Negativity of the Wigner function is seen as a crucial resource for reaching a quantum computational advantage with continuous variable systems. However, these systems, while they allow for the deterministic generation of large entangled states, require an extra element such as photon subtraction to obtain such negativity. Photon subtraction is known to affect modes beyond the one where the photon is subtracted, an effect which is governed by the correlations of the state. In this Letter, we build upon this effect to remotely prepare states with Wigner negativity. More specifically, we show that photon subtraction can induce Wigner negativity in a correlated mode if and only if that correlated mode can perform Einstein-Podolsky-Rosen steering in the mode of subtraction.

Ionization of atoms by strong laser fields produces photoelectron momentum distributions that exhibit modulations due to the interference of outgoing electron trajectories. For a faithful modeling, it is essential to include previously overlooked phase shifts occurring when trajectories pass through focal points. Such phase shifts are known as Gouy’s phase anomaly in optics or as Maslov phases in semiclassical theory. Because of Coulomb focusing in three dimensions, one out of two trajectories in photoelectron holography goes through a focal point as it crosses the symmetry axis in momentum space. In addition, there exist observable Maslov phases already in two dimensions. Clustering algorithms enable us to implement a semiclassical model with the correct preexponential factor that affects both the weight and the phase of each trajectory. We also derive a simple rule to relate two-dimensional and three-dimensional models for linear polarization. It explains the shifted interference fringes and weaker high-energy yield in three dimensions. The results are in excellent agreement with solutions of the time-dependent Schrödinger equation.

We demonstrate a novel method for coherent optical manipulation of individual nuclear spins in the solid state, mediated by the electronic states of a proximal quantum emitter. Specifically, using the nitrogen-vacancy (NV) color center in diamond, we demonstrate control of a proximal ${}^{14}\mathrm{N}$ nuclear spin via an all-optical Raman technique. We evaluate the extent to which the intrinsic physical properties of the NV center limit the performance of coherent control, and we find that it is ultimately constrained by the relative rates of transverse hyperfine coupling and radiative decay in the NV center’s excited state. Possible extensions and applications to other color centers are discussed.

We present a joint experiment-theory analysis of the temperature-dependent emission spectra, zero-phonon linewidth, and second-order correlation function of light emitted from a single organic molecule. We observe spectra with a zero-phonon line together with several additional sharp peaks, broad phonon sidebands, and a strongly temperature dependent homogeneous broadening. Our model includes both localized vibrational modes of the molecule and a thermal phonon bath, which we include nonperturbatively, and is able to capture all observed features. For resonant driving we measure Rabi oscillations that become increasingly damped with temperature, which our model naturally reproduces. Our results constitute an essential characterization of the photon coherence of molecules, paving the way to their use in future quantum information applications.

We investigate, experimentally and theoretically, the dynamics of a laser-driven cavity with noninstantaneous effective photon-photon interactions. Scanning the laser-cavity frequency detuning at different speeds across an optical bistability, we find a hysteresis area that is a nonmonotonic function of the speed. In the limit of fast scans comparable to the memory time of the interactions, we demonstrate that the hysteresis area decays following a universal power law with scaling exponent $-1$. We further demonstrate a regime of non-Markovian dynamics emerging from white noise. This regime is evidenced by peaked distributions of residence times in the metastable states of our system. Our results offer new perspectives for exploring the physics of scaling, universality, and metastability, in non-Markovian regimes using arrays of bistable optical cavities with low quality factors, driven by low laser powers, and at room temperature.

A Doppler shifted resonance minority species ion cyclotron range of frequency (ICRF) scheme for heating neutral beam ions has been identified and optimized for the Wendelstein 7-X stellarator. Compared with more conventional methods, the synergetic scheme increases the normalized core collisional power transfer to the background plasma, and induces larger concentrations of energetic ions. Simulations in the intricate 3D magnetic stellarator geometry reveal an energetic distribution function that is only weakly anisotropic, and is thus relevant to fast ion and alpha particle driven Alfvén eigenmode experimental preparation. Quasilinear theory and simulations of the Joint European Torus indicate that the excellent confinement properties are due to increased velocity diffusion from ICRF interaction along the magnetic field lines. Agreement is found between SCENIC simulations and Joint European Torus experimental measurements for the total neutron rate and the energy distribution of the fast ions.

