Microscale Janus emulsions represent a versatile material platform for dynamic refractive, reflective, and light-emitting optical components. Here, we present a mechanism for droplet actuation that exploits thermocapillarity. Using optically induced thermal gradients, an interfacial tension differential is generated across the surfactant-free internal capillary interface of Janus droplets. The interfacial tension differential causes droplet-internal Marangoni flows and a net torque, resulting in a predictable and controllable reorientation of the droplets. The effect can be quantitatively described with a simple model that balances gravitational and thermal torques. Occurring in small thermal gradients, these optothermally induced Marangoni dynamics represent a promising mechanism for controlling droplet-based micro-optical components.

We report the observation of gravity-capillary waves on a torus of fluid. By means of an original technique, a stable torus is achieved by depositing water on a superhydrophobic groove with a shallow wedge-shaped channel running along its perimeter. Using a spatiotemporal optical measurement, we report the full dispersion relation of azimuthal waves propagating along the inner and outer torus borders, highlighting several branches modeled as varicose, sinuous, and sloshing modes. Standing azimuthal waves are also studied leading to polygonlike patterns arising on the two torus borders with a number of sides different when a tunable decoupling of the two interfaces occurs. The quantized nature of the dispersion relation is also evidenced.

We present large-scale dynamical simulations of electronic phase separation in the single-band double-exchange model based on deep-learning neural-network potentials trained from small-size exact diagonalization solutions. We uncover an intriguing correlation-induced freezing behavior as doped holes are segregated from half filled insulating background during equilibration. While the aggregation of holes is stabilized by the formation of ferromagnetic clusters through Hund’s coupling between charge carriers and local magnetic moments, this stabilization also creates confining potentials for holes when antiferromagnetic spin-spin correlation is well developed in the background. The dramatically reduced mobility of the self-trapped holes prematurely disrupts further growth of the ferromagnetic clusters, leading to an arrested phase separation. Implications of our findings for phase separation dynamics in materials that exhibit colossal magnetoresistance effect are discussed.

Exotic high-rank multipolar order parameters have been found to be unexpectedly active in more and more correlated materials in recent years. Such multipoles are usually dubbed “hidden orders” since they are insensitive to common experimental probes. Theoretically, it is also difficult to predict multipolar orders via ab initio calculations in real materials. Here, we present an efficient method to predict possible multipoles in materials based on linear response theory under random phase approximation. Using this method, we successfully predict two pure metastable magnetic octupolar states in monolayer $\alpha \text{−}{\mathrm{RuCl}}_3$, which is confirmed by self-consistent unrestricted Hartree-Fock calculations. We then demonstrate that these octupolar states can be stabilized in monolayer $\alpha \text{−}{\mathrm{RuI}}_3$, one of which becomes the octupolar ground state. Furthermore, we also predict a fingerprint of an orthogonal magnetization pattern produced by the octupole moment that can be easily detected by experiment. The method and the example presented in this Letter serve as a guide for searching multipolar order parameters in other correlated materials.

We report on finite-size exact-diagonalization calculations in a Hilbert space defined by the continuum-model flat moiré bands of magic angle twisted bilayer graphene. For moiré band filling $3>|\nu |>2$, where superconductivity is strongest, we obtain evidence that the ground state is a spin ferromagnet. Near $|\nu |=3$, we find Chern insulator ground states that have spontaneous spin, valley, and sublattice polarization, and demonstrate that the anisotropy energy in this order-parameter space is strongly band-filling-factor dependent. We emphasize that inclusion of the remote band self-energy is necessary for a reliable description of magic angle twisted bilayer graphene flat band correlations.

Organic salts represent an ideal experimental playground for studying the interplay between magnetic and charge degrees of freedom, which has culminated in the discovery of several spin-liquid candidates such as $\kappa \text{−}(\mathrm{ET}{)}_2{\mathrm{Cu}}_2(\mathrm{CN}{)}_3$ ($\kappa \text{−}\mathrm{Cu}$). Recent theoretical studies indicate the possibility of chiral spin liquids stabilized by ring exchange, but the parent states with chiral magnetic order have not been observed in this material family. In this Letter, we discuss the properties of the recently synthesized $\kappa \text{−}(\mathrm{BETS}{)}_2\mathrm{Mn}[\mathrm{N}(\mathrm{CN}{)}_2{]}_3$ ($\kappa \text{−}\mathrm{Mn}$). Based on analysis of specific heat, magnetic torque, and NMR measurements combined with ab initio calculations, we identify a spin-vortex crystal order. These observations definitively confirm the importance of ring exchange in these materials and support the proposed chiral spin-liquid scenario for triangular lattice organics.

