The long search for insulating materials that possess low-energy quasiparticles carrying electron’s quantum numbers except charge—inspired by the neutral spin-$1/2$ excitations, the so-called spinons, exhibited by Anderson’s resonating-valence-bond state—seems to have reached a turning point after the discovery of several Mott insulators displaying the same thermal and magnetic properties as metals, including quantum oscillations in a magnetic field. Here, we show that such anomalous behavior is not inconsistent with Landau’s Fermi liquid theory of quasiparticles at a Luttinger surface. That is the manifold of zeros within the Brillouin zone of the single-particle Green’s function at zero frequency, and which thus defines the spinon Fermi surface conjectured by Anderson.

The determination of depth profiles across interfaces is of primary importance in many scientific and technological areas. Photoemission spectroscopy is in principle well suited for this purpose, yet a quantitative implementation for investigations of liquid-vapor interfaces is hindered by the lack of understanding of electron-scattering processes in liquids. Previous studies have shown, however, that core-level photoelectron angular distributions (PADs) are altered by depth-dependent elastic electron scattering and can, thus, reveal information on the depth distribution of species across the interface. Here, we explore this concept further and show that the experimental anisotropy parameter characterizing the PAD scales linearly with the average distance of atoms along the surface normal obtained by molecular dynamics simulations. This behavior can be accounted for in the low-collision-number regime. We also show that results for different atomic species can be compared on the same length scale. We demonstrate that atoms separated by about 1 Å along the surface normal can be clearly distinguished with this method, achieving excellent depth resolution.

We report solutions for stable compound solitons in a three-dimensional quasi-phase-matched photonic crystal with the quadratic (${\chi }^{(2)}$) nonlinearity. The photonic crystal is introduced with a checkerboard structure, which can be realized by means of the available technology. The solitons are built as four-peak vortex modes of two types, rhombuses and squares (intersite- and onsite-centered self-trapped states, respectively). Their stability areas are identified in the system’s parametric space (rhombuses occupy an essentially broader stability domain), while all bright vortex solitons are subject to strong azimuthal instability in uniform ${\chi }^{(2)}$ media. Possibilities for experimental realization of the solitons are outlined.

Chiral active fluids break both time-reversal and parity symmetry, leading to exotic transport phenomena unobservable in ordinary passive fluids. We develop a generalized Green-Kubo relation for the anomalous lift experienced by a passive tracer suspended in a two-dimensional chiral active fluid subjected to an applied force. This anomalous lift is characterized by a transport coefficient termed the odd mobility. We validate our generalized response theory using molecular dynamics simulations, and we show that the asymmetric tracer mobility may be understood mechanically in terms of asymmetric deformations of the tracer-fluid density distribution function. We show that the even and odd components of the mobility decay at different rates with tracer size, suggesting the possibility of size-based particle separation using a chiral active working fluid.

Identifying and characterizing mutational paths is an important issue in evolutionary biology, with potential applications to bioengineering. We here propose an algorithm to sample mutational paths, which we benchmark on exactly solvable models of proteins in silico, and apply to data-driven models of natural proteins learned from sequence data with restricted Boltzmann machines. We then use mean-field theory to characterize paths for different mutational dynamics of interest, and to extend Kimura’s estimate of evolutionary distances to sequence-based epistatic models of selection.

We analyze the recoil corrections in superallowed beta decays of $T=1$, $J^P=0^{+}$ nuclei by fixing the mean square charged weak radius model independently using the data of multiple charge radii across the nuclear isotriplet. By comparing to model estimations, we argue that the existing theory uncertainty in the statistical rate function $f$ might have been substantially underestimated. We discuss the implications of our proposed strategy for precision tests of the standard model, including a potential alleviation of the first-row CKM unitarity deficit, and motivate new experiments for charge radii measurements.

We propose a universal framework to compute record age statistics of a stochastic time series that undergoes random restarts. The proposed framework makes minimal assumptions on the underlying process and is furthermore suited to treat generic restart protocols going beyond the Markovian setting. After benchmarking the framework for classical random walks on the 1D lattice, we derive a universal criterion underpinning the impact of restart on the age of the $n$th record for generic time series with nearest-neighbor transitions. Crucially, the criterion contains a penalty of order $n$ that puts strong constraints on restart expediting the creation of records, as compared to the simple first-passage completion. The applicability of our approach is further demonstrated on an aggregation-shattering process where we compute the typical growth rates of aggregate sizes. This unified framework paves the way to explore record statistics of time series under restart in a wide range of complex systems.

Defective spectral degeneracy, known as exceptional point (EP), lies at the heart of various intriguing phenomena in optics, acoustics, and other nonconservative systems. Despite extensive studies in the past two decades, the collective behaviors (e.g., annihilation, coalescence, braiding, etc.) involving multiple exceptional points or lines and their interplay have been rarely understood. Here we put forward a universal non-Abelian conservation rule governing these collective behaviors in generic multiband non-Hermitian systems and uncover several counterintuitive phenomena. We demonstrate that two EPs with opposite charges (even the pairwise created) do not necessarily annihilate, depending on how they approach each other. Furthermore, we unveil that the conservation rule imposes strict constraints on the permissible exceptional-line configurations. It excludes structures like Hopf link yet permits novel staggered rings composed of noncommutative exceptional lines. These intriguing phenomena are illustrated by concrete models which could be readily implemented in platforms like coupled acoustic cavities, optical waveguides, and ring resonators. Our findings lay the cornerstone for a comprehensive understanding of the exceptional non-Abelian topology and shed light on the versatile manipulations and applications based on exceptional degeneracies in nonconservative systems.