Interfacial Dzyaloshinskii–Moriya interaction (DMI) is experimentally investigated in Pt/Co/Pt multilayer films under strain. A strong variation (from 0.1 to $0.8\mathrm{mJ}/{\mathrm{m}}^2$) of the DMI constant is demonstrated at $\pm 0.1\%$ in-plane uniaxial deformation of the films. The anisotropic strain induces strong DMI anisotropy. The DMI constant perpendicular to the strain direction changes sign, while the constant along the strain direction does not. Estimates show that the DMI can be controlled with an electric field in hybrid ferroelectric-ferromagnetic systems. So, the observed effect opens the way to control the DMI and eventually skyrmions with a voltage via a strain-mediated magnetoelectric coupling.

Microscopic corrugations are ubiquitous in graphene even when placed on atomically flat substrates. These result in random local strain fluctuations limiting the carrier mobility of high quality hBN-supported graphene devices. We present transport measurements in hBN-encapsulated devices where such strain fluctuations can be in situ reduced by increasing the average uniaxial strain. When $\sim 0.2\%$ of uniaxial strain is applied to the graphene, an enhancement of the carrier mobility by $\sim 35\%$ is observed while the residual doping reduces by $\sim 39\%$. We demonstrate a strong correlation between the mobility and the residual doping, from which we conclude that random local strain fluctuations are the dominant source of disorder limiting the mobility in these devices. Our findings are also supported by Raman spectroscopy measurements.

We construct a polarization-mediated magic-intensity (MI) optical dipole trap (ODT) array, in which the detrimental effects of light shifts on the mixed-species qubits are efficiently mitigated so that the coherence times of the mixed-species qubits are both substantially enhanced and balanced for the first time. This mixed-species magic trapping technique relies on the tunability of the coefficient of the third-order cross term and ground state hyperpolarizability, which are inherently dependent on the degree of circular polarization of the trapping laser. Experimentally, polarization of the ODT array for ${}^{85}\mathrm{Rb}$ qubits is finely adjusted to a definite value so that its working magnetic field required for magic trapping amounts to the one required for magically trapping ${}^{87}\mathrm{Rb}$ qubits in another ODT array with fully circular polarization. Ultimately, in such a polarization-mediated MI-ODT array, the coherence times of ${}^{87}\mathrm{Rb}$ and ${}^{85}\mathrm{Rb}$ qubits are, respectively, enhanced up to $891\pm 47\mathrm{ms}$ and $943\pm 35\mathrm{ms}$. Moreover, we reveal that the noise of the elliptic polarization causes dephasing effect on the ${}^{85}\mathrm{Rb}$ qubits but it could be efficiently mitigated by choosing the dynamical range of active polarization device. We also show that light shifts seen by qubits in an elliptically polarized MI-ODT can be more efficiently compensated due to the decrease in the ground state hyperpolarizability. It is anticipated that the novel mixed-species MI-ODT array is a versatile platform for building scalable quantum computers with neutral atoms.

We observe clear evidence of adiabatic passage between photon populations via a four-wave mixing process, implemented through a dispersion sweep arranged by a core diameter taper of an optical fiber. Photonic rapid adiabatic passage through the cubic electric susceptibility thus opens precise control of frequency translation between broadband light fields to all common optical media. Areas of potential impact include optical fiber and on-chip waveguide platforms for quantum information, ultrafast spectroscopy and metrology, and extreme light-matter interaction science.

The McLachlan “minimum-distance” principle for optimizing approximate solutions of the time-dependent Schrödinger equation is revisited, with a focus on the local-in-time error accompanying the variational solutions. Simple, exact expressions are provided for this error, which are then evaluated in illustrative cases, notably the widely used mean-field approach and the adiabatic quantum molecular dynamics. Based on these findings, we demonstrate the rigorous formulation of an adaptive scheme that resizes on the fly the underlying variational manifold and, hence, optimizes the overall computational cost of a quantum dynamical simulation. Such adaptive schemes are a crucial requirement for devising and applying direct quantum dynamical methods to molecular and condensed-phase problems.

We study nonadiabatic effects of geometric pumping. With arbitrary choices of periodic control parameters, we go beyond the adiabatic approximation to obtain the exact pumping current. We find that a geometrical interpretation for the nontrivial part of the current is possible even in the nonadiabatic regime. The exact result allows us to find a smooth connection between the adiabatic Berry phase theory at low frequencies and the Floquet theory at high frequencies. We also study how to control the geometric current. Using the method of shortcuts to adiabaticity with the aid of an assisting field, we illustrate that it enhances the current.

