We report an experimental investigation of quantum correlations in a two-qutrit spin system in a single nitrogen-vacancy center in diamond at room temperatures. Quantum entanglement between two qutrits was observed at room temperature, and the existence of nonclassical correlations beyond entanglement in the qutrit case has been revealed. Our work demonstrates the potential of the NV centers as the multiqutrit system to execute quantum information tasks and provides a powerful experimental platform for studying the fundamental physics of high-dimensional quantum systems in the future.

Axions with masses of order keV can be produced in great abundance within the Solar core. The majority of Sun-produced axions escape to infinity, but a small fraction of the flux is produced with speeds below the escape velocity. Over time, this process populates a basin of slow-moving axions trapped on bound orbits. These axions can decay to two photons, yielding an observable signature. We place the first limits on this solar basin of axions using recent quiescent solar observations made by the NuSTAR x-ray telescope. We compare three different methodologies for setting constraints, and obtain world-leading limits for axions with masses between 5 and 30 keV, in some cases improving on stellar cooling bounds by more than an order of magnitude in coupling.

We point out that an infinite class of Witten diagrams is invariant under a Yangian symmetry. These diagrams are building blocks of holographic correlators and are related by a web of differential recursion relations. We show that Yangian invariance is equivalent to the consistency conditions of the recursion relations.

Quantum coherences in electronic motions play a critical role in determining the pathways and outcomes of virtually all photophysical and photochemical molecular processes. However, the direct observation of electronic coherences in the vicinity of conical intersections remains a formidable challenge. We propose a novel time-resolved twisted x-ray diffraction technique that can directly monitor the electronic coherences created as the molecule passes through a conical intersection. We show that the contribution of electronic populations to this signal is canceled out when using twisted x-ray beams that carry a light orbital angular momentum, providing a direct measurement of transient electronic coherences in gas-phase molecules.

Enantiodetection of chiral molecules is important to chemical reaction control and biological function designs. Traditional optical methods of enantiodetection rely on the weak magnetic-dipole or electric-quadrupole interactions, and in turn suffer from the weak signal and low sensitivity. We propose a new optical enantiodetection method to determine the enantiomeric excess via two-dimensional (2D) spectroscopy of the chiral mixture driven by three electromagnetic fields. The quantities of left- and right-handed chiral molecules are reflected by the intensities of different peaks on the 2D spectrum, separated by the chirality-dependent frequency shifts resulting from the relative strong electric-dipole interactions between the chiral molecules and the driving fields. Thus, the enantiomeric excess can be determined via the intensity ratio of the peaks for the two enantiomers.

Spin current is a key to realizing various phenomena and functionalities related to spintronics. Recently, the possibility of generating spin current through a photogalvanic effect of magnons was pointed out theoretically. However, neither a candidate material nor a general formula for calculating the photogalvanic spin current in materials is known so far. In this Letter, we develop a general formula for the photogalvanic spin current through a magnetic resonance process. This mechanism involves a one-magnon excitation process in contrast to the two-particle processes studied in earlier works. Using the formula, we show that GHz and THz waves create a large photogalvanic spin current in the antiferromagnetic phase of bilayer ${\mathrm{CrI}}_3$ and ${\mathrm{CrBr}}_3$. The large spin current arises from an optical process involving two magnon bands, which is a contribution unknown to date. This spin current appears only in the antiferromagnetic ordered phase and is reversible by controlling the order parameter. These results open a route to material design for the photogalvanic effect of magnetic excitations.

Characterizing elementary excitations in quantum fluids is essential to study their collective effects. We present an original angle-resolved coherent probe spectroscopy technique to study the dispersion of these excitation modes in a fluid of polaritons under resonant pumping. Thanks to the unprecedented spectral and spatial resolution, we observe directly the low-energy phononic behavior and detect the negative-energy modes, i.e., the ghost branch, of the dispersion relation. In addition, we reveal narrow spectral features precursory of dynamical instabilities due to the intrinsic out-of-equilibrium nature of the system. This technique provides the missing tool for the quantitative study of quantum hydrodynamics in polariton fluids.

Drug persistence is a phenomenon by which a small percentage of cancer cells survive the presentation of targeted therapy by transitioning to a quiescent state. Eventually some of these persister cells can transition back to an active growing state and give rise to resistant tumors. Here we introduce a quantitative genetics approach to drug-exposed populations of cancer cells in order to interpret recent experimental data regarding inheritance of persister probability. Our results indicate that alternating periods of drug treatment and drug removal may not be an effective strategy for eliminating persisters.

Second order quantum phase transitions, with well-known features such as long-range entanglement, symmetry breaking, and gap closing, exhibit quantum enhancement for sensing at criticality. However, it is unclear which of these features are responsible for this enhancement. To address this issue, we investigate phase transitions in free-fermionic topological systems that exhibit neither symmetry-breaking nor long-range entanglement. We analytically demonstrate that quantum enhanced sensing is possible using topological edge states near the phase boundary. Remarkably, such enhancement also endures for ground states of such models that are accessible in solid state experiments. We illustrate the results with 1D Su-Schrieffer-Heeger chain and a 2D Chern insulator which are both experimentally accessible. While neither symmetry-breaking nor long-range entanglement are essential, gap closing remains as the major candidate for the ultimate source of quantum enhanced sensing. In addition, we also provide a fixed and simple measurement strategy that achieves near-optimal precision for sensing using generic edge states irrespective of the parameter value. This paves the way for development of topological quantum sensors which are expected to also be robust against local perturbations.

