Energy flow and balance in convergent systems beyond petapascal energy densities controls the fate of late-stage stars and the potential for controlling thermonuclear inertial fusion ignition. Time-resolved x-ray self-emission imaging combined with a Bayesian inference analysis is used to describe the energy flow and the potential information stored in the rebounding spherical shock at 0.22 PPa (2.2 Gbar or billions of atmospheres pressure). This analysis, together with a simple mechanical model, describes the trajectory of the shell and the time history of the pressure at the fuel-shell interface, ablation pressure, and energy partitioning including kinetic energy of the shell and internal energy of the fuel. The techniques used here provide a fully self-consistent uncertainty analysis of integrated implosion data, a thermodynamic-path independent measurement of pressure in the petapascal range, and can be used to deduce the energy flow in a wide variety of implosion systems to petapascal energy densities.

Despite extensive shock wave and static compression experiments and corresponding theoretical work, consensus on the crystal structure and the melt boundary of Fe at Earth’s core conditions is lacking. We present in situ x-ray diffraction measurements in laser-shock compressed Fe that establish the stability of the hexagonal-close-packed (hcp) structure along the Hugoniot through shock melting, which occurs between $\sim 242$ to $\sim 247\mathrm{GPa}$. Using previously reported hcp Fe Hugoniot temperatures, the melt temperature is estimated to be 5560(360) K at 242 GPa, consistent with several reported Fe melt curves. Extrapolation of this value suggests $\sim 6400\mathrm{K}$ melt temperature at Earth’s inner core boundary pressure.

Even though no local order parameter in the sense of the Landau theory exists for topological quantum phase transitions in Chern insulators, the highly nonlocal Berry curvature exhibits critical behavior near a quantum critical point. We investigate the critical properties of its real space analog, the local Chern marker, in weakly disordered Chern insulators. Because of disorder, inhomogeneities appear in the spatial distribution of the local Chern marker. Their size exhibits power-law scaling with the critical exponent matching the one extracted from the Berry curvature of a clean system. We drive the system slowly through such a quantum phase transition. The characteristic size of inhomogeneities in the nonequilibrium postquench state obeys the Kibble-Zurek scaling. In this setting, the local Chern marker thus does behave in a similar way as a local order parameter for a symmetry breaking second order phase transition. The Kibble-Zurek scaling also holds for the inhomogeneities in the spatial distribution of excitations and of the orbital polarization.

It is well known that superconductivity in quasi-one-dimensional (Q1D) materials is hindered by large fluctuations of the order parameter. They reduce the critical temperature and can even destroy the superconductivity altogether. Here it is demonstrated that the situation changes dramatically when a Q1D pair condensate is coupled to a higher-dimensional stable one, as in recently discovered multiband Q1D superconductors. The fluctuations are suppressed even by vanishingly small pair-exchange coupling between different band condensates and the superconductor is well described by the mean field theory. In this case the low dimensionality effects enhance the coherence of the system instead of suppressing it. As a result, the critical temperature of the multiband Q1D superconductor can increase by orders of magnitude when the system is tuned to the Lifshitz transition with the Fermi level close to the edge of the Q1D band.

Recent observations [A. Pustogow et al., Nature (London) 574, 72 (2019).] of a drop of the ${}^{17}\mathrm{O}$ nuclear magnetic resonance (NMR) Knight shift in the superconducting state of ${\mathrm{Sr}}_2{\mathrm{RuO}}_4$ challenged the popular picture of a chiral odd-parity paired state in this compound. Here we use polarized neutron scattering (PNS) to show that there is a $34\pm 6\%$ drop in the magnetic susceptibility at the Ru site below the superconducting transition temperature. We measure at lower fields $H\sim \frac{1}{3}{H}_{c2}$ than a previous PNS study allowing the suppression to be observed. The PNS measurements show a smaller susceptibility suppression than NMR measurements performed at similar field and temperature. Our results rule out the chiral odd-parity $\mathbf{d}=\widehat{\mathbf{z}}(k_x\pm i{k}_y)$ state and are consistent with several recent proposals for the order parameter including even-parity $B_{1g}$ and odd-parity helical states.

