The combination of electride state and superconductivity within the same compound, e.g., ${[{\mathrm{Ca}}_{24}{\mathrm{Al}}_{28}{\mathrm{O}}_6]}^{4+}(4e^{-})$, opens up a new category of conventional superconductors. However, neither the underlying causations to explain superconducting behaviors nor effects of interstitial quasiatoms (ISQs) on superconductivity remain unclear. Here we have designed an efficient and resource-saving method to identify superconducting electrides only by chemical compositions and bonding characteristics. A representative superconducting electride ${\mathrm{Li}}_6\mathrm{C}$ with a noteworthy $T_c$ of 10 K below 1 Mbar among the known binary electrides has been revealed. Our first-principles studies unveil that the anomalous $sp$-hybridized cage-state ISQs, as a guest in ${\mathrm{Li}}_6\mathrm{C}$, exhibit unexpected ionic and covalent bonds, which act as a chemical precompression to lower dynamically stable pressure. More importantly, we uncover that, contrary to common expectations, the high $T_c$ is attributed to the strong electron-phonon coupling derived from the synergy of interatomic coupling effect, phonon softening caused by Fermi surface nesting, and phonon-coupled bands, which are mainly dominated by host $sp$-hybridized electrons, rather than the ISQs. Our present results elucidate a new superconducting mechanism of electrides and shed light on the way for seeking a high-$T_c$ superconductor at lower pressures in cage-state electrides.

Dynamical diffraction effects in thin single crystals produce highly monochromatic parallel x-ray beams with a mutual separation of a few microns and a time delay of a few femtoseconds—the so-called echoes. This ultrafast diffraction effect is used at X-Ray Free Electron Lasers in self-seeding schemes to improve beam monochromaticity. Here, we present a coherent x-ray imaging measurement of echoes from Si crystals and demonstrate that a small surface strain can be used to tune their temporal delay. These results represent a first step toward the ambitious goal of strain tailoring new x-ray optics and, conversely, open up the possibility of using ultrafast dynamical diffraction effects to study strain in materials.

While valleys (energy extrema) are present in all band structures of solids, their preeminent role in determining exciton resonances and dynamics in atomically thin transition metal dichalcogenides (TMDC) is unique. Using two-dimensional coherent electronic spectroscopy, we find that exciton decoherence occurs on a much faster timescale in ${\mathrm{MoSe}}_2$ bilayers than that in the monolayers. We further identify two population relaxation channels in the bilayer, a coherent and an incoherent one. Our microscopic model reveals that phonon-emission processes facilitate scattering events from the $K$ valley to other lower-energy $\mathrm{\Gamma }$ and $\mathrm{\Lambda }$ valleys in the bilayer. Our combined experimental and theoretical studies unequivocally establish different microscopic mechanisms that determine exciton quantum dynamics in TMDC monolayers and bilayers. Understanding exciton quantum dynamics provides critical guidance to the manipulation of spin-valley degrees of freedom in TMDC bilayers.

Probing optical excitations with high resolution is important for understanding their dynamics and controlling their interaction with other photonic elements. This can be done using state-of-the-art electron microscopes, which provide the means to sample optical excitations with combined meV–sub-nm energy-space resolution. For reciprocal photonic systems, electrons traveling in opposite directions produce identical signals, while this symmetry is broken in nonreciprocal structures. Here, we theoretically investigate this phenomenon by analyzing electron energy-loss spectroscopy (EELS) and cathodoluminescence (CL) for structures consisting of magnetically biased InAs as an instance of gyrotropic nonreciprocal material. We find that the spectral features associated with excitations of InAs films depend on the electron propagation direction in both EELS and CL, and can be tuned by varying the applied magnetic field within a relatively modest subtesla regime. The magnetic field modifies the optical field distribution of the sampled resonances, and this in turn produces a direction-dependent coupling to the electron. The present results pave the way to the use of electron microscope spectroscopies to explore the near-field characteristics of nonreciprocal systems with high spatial resolution.