Adiabatic pumping is characterized by a geometric contribution to the pumped charge, which can be nonzero even in the absence of a bias. However, as the driving speed is increased, nonadiabatic excitations gradually reduce the pumped charge, thereby limiting the maximal applicable driving frequencies. To circumvent this problem, we here extend the concept of shortcuts to adiabaticity to construct a control protocol which enables geometric pumping well beyond the adiabatic regime. Our protocol allows for an increase, by more than an order of magnitude, in the driving frequencies, and the method is also robust against moderate fluctuations of the control field. We provide a geometric interpretation of the control protocol and analyze the thermodynamic cost of implementing it. Our findings can be realized using current technology and potentially enable fast pumping of charge or heat in quantum dots, as well as in other stochastic systems from physics, chemistry, and biology.

We derive the general analytical solution of the viscous hydrodynamic equations for an ultrarelativistic gas of hard spheres undergoing Bjorken expansion, taking into account effects from particle number conservation, and use it to analytically determine its attractor at late times. Differently than all the cases considered before involving rapidly expanding fluids, in this example the gradient expansion converges. We exactly determine the hydrodynamic attractor of this system when its microscopic dynamics is modeled by the Boltzmann equation with a fully nonlinear collision kernel. The exact late time attractor of this system can be reasonably described by hydrodynamics even when the gradients are large.

In this Letter, we discuss two general classes of apparent violations of the bulk-edge correspondence principle for continuous topological photonic materials, associated with the asymptotic behavior of the surface modes for diverging wave numbers. Considering a nonreciprocal plasma as a model system, we show that the inclusion of spatial dispersion (e.g., hydrodynamic nonlocality) formally restores the bulk-edge correspondence by avoiding an unphysical response at large wave numbers. Most importantly, however, our findings show that, for the considered cases, the correspondence principle is physically violated for all practical purposes, as a result of the unavoidable attenuation of highly confined modes even if all materials are assumed perfect, with zero intrinsic bulk losses, due to confinement-induced Landau damping or nonlocality-induced radiation leakage. Our work helps clarifying the subtle and rich topological wave physics of continuous media.

We study sharp-edge structures that are used in microfluidic systems for particle and cell manipulation. Experiments show that oscillating sharp edges can attract or repel particles suspended in a microfluidic channel. This effect is caused by acoustic radiation forces induced by sharp edges. We propose an analytical theory that allows one to evaluate the acoustic radiation force produced by a sharp-edge structure on elastic particles and to study which parameters govern the interaction of particles with a sharp-edge structure, forcing them to be attracted in one situation and to be repelled in another situation. The proposed theory gives foundations for the design of microfluidic systems making use of sharp edges for particle trapping. We also provide experimental data to validate the theory.

When a charge selective surface consumes or transports only cations or anions in the electrolyte, biased ion rejection initiates hydrodynamic instability, resulting in vortical fluid motions called electroconvection. In this Letter, we describe the first laboratory observation of three-dimensional electroconvection on a charge selective surface. Combining experiment and scaling analysis, we successfully categorized three distinct patterns of 3D electroconvection according to [$({\mathrm{Ra}}_E)/({\mathrm{Re}}^2\mathrm{Sc})$] [electric Rayleigh number (${\mathrm{Ra}}_E$), Reynolds number (Re), Schmidt number (Sc)] as (i) polygonal, (ii) transverse, or (iii) longitudinal rolls. If Re increases or ${\mathrm{Ra}}_E$ decreases, pure longitudinal rolls are presented. On the other hand, transverse rolls are formed between longitudinal rolls, and two rolls are transformed as polygonal one at higher ${\mathrm{Ra}}_E$ or lower Re. In this pattern selection scenario, Sc determines the critical electric Rayleigh number (${\mathrm{Ra}}_E^{*}$) for the onset of each roll, resulting in ${\mathrm{Ra}}_E^{*}\sim {\mathrm{Re}}^2\mathrm{Sc}$. We also verify that convective ion flux by electroconvection (represented by an electric Nusselt number ${\mathrm{Nu}}_E$) is fitted to a power law, ${\mathrm{Nu}}_E\sim [({\mathrm{Ra}}_E-{\mathrm{Ra}}_E^{*})/({\mathrm{Re}}^2\mathrm{Sc}){]}^{{\alpha }_1}{\mathrm{Re}}^{{\alpha }_2}\text{P}{\text{e}}^{{\alpha }_3}$ [Péclet number (Pe)], where each term represents the characteristics of electroconvection, shear flow, and ion transport.