\mathrm{Sr}}_2{\mathrm{CrO}}_4$, which are carefully prepared with regard to their stoichiometry. These measurements reveal contrasting and peculiar metallization processes of these compounds with increasing pressure. In contrast to a previously reported one in a V compound, we find two kinds of pressure-induced metallic states at low- ($T<50\mathrm{K}$) and high-temperature ($T>100\mathrm{K}$) regions. The high-temperature one seems to emerge beyond the pressure-induced Mott transition. The low-temperature one might imply a topological nature of the V compound, which is expected in the spin-orbit coupled $3d^1$ state that arises from their degenerated $d_{zx}$ and $d_{yz}$ orbits.

The tracer diffusion coefficient of six different permanent gases in polymer-grafted nanoparticle (GNP) membranes, i.e., neat GNP constructs with no solvent, show a maximum as a function of the grafted chain length at fixed grafting density. This trend is reproduced for two different NP sizes and three different polymer chemistries. We postulate that nonmonotonic changes in local, segmental friction as a function of graft chain length (at fixed grafting density) must underpin these effects, and use quasielastic neutron scattering to probe the self-motions of polymer chains at the relevant segmental scale (i.e., sampling local friction or viscosity). These data, when interpreted with a jump diffusion model, show that, in addition to the speeding-up in local chain dynamics, the elementary distance over which segments hop is strongly dependent on graft chain length. We therefore conclude that transport modifications in these GNP layers, which are underpinned by a structural transition from a concentrated brush to semidilute polymer brush, are a consequence of both spatial and temporal changes, both of which are likely driven by the lower polymer densities of the GNPs relative to the neat polymer.

We show that the generalization of the relative entropy of a resource from states to channels is not unique, and there are at least six such generalizations. Then, we show that two of these generalizations are asymptotically continuous, satisfy a version of the asymptotic equipartition property, and their regularizations appear in the power exponent of channel versions of the quantum Stein’s lemma. To obtain our results, we use a new type of “smoothing” that can be applied to functions of channels (with no state analog). We call it “liberal smoothing” as it allows for more spread in the optimization. Along the way, we show that the diamond norm can be expressed as a max relative entropy distance to the set of quantum channels, and prove a variety of properties of all six generalizations of the relative entropy of a resource.

Gravitational waves emitted during the merger of two black holes carry information about the remnant black hole, namely its mass and spin. This information is typically found from the ringdown radiation as the black hole settles to a final state. We find that the remnant black hole spin is already known at the peak amplitude of the gravitational wave strain. Using this knowledge, we present a new method for measuring the final spin that is template independent, using only the chirp mass, the instantaneous frequency of the strain, and its derivative at maximum amplitude, all template independent.

We investigate the influence of laser phase noise heating on resolved sideband cooling in the context of cooling the center-of-mass motion of a levitated nanoparticle in a high-finesse cavity. Although phase noise heating is not a fundamental physical constraint, the regime where it becomes the main limitation in Levitodynamics has so far been unexplored and hence embodies from this point forward the main obstacle in reaching the motional ground state of levitated mesoscopic objects with resolved sideband cooling. We reach minimal center-of-mass temperatures comparable to $T_{\min }=10\mathrm{mK}$ at a pressure of $p=3\times {10}^{-7}\mathrm{mbar}$, solely limited by phase noise. Finally we present possible strategies towards motional ground state cooling in the presence of phase noise.

We present a diagrammatic decomposition of the transition pair correlation function for the uniform electron gas. We demonstrate explicitly that ring and ladder diagrams are dual counterparts that capture significant long- and short-ranged interelectronic correlation effects, respectively. Our findings help to guide the further development of approximate many-electron theories and reveal that the contribution of the ladder diagrams to the electronic correlation energy can be approximated in an effective manner using second-order perturbation theory. We employ the latter approximation to reduce the computational cost of coupled cluster theory calculations for insulators and semiconductors by 2 orders of magnitude without compromising accuracy.

An extended Hubbard model on a honeycomb lattice with two orbitals per site at charge neutrality is investigated with unbiased large-scale quantum Monte Carlo simulations. The Fermi velocity of the Dirac fermions is renormalized as the cluster charge interaction increases, until a mass term emerges and a quantum phase transition from Dirac semimetal to valence bond solid (VBS) insulator is established. The quantum critical point is discovered to belong to the 3D $N=4$ Gross-Neveu chiral $XY$ universality with the critical exponents obtained at high precision. Further enhancement of the interaction drives the system into two different VBS phases, the properties and transition between them are also revealed. Since the model is related to magic-angle twisted bilayer graphene, our results may have relevance towards the symmetry breaking order at the charge neutrality point of the material, and associate the wide range of universal strange metal behavior around it with quantum critical fluctuations.

We study the modulus mediation of supersymmetry breaking motivated by superstring theory. We show that the renormalization group running of the soft supersymmetry breaking parameters due to the interactions of massive fields is canceled by the threshold corrections at one-loop order, if their mass is given by nonperturbative dynamics controlled by the same modulus that mediates supersymmetry breaking and a sum rule of the modular weights holds for the Yukawa couplings. As an example, we discuss order reduction of lepton flavor violation in the supersymmetric seesaw mechanism, which revives the parameter space already excluded.