Despite the fundamental nature of the edge state in topological physics, direct measurement of electronic and optical properties of the Fermi arcs of topological semimetals has posed a significant experimental challenge, as their response is often overwhelmed by the metallic bulk. However, laser-driven currents carried by surface and bulk states can propagate in different directions in nonsymmorphic crystals, allowing for the two components to be easily separated. Motivated by a recent theoretical prediction G. Chang et al., Phys. Rev. Lett. 124, 166404 (2020), we have measured the linear and circular photogalvanic effect currents deriving from the Fermi arcs of the nonsymmorphic, chiral Weyl semimetal RhSi over the 0.45–1.1 eV incident photon energy range. Our data are in good agreement with the predicted spectral shape of the circular photogalvanic effect as a function of photon energy, although the direction of the surface photocurrent departed from the theoretical expectation over the energy range studied. Surface currents arising from the linear photogalvanic effect were observed as well, with the unexpected result that only two of the six allowed tensor element were required to describe the measurements, suggesting an approximate emergent mirror symmetry inconsistent with the space group of the crystal.

Current quantum simulation experiments are starting to explore nonequilibrium many-body dynamics in previously inaccessible regimes in terms of system sizes and timescales. Therefore, the question emerges as to which observables are best suited to study the dynamics in such quantum many-body systems. Using machine learning techniques, we investigate the dynamics and, in particular, the thermalization behavior of an interacting quantum system that undergoes a nonequilibrium phase transition from an ergodic to a many-body localized phase. We employ supervised and unsupervised training methods to distinguish nonequilibrium from equilibrium data, using the network performance as a probe for the thermalization behavior of the system. We test our methods with experimental snapshots of ultracold atoms taken with a quantum gas microscope. Our results provide a path to analyze highly entangled large-scale quantum states for system sizes where numerical calculations of conventional observables become challenging.

We study kinetic Monte Carlo (KMC) descriptions of active particles. We show that, when they rely on purely persistent, active steps, their continuous-time limit is ill-defined, leading to the vanishing of trademark behaviors of active matter such as the motility-induced phase separation, ratchet effects, as well as to a diverging mechanical pressure. We then show how, under an appropriate scaling, mixing passive steps with active ones leads to a well-defined continuous-time limit that however differs from standard active dynamics. Finally, we propose new KMC algorithms whose continuous-time limits lead to the dynamics of active Ornstein-Uhlenbeck, active Brownian, and run-and-tumble particles.

Temporal interfaces introduced by abrupt switching of the constitutive parameters of unbounded media enable unusual wave phenomena. So far, their explorations have been mostly limited to lossless media. Yet, non-Hermitian phenomena leveraging material loss and gain, and their balanced combination in parity-time (PT)-symmetric systems, have been opening new vistas in photonics. Here, we unveil the role that temporal interfaces offer in non-Hermitian physics, introducing the dual of PT symmetry for temporal boundaries. Our findings reveal unexplored interference mechanisms enabling extreme energy manipulation, and open new scenarios for time-switched metamaterials, connecting them with the broad opportunities offered by non-Hermitian phenomena.

Observations in Earth’s turbulent magnetosheath downstream of a quasiparallel bow shock reveal a prevalence of electron-scale current sheets favorable for electron-only reconnection where ions are not coupled to the reconnecting magnetic fields. In small-scale turbulence, magnetic structures associated with intense current sheets are limited in all dimensions. And since the coupling of ions are constrained by a minimum length scale, the dynamics of electron reconnection is likely to be 3D. Here, both 2D and 3D kinetic particle-in-cell simulations are used to investigate electron-only reconnection, focusing on the reconnection rate and associated electron flows. A new form of 3D electron-only reconnection spontaneously develops where the magnetic X-line is localized in the out-of-plane ($z$) direction. The consequence is an enhancement of the reconnection rate compared with two dimensions, which results from differential mass flux out of the diffusion region along $z$, enabling a faster inflow velocity and thus a larger reconnection rate. This outflow along $z$ is due to the magnetic tension force in $z$ just as the conventional exhaust tension force, allowing particles to leave the diffusion region efficiently along $z$ unlike the 2D configuration.