The existence of a transition from a clogged to an unclogged state has been recently proposed for the flow of macroscopic particles through bottlenecks in systems as diverse as colloidal suspensions, granular matter, or live beings. Here, we experimentally demonstrate that, for vibrated granular media, such a transition genuinely exists, and we characterize it as a function of the outlet size and vibration intensity. We confirm the suitability of the “flowing parameter” as the order parameter, and we find out that the rescaled maximum acceleration of the system should be replaced as the control parameter by a dimensionless velocity that can be seen as the square root of the ratio between kinetic and potential energy. In all the investigated scenarios, we observe that, for a critical value of this control parameter $S_c$, there seems to be a continuous transition to an unclogged state. The data can be rescaled with this critical value, which, as expected, decreases with the orifice size $D$. This leads to a phase diagram in the $S\text{−}D$ plane in which clogging appears as a concave surface.

Biological neuronal networks excel over artificial ones in many ways, but the origin of this is still unknown. Our symbolic dynamics-based tool of excess entropies suggests that neuronal cultures naturally implement data structures of a higher level than what we expect from artificial neural networks, or from close-to-biology neural networks. This points to a new pathway for improving artificial neural networks towards a level demonstrated by biology.

We discuss certain structural analogies between supersymmetric quiver gauge theories and lattice models leading to fracton phases of matter. In particular, classes of quiver models can be viewed as lattice models having subsystem symmetries, dimensions of moduli spaces growing linearly with the size of the lattice, and having excitations with limited mobility (with “excitations” and “mobility” properly defined).

We consider the nonequilibrium orbital dynamics of spin-polarized ultracold fermions in the first excited band of an optical lattice. A specific lattice depth and filling configuration is designed to allow the $p_x$ and $p_y$ excited orbital degrees of freedom to act as a pseudospin. Starting from the full Hamiltonian for $p$-wave interactions in a periodic potential, we derive an extended Hubbard-type model that describes the anisotropic lattice dynamics of the excited orbitals at low energy. We then show how dispersion engineering can provide a viable route to realizing collective behavior driven by $p$-wave interactions. In particular, Bragg dressing and lattice depth can reduce single-particle dispersion rates, such that a collective many-body gap is opened with only moderate Feshbach enhancement of $p$-wave interactions. Physical insight into the emergent gap-protected collective dynamics is gained by projecting the Hamiltonian into the Dicke manifold, yielding a one-axis twisting model for the orbital pseudospin that can be probed using conventional Ramsey-style interferometry. Experimentally realistic protocols to prepare and measure the many-body dynamics are discussed, including the effects of band relaxation, particle loss, spin-orbit coupling, and doping.

The polarization dependence of magnon-photon scattering in an optical microcavity is reported. Because of the short cavity length, the longitudinal mode-matching conditions found in previously explored, large path-length whispering gallery resonators are absent. Nonetheless, for cross-polarized scattering a strong and broadband suppression of one sideband is observed. This arises due to an interference between the Faraday and second-order Cotton-Mouton effects. To fully account for the suppression of the cross-polarized scattering, it is necessary to consider the squeezing of magnon modes intrinsic to thin-film geometry. A copolarized scattering due to Cotton-Mouton effect is also observed. In addition, the magnon modes involved are identified as Damon-Eshbach surface modes, whose nonreciprocal propagation could be exploited in device applications. This Letter experimentally demonstrates the important role of second-order Cotton-Mouton effect for optomagnonic devices.

We demonstrate the self-propulsion of a volatile drop on the surface of a bath of an immiscible liquid. Evaporative heat pumping is converted into directed motion through thermocapillary stresses, which arise from the coupling between surface-tension-driven flows and temperature advection. A propulsive force arises from convection-sustained temperature gradients along the drop interface, resulting in a warmer pool of liquid being advected by the hydrodynamic flow in the underlying bath toward the back of the drop. The dependence of the drop speed on the activity source, i.e., the evaporation flux, is derived with scaling arguments and captures the experimental data.

Discovering new topological phases of matter is a major theme in fundamental physics and materials science. Dirac semimetal provides an exceptional platform for exploring topological phase transitions under symmetry breaking. Recent theoretical studies have revealed that a three-dimensional Dirac semimetal can harbor fascinating hinge states, a higher-order topological manifestation not known before. However, its realization in experiment is yet to be achieved. In this Letter, we propose a minimum model to construct a spinless higher-order Dirac semimetal protected by $C_{6v}$ symmetry. By breaking different symmetries, this parent phase transitions into a variety of novel topological phases including higher-order topological insulator, higher-order Weyl semimetal, and higher-order nodal-ring semimetal. Furthermore, for the first time, we experimentally realize this unprecedented higher-order topological phase in a sonic crystal and present an unambiguous observation of the desired hinge states via momentum-space spectroscopy and real-space visualization. Our findings may offer new opportunities to manipulate classical waves such as sound and light.