The transverse-field Ising model is one of the fundamental models in quantum many-body systems, yet a full understanding of its dynamics remains elusive in higher than one dimension. Here, we show for the first time the breakdown of ergodicity in $d$-dimensional Ising models with a weak transverse field in a prethermal regime. We demonstrate that novel Hilbert-space fragmentation occurs in the effective nonintegrable model with $d\ge 2$ as a consequence of only one emergent global conservation law of the domain wall number. Our results indicate nontrivial initial-state dependence for nonequilibrium dynamics of the Ising models with a weak transverse field.

We study the generation and evolution of second-order energy-density perturbations arising from primordial gravitational waves. Such “tensor-induced scalar modes” approximately evolve as standard linear matter perturbations and may leave observable signatures in the large-scale structure of the Universe. We study the imprint on the matter power spectrum of some primordial models which predict a large gravitational-wave signal at high frequencies. This novel mechanism, in principle, allows us to constrain or detect primordial gravitational waves by looking at specific features in the matter or galaxy power spectrum, thereby allowing us to probe them on a range of scales unexplored so far.

While non-Hermitian Hamiltonians have been experimentally realized in cold atom systems, it remains an outstanding open question of how to experimentally measure their complex energy spectra in momentum space for a realistic system with boundaries. The existence of non-Hermitian skin effects may make the question even more difficult to address given the fact that energy spectra for a system with open boundaries are dramatically different from those in momentum space; the fact may even lead to the notion that momentum-space band structures are not experimentally accessible for a system with open boundaries. Here, we generalize the widely used radio-frequency spectroscopy to measure both real and imaginary parts of complex energy spectra of a non-Hermitian quantum system for either bosonic or fermionic atoms. By weakly coupling the energy levels of a non-Hermitian system to auxiliary energy levels, we theoretically derive a formula showing that the decay of atoms on the auxiliary energy levels reflects the real and imaginary parts of energy spectra in momentum space. We further prove that measurement outcomes are independent of boundary conditions in the thermodynamic limit, providing strong evidence that the energy spectrum in momentum space is experimentally measurable. We finally apply our non-Hermitian absorption spectroscopy protocol to the Hatano-Nelson model and non-Hermitian Weyl semimetals to demonstrate its feasibility.

We reveal a wealth of nonlinear and recoil effects in the interaction between individual low-energy electrons ($\lesssim 100\mathrm{eV}$) and samples comprising a discrete number of states. Adopting a quantum theoretical description of combined free-electron and two-level systems, we find a maximum achievable excitation probability of 100%, which requires specific conditions relating to the coupling strength and the transition symmetry, as we illustrate through calculations for dipolar and quadrupolar modes. Strong recoil effects are observed when the kinetic energy of the probe lies close to the transition threshold, although the associated probability remains independent of the electron wave function even when fully accounting for nonlinear interactions with arbitrarily complex multilevel samples. Our work reveals the potential of free electrons to control localized excitations and delineates the boundaries of such control.

We investigate ultracold collisions in a novel mixture of ${}^6\mathrm{Li}$ and ${}^{53}\mathrm{Cr}$ fermionic atoms, discovering more than 50 interspecies Feshbach resonances via loss spectroscopy. Building a full coupled-channel model, we unambiguously characterize the ${}^6\mathrm{Li}\text{−}{}^{53}\mathrm{Cr}$ scattering properties and yield predictions for other isotopic pairs. In particular, we identify various Feshbach resonances that enable the controlled tuning of elastic $s$- and $p$-wave ${}^6\mathrm{Li}\text{−}{}^{53}\mathrm{Cr}$ interactions. Our studies thus make lithium-chromium mixtures emerge as optimally suited platforms for the experimental search of elusive few- and many-body regimes of highly correlated fermionic matter, and for the realization of a new class of ultracold polar molecules possessing both electric and magnetic dipole moments.

Two-dimensional confinement of lattices produces a variety of order and disorder phenomena. When the confining walls have atomic granularity, unique structural phases are expected, of relevance in nanotribology, porous materials, or intercalation compounds where, e.g., electronic states can emerge accordingly. The interlayer’s own order is frustrated by the competing interactions exerted by the two confining surfaces. We revisit the concept of orientational ordering, introduced by Novaco and McTague to describe the twist of incommensurate monolayers on crystalline surfaces. We predict a two-way twist of the monolayer as its density increases. We discover such a behavior in alkali atom monolayers (sodium, cesium) confined between graphene and an iridium surface, using scanning tunneling microscopy and electron diffraction.

Disclinations in a 2D sheet create regions of Gaussian curvature whose inversion produces a reconfigurable surface with many distinct metastable shapes, as shown by molecular dynamics of a disclinated graphene monolayer. This material has a near-Gaussian “density of shapes” and an effectively antiferromagnetic interaction between adjacent cones. $\mathrm{A}\sim 10\mathrm{nm}$ patch has hundreds of distinct metastable shapes with tunable stability and topography on the size scale of biomolecules. As every conical disclination provides an Ising-like degree of freedom, we call this technique “Isigami.”