We discuss the response of biopolymer filament bundles bound by transient cross-linkers to compressive loading. These systems admit a mechanical instability at stresses typically below that of traditional Euler buckling. In this instability, there is thermally activated pair production of topological defects that generate localized regions of bending—kinks. These kinks shorten the bundle’s effective length, thereby reducing the elastic energy of the mechanically loaded structure. This effect is the thermal analog of the Schwinger effect, in which a sufficiently large electric field causes electron-positron pair production. We discuss this analogy and describe the implications of this analysis for the mechanics of biopolymer filament bundles of various types under compression.

We here unify the field-theoretical approach to neuronal networks with large deviations theory. For a prototypical random recurrent network model with continuous-valued units, we show that the effective action is identical to the rate function and derive the latter using field theory. This rate function takes the form of a Kullback-Leibler divergence which enables data-driven inference of model parameters and calculation of fluctuations beyond mean-field theory. Lastly, we expose a regime with fluctuation-induced transitions between mean-field solutions.

The restricted Boltzmann machine is a basic machine learning tool able, in principle, to model the distribution of some arbitrary dataset. Its standard training procedure appears, however, delicate and obscure in many respects. We bring some new insights to it by considering the situation where the data have low intrinsic dimension, offering the possibility of an exact treatment and revealing a fundamental failure of the standard training procedure. The reasons for this failure—like the occurrence of first-order phase transitions during training—are clarified thanks to a Coulomb interactions reformulation of the model. In addition, a convex relaxation of the original optimization problem is formulated, thereby resulting in a unique solution, obtained in precise numerical form on $d=1$, 2 study cases, while a constrained linear regression solution can be conjectured on the basis of an information theory argument.

Counter-diabatic driving (CD) is a technique in quantum control theory designed to counteract nonadiabatic excitations and guide the system to follow its instantaneous energy eigenstates, and hence has applications in state preparation, quantum annealing, and quantum thermodynamics. However, in many practical situations, the effect of the environment cannot be neglected, and the performance of the CD is expected to degrade. To arrive at general bounds on the resulting error of CD in this situation we consider a driven spin-boson model as a prototypical setup. The inequalities we obtain, in terms of either the Bures angle or the fidelity, allow us to estimate the maximum error solely characterized by the parameters of the system and the bath. By utilizing the analytical form of the upper bound, we demonstrate that the error can be systematically reduced through optimization of the external driving protocol of the system. We also show that if we allow a time-dependent system-bath coupling angle, the obtained bound can be saturated and realizes unit fidelity.

Quantum many-body scars have been put forward as counterexamples to the eigenstate thermalization hypothesis. These atypical states are observed in a range of correlated models as long-lived oscillations of local observables in quench experiments starting from selected initial states. The long-time memory is a manifestation of quantum nonergodicity generally linked to a subextensive generation of entanglement entropy, the latter of which is widely used as a diagnostic for identifying quantum many-body scars numerically as low entanglement outliers. Here we show that by adding kinetic constraints to a fractionalized orthogonal metal, we can construct a minimal model with orthogonal quantum many-body scars leading to persistent oscillations with infinite lifetime coexisting with rapid volume-law entanglement generation. Our example provides new insights into the link between quantum ergodicity and many-body entanglement while opening new avenues for exotic nonequilibrium dynamics in strongly correlated multicomponent quantum systems.

We present a search for gravitational waves from the coalescence of subsolar-mass black hole binaries using data from the first half of Advanced LIGO and Virgo’s third observing run. The observation of a subsolar-mass black hole merger may be an indication of primordial origin; primordial black holes may contribute to the dark matter distribution. We search for black hole mergers where the primary mass is $0.1–7M_{\odot }$ and the secondary mass is $0.1–1M_{\odot }$. A variety of models predict the production and coalescence of binaries containing primordial black holes; some involve dynamical assembly, which may allow for residual eccentricity to be observed. For component masses $>0.5M_{\odot }$, we also search for sources in eccentric orbits, measured at a reference gravitational-wave frequency of 10 Hz, up to $e_{10}\sim 0.3$. We find no convincing candidates and place new upper limits on the rate of primordial black hole mergers. The merger rate of 0.5–0.5 $(1.0–1.0)M_{\odot }$ sources is $<7100(1200){\mathrm{Gpc}}^{-3}{\mathrm{yr}}^{-1}$. Our limits are $\sim 3–4$ times more constraining than prior analyses. Finally, we demonstrate how our limits can be used to constrain arbitrary models of the primordial black hole mass distribution and merger rate.