We demonstrate a nanoscale materials design path that allows us to bypass universality in thin ferromagnetic films and enables us to tune the critical exponents of ferromagnetic phase transitions in a very wide parameter range, while at the same time preserving scaling in an extended phase space near the Curie temperature. Our detailed magnetometry results reveal that single crystal CoRu alloy films, in which the predefined depth dependent exchange coupling strength follows a V-shaped profile, exhibit critical scaling behavior over many orders of magnitude. Their critical exponents, however, can be designed and controlled by modifying their specific nanoscale structures, thus demonstrating full tunability of critical behavior. The reason for this tunability and the disappearance of universality is shown to be the competing relevance of collective versus interface propagating progression of ferromagnetic phase transitions, whose balance we find to be dependent on the specifics of the underlying exchange coupling strength profile.

Quantum emitters in diamond are leading optically accessible solid-state qubits. Among these, Group IV-vacancy defect centers have attracted great interest as coherent and stable optical interfaces to long-lived spin states. Theory indicates that their inversion symmetry provides first-order insensitivity to stray electric fields, a common limitation for optical coherence in any host material. Here we experimentally quantify this electric field dependence via an external electric field applied to individual tin-vacancy (SnV) centers in diamond. These measurements reveal that the permanent electric dipole moment and polarizability are at least 4 orders of magnitude smaller than for the diamond nitrogen vacancy (NV) centers, representing the first direct measurement of the inversion symmetry protection of a Group IV defect in diamond. Moreover, we show that by modulating the electric-field-induced dipole we can use the SnV as a nanoscale probe of local electric field noise, and we employ this technique to highlight the effect of spectral diffusion on the SnV.

Multipartite entanglement is an essential resource for quantum communication, quantum computing, quantum sensing, and quantum networks. The utility of a quantum state $|\psi ⟩$ for these applications is often directly related to the degree or type of entanglement present in $|\psi ⟩$. Therefore, efficiently quantifying and characterizing multipartite entanglement is of paramount importance. In this work, we introduce a family of multipartite entanglement measures, called concentratable entanglements. Several well-known entanglement measures are recovered as special cases of our family of measures, and hence we provide a general framework for quantifying multipartite entanglement. We prove that the entire family does not increase, on average, under local operations and classical communications. We also provide an operational meaning for these measures in terms of probabilistic concentration of entanglement into Bell pairs. Finally, we show that these quantities can be efficiently estimated on a quantum computer by implementing a parallelized SWAP test, opening up a research direction for measuring multipartite entanglement on quantum devices.

Quantum state tomography (QST) is a challenging task in intermediate-scale quantum devices. Here, we apply conditional generative adversarial networks (CGANs) to QST. In the CGAN framework, two dueling neural networks, a generator and a discriminator, learn multimodal models from data. We augment a CGAN with custom neural-network layers that enable conversion of output from any standard neural network into a physical density matrix. To reconstruct the density matrix, the generator and discriminator networks train each other on data using standard gradient-based methods. We demonstrate that our QST-CGAN reconstructs optical quantum states with high fidelity, using orders of magnitude fewer iterative steps, and less data, than both accelerated projected-gradient-based and iterative maximum-likelihood estimation. We also show that the QST-CGAN can reconstruct a quantum state in a single evaluation of the generator network if it has been pretrained on similar quantum states.

We construct Brownian Sachdev-Ye-Kitaev (SYK) chains subjected to continuous monitoring and explore possible entanglement phase transitions therein. We analytically derive the effective action in the large-$N$ limit and show that an entanglement transition is caused by the symmetry breaking in the enlarged replica space. In the noninteracting case with ${\mathrm{SYK}}_2$ chains, the model features a continuous $O(2)$ symmetry between two replicas and a transition corresponding to spontaneous breaking of that symmetry upon varying the measurement rate. In the symmetry broken phase at low measurement rate, the emergent replica criticality associated with the Goldstone mode leads to a log-scaling entanglement entropy that can be attributed to the free energy of vortices. In the symmetric phase at higher measurement rate, the entanglement entropy obeys area-law scaling. In the interacting case, the continuous $O(2)$ symmetry is explicitly lowered to a discrete $C_4$ symmetry, giving rise to volume-law entanglement entropy in the symmetry-broken phase due to the enhanced linear free energy cost of domain walls compared to vortices. The interacting transition is described by $C_4$ symmetry breaking. We also verify the large-$N$ critical exponents by numerically solving the Schwinger-Dyson equation.