Predicting the behavior of heterogeneous nonequilibrium systems is currently analytically intractable. Consequently, complex biological systems have resisted unifying principles. Here, I introduce a mapping from dynamical systems to battery-resistor circuits. I show that in these transformed variables (i) arbitrary numbers of heterogeneous dynamical transitions can be reduced to a Thevenin equivalent resistor which is invariant to driving from equilibrium, (ii) resistors (together with the external driving sources) are sufficient to describe system behavior, and (iii) the resistor’s directional symmetry leads to universal theorems of nonequilibrium behavior. This mapping is used to derive two general steady-state relations. First, for any cyclic process, the maximum amplification of any state is tightly bounded by the total dissipation of all states; experimental data are used to show that the master signal protein Ras achieves this bound. Second, for any process, the response of any reaction due to driving any other reaction is identical to the reciprocal response rescaled by the ratio of the corresponding Thevenin resistors. This result generalizes Onsager’s reciprocal relation to the strongly driven regime and makes a testable prediction about how systems should be designed or evolved to maximize response. These analytic results represent a new perspective applicable to biological complexity and suggest that this mapping provides the natural variables to study heterogeneous nonequilibrium systems.

Quantum no-cloning, the impossibility of perfectly cloning an arbitrary unknown quantum state, is one of the most fundamental limitations due to the laws of quantum mechanics, which underpin the physical security of quantum key distribution. Quantum physics does allow, however, approximate cloning with either imperfect state fidelity and/or probabilistic success. Whereas approximate quantum cloning of single-particle states has been tested previously, experimental cloning of quantum entanglement—a highly nonclassical correlation—remained unexplored. Based on a multiphoton linear optics platform, we demonstrate quantum cloning of two-photon entangled states for the first time. Remarkably our results show that one maximally entangled photon pair can be broadcast into two entangled pairs, both with state fidelities above 50%. Our results are a key step towards cloning of complex quantum systems, and are likely to provide new insights into quantum entanglement.

We present numerical evidence for an additional discontinuous transition, upon compression, inside the jammed regime for an asymmetric bidisperse granular packing. This additional transition line separates jammed states with networks of predominantly large particles from jammed networks formed by both large and small particles, and the transition is indicated by a discontinuity in the number of particles contributing to the jammed network. The additional transition line emerges from the curves of jamming transitions and terminates in an end point where the discontinuity vanishes. The additional line is starting at a size ratio around $\delta =0.22$ and grows longer for smaller $\delta$. For $\delta \to 0$, the additional transition line approaches a limit that can be derived analytically. The observed jamming scenarios are reminiscent of glass-glass transitions found in colloidal glasses.

The nuclear tunneling crossover temperature ($T_c$) of hydrogen transfer reactions in supported molecular-switch architectures can lie close to room temperature. This calls for the inclusion of nuclear quantum effects (NQEs) in the calculation of reaction rates even at high temperatures. However, computations of NQEs relying on standard parametrized dimensionality-reduced models quickly become inadequate in these environments. In this Letter, we study the paradigmatic molecular switch based on porphycene molecules adsorbed on metallic surfaces with full-dimensional calculations that combine density-functional theory for the electrons with the semiclassical ring-polymer instanton approximation for the nuclei. We show that the double intramolecular hydrogen transfer (DHT) rate can be enhanced by orders of magnitude due to surface fluctuations in the deep-tunneling regime. We also explain the origin of an Arrhenius temperature dependence of the rate below $T_c$ and why this dependence differs at different surfaces. We propose a simple model to rationalize the temperature dependence of DHT rates spanning diverse fcc [110] surfaces.

We present a microscopic Fermi liquid view on the low-energy transport through an Anderson impurity with $N$ discrete levels, at arbitrary electron filling $N_d$. It is applied to nonequilibrium current fluctuations, for which the two-quasiparticle collision integral and the three-body correlations that determine the quasiparticle energy shift play important roles. Using the numerical renormalization group up to $N=6$, we find that for strong interactions the three-body fluctuations are determined by a single parameter other than the Kondo energy scale in a wide filling range $1\lesssim N_d\lesssim N-1$. It significantly affects the current noise for $N>2$ and the behavior of noise in magnetic fields.