We show that the rate for dark-matter–electron scattering in an arbitrary material is determined by an experimentally measurable quantity, the complex dielectric function, for any dark matter interaction that couples to electron density. This formulation automatically includes many-body effects, eliminates all systematic theoretical uncertainties on the electronic wave functions, and allows a direct calibration of the spectrum by electromagnetic probes such as infrared spectroscopy, x-ray scattering, and electron energy-loss spectroscopy. Our formalism applies for several common benchmark models, including spin-independent interactions through scalar and vector mediators of arbitrary mass. We discuss the consequences for standard semiconductor and superconductor targets and find that the true reach of superconductor detectors for light mediators exceeds previous estimates by several orders of magnitude, with further enhancements possible due to the low-energy tail of the plasmon. Using a heavy-fermion superconductor as an example, we show how our formulation allows a rapid and systematic investigation of novel electron scattering targets.

We present a search for the decays of a neutral scalar boson produced by kaons decaying at rest, in the context of the Higgs portal model, using the MicroBooNE detector. We analyze data triggered in time with the Fermilab NuMI neutrino beam spill, with an exposure of $1.93\times {10}^{20}$ protons on target. We look for monoenergetic scalars that come from the direction of the NuMI hadron absorber, at a distance of 100 m from the detector, and decay to electron-positron pairs. We observe one candidate event, with a standard model background prediction of $1.9\pm 0.8$. We set an upper limit on the scalar–Higgs mixing angle of $\theta <(3.3-4.6)\times {10}^{-4}$ at the 95% confidence level for scalar boson masses in the range $(100–200)\mathrm{MeV}/c^2$. We exclude, at the 95% confidence level, the remaining model parameters required to explain the central value of a possible excess of $K_L^0\to {\pi }^0\nu \overline{\nu }$ decays reported by the KOTO collaboration. We also provide a model-independent limit on a new boson $X$ produced in $K\to \pi X$ decays and decaying to $e^{+}{e}^{-}$.

Multijet rates at hadron colliders provide a unique possibility for probing quantum chromodynamics (QCD), the theory of strong interactions. By comparing theory predictions with collider data, one can directly test perturbative QCD, extract fundamental parameters like the strong coupling ${\alpha }_s$, and search for physics beyond the standard model. In this work we calculate, for the first time, the next-to-next-to-leading order (NNLO) QCD corrections to typical three-jet observables and to differential three-to-two jet ratios. The calculation is complete apart from the three-jet double virtual contributions which are included in the leading-color approximation. We demonstrate that the inclusion of the NNLO corrections significantly reduces the dependence of those observables on the factorization and renormalization scales. Besides its phenomenological value, this proof-of-principle computation represents a milestone in perturbative QCD.

Boosting second-order optical nonlinear frequency conversion over subwavelength thickness has long been pursued through optical resonance in micro- and nanophotonics. However, the availability of thin film materials with high second-order nonlinearity is limited to III-V semiconductors, which have low transparency in the visible. Here, we experimentally demonstrated strongly enhanced second harmonic generation in one-dimensional heterostructure cavities on thin film lithium niobate. A guided-mode resonance resonator and distributed Bragg reflectors are combined for both efficient coupling and electromagnetic field localization. Over 1200 times second harmonic generation enhancement is experimentally realized compared with flat thin film lithium niobate through optimizing the trade-off between quality factor and mode volume, leading to a record high normalized conversion efficiency of $2.03\times {10}^{-5}{\mathrm{cm}}^2/\mathrm{GW}$ under $1.92\mathrm{MW}/{\mathrm{cm}}^2$ pump intensity. Our approach could inspire the miniaturization and integration of compact resonant nonlinear photonic devices on thin film lithium niobate.