We studied the electronic Raman spectra of $({\mathrm{Li}}_{1-x}{\mathrm{Fe}}_x)\mathrm{OHFeSe}$ as a function of light polarization and temperature. In the $B_{1g}$ spectra alone we observe the redistribution of spectral weight expected for a superconductor and two well-resolved peaks below $T_c$. The nearly resolution-limited peak at $110{\mathrm{cm}}^{-1}$ (13.6 meV) is identified as a collective mode. The peak at $190{\mathrm{cm}}^{-1}$ (23.6 meV) is presumably another collective mode since the line is symmetric and its energy is significantly below the gap energy observed by single-particle spectroscopies. Given the experimental band structure of $({\mathrm{Li}}_{1-x}{\mathrm{Fe}}_x)\mathrm{OHFeSe}$, the most plausible explanations include conventional spin-fluctuation pairing between the electron bands and the incipient hole band and pairing between the hybridized electron bands. The absence of gap features in $A_{1g}$ and $B_{2g}$ symmetry favors the second case. Thus, in spite of various differences between the pnictides and chalcogenides, this Letter demonstrates the proximity of pairing states and the importance of band structure effects in the Fe-based compounds.

Magnon polarons, a type of hybridized excitations between magnons and phonons, were first reported in yttrium iron garnet as anomalies in the spin Seebeck effect responses. Here, we report an observation of antiferromagnetic (AFM) magnon polarons in a uniaxial AFM insulator ${\mathrm{Cr}}_2{\mathrm{O}}_3$. Despite the relatively higher energy of magnon than that of the acoustic phonons, near the spin-flop transition of $\sim 6\mathrm{T}$, the left-handed magnon spectrum shifts downward to hybridize with the acoustic phonons to form AFM magnon polarons, which can also be probed by the spin Seebeck effect. The spin Seebeck signal is founded to be enhanced due to the magnon polarons at low temperatures.

We analyze the quantum entanglement between opposite spin projection electrons in the ground state of the Anderson impurity model. In this model, a single level impurity with intralevel repulsion $U$ is tunnel coupled to a free electron gas. The Anderson model presents a strongly correlated many body ground state with mass enhanced quasiparticle excitations. We find, using both analytical and numerical tools, that the quantum entanglement between opposite spin projection electrons is a monotonic universal function of the quasiparticle mass enhancement $Z$ in the Kondo regime. This indicates that the interaction induced mass enhancement, which is generally used to quantify correlations in quantum many body systems, could be used as a measure of entanglement in the Kondo problem.

One of the intrinsic characteristics of far-from-equilibrium systems is the nonrelaxational nature of the system dynamics, which leads to novel properties that cannot be understood and described by conventional pathways based on thermodynamic potentials. Of particular interest are the formation and evolution of ordered patterns composed of active particles that exhibit collective behavior. Here we examine such a type of nonpotential active system, focusing on effects of coupling and competition between chiral particle self-propulsion and self-spinning. It leads to the transition between three bulk dynamical regimes dominated by collective translative motion, spinning-induced structural arrest, and dynamical frustration. In addition, a persistently dynamical state of self-rotating crystallites is identified as a result of a localized-delocalized transition induced by the crystal-melt interface. The mechanism for the breaking of localized bulk states can also be utilized to achieve self-shearing or self-flow of active crystalline layers.

When an observable is measured on an evolving coherent quantum system twice, the first measurement generally alters the statistics of the second one, which is known as measurement backaction. We introduce, and push to its theoretical and experimental limits, a novel method of backaction evasion, whereby entangled collective measurements are performed on several copies of the system. This method is inspired by a similar idea designed for the problem of measuring quantum work [Perarnau-Llobet et al., Phys. Rev. Lett. 118, 070601 (2017)]. By using entanglement as a resource, we show that the backaction can be extremely suppressed compared to all previous schemes. Importantly, the backaction can be eliminated in highly coherent processes.