The dynamics generated by non-Hermitian Hamiltonians are often less intuitive than those of conventional Hermitian systems. Even for models as simple as a complexified harmonic oscillator, the dynamics for generic initial states shows surprising features. Here we analyze the dynamics of the Husimi distribution in a semiclassical limit, illuminating the foundations of the full quantum evolution. The classical Husimi evolution is composed of two factors: (i) the initial Husimi distribution evaluated along phase-space trajectories and (ii) the final value of the norm corresponding to each phase-space point. Both factors conspire to lead to intriguing dynamical behaviors. We demonstrate how the full quantum dynamics unfolds on top of the classical Husimi dynamics for two instructive examples.

Despite the wide existence of protein aggregation in nature and its intimate connection to many human diseases, the underlying mechanism remains unclear. Here, we develop a molecular theory by systematically incorporating the self-consistent field theory for charged macromolecules into the dilute solution thermodynamics. The kinetic pathway is tracked without any restriction on the morphology of the aggregates. We find that protein aggregation at low salt concentrations is via a two-step nucleated process involving a conformational transition from metastable spherical oligomer to elongated fibril. The scaling analysis elucidates the electrostatic origin of the conformational transition: the fibril enters the screening region much earlier than the spherical aggregate. As salt concentration increases, the classical mode of one-step nucleation corresponding to macroscopic liquid-liquid phase separation is recovered. Our results reveal that the screened electrostatic interaction is essential for the existence of the metastable oligomer and its subsequent conformational transition to fibril. The theoretical predictions of the kinetic pathway and the morphology of the aggregates are in good agreement with the experimental observations of real proteins.

Parametrized quantum circuits can be used as quantum neural networks and have the potential to outperform their classical counterparts when trained for addressing learning problems. To date, much of the results on their performance on practical problems are heuristic in nature. In particular, the convergence rate for the training of quantum neural networks is not fully understood. Here, we analyze the dynamics of gradient descent for the training error of a class of variational quantum machine learning models. We define wide quantum neural networks as parametrized quantum circuits in the limit of a large number of qubits and variational parameters. Then, we find a simple analytic formula that captures the average behavior of their loss function and discuss the consequences of our findings. For example, for random quantum circuits, we predict and characterize an exponential decay of the residual training error as a function of the parameters of the system. Finally, we validate our analytic results with numerical experiments.

We show that non-Hermitian Ginibre random matrix behaviors emerge in spatially extended many-body quantum chaotic systems in the space direction, just as Hermitian random matrix behaviors emerge in chaotic systems in the time direction. Starting with translational invariant models, which can be associated with dual transfer matrices with complex-valued spectra, we show that the linear ramp of the spectral form factor necessitates that the dual spectra have nontrivial correlations, which in fact fall under the universality class of the Ginibre ensemble, demonstrated by computing the level spacing distribution and the dissipative spectral form factor. As a result of this connection, the exact spectral form factor for the Ginibre ensemble can be used to universally describe the spectral form factor for translational invariant many-body quantum chaotic systems in the scaling limit where $t$ and $L$ are large, while the ratio between $L$ and $L_{\mathrm{Th}}$, the many-body Thouless length is fixed. With appropriate variations of Ginibre models, we analytically demonstrate that our claim generalizes to models without translational invariance as well. The emergence of the Ginibre ensemble is a genuine consequence of the strongly interacting and spatially extended nature of the quantum chaotic systems we consider, unlike the traditional emergence of Hermitian random matrix ensembles.

We discuss the dynamics of three-dimensional Maxwell theory coupled to a level-$k$ Chern-Simons term. Motivated by S-duality in string theory, we argue that the theory admits an S-dual description. The S-dual theory contains a nongauge one-form field, previously proposed by Deser and Jackiw [Phys. Lett. 139B, 371 (1984).] and a level-$k$ $U(1)$ Chern-Simons term, ${\mathcal{Z}}_{\mathrm{MCS}}={\mathcal{Z}}_{\mathrm{DJ}}{\mathcal{Z}}_{\mathrm{CS}}$. The couplings to external electric and magnetic currents and their string theory realizations are also discussed.

Many attempts have been made to observe the decay of the Higgs boson to a photon and an invisible massless dark photon. For this decay to be potentially observable at the LHC, new mediators that communicate between the standard model and the dark photon must exist. In this Letter, we study bounds on such mediators coming from the Higgs signal strengths, oblique parameters, electric dipole moment of the electron, and unitarity. We find that the branching ratio of the Higgs boson to a photon and a dark photon is constrained to be far smaller than the sensitivity of current collider searches, thus calling for a reconsideration of current experimental efforts.

Photoelectron spectroscopy for chiral discrimination is routinely performed for low photoelectron kinetic energies (PKEs), whereas it is considered impossible for high PKEs. We demonstrate theoretically that chiral photoelectron spectroscopy for high PKEs is possible using chirality-selective molecular orientation. The photoelectron angular distribution associated with one-photon ionization by unpolarized light can be characterized by a single parameter, $\beta$. We show that most other anisotropy parameters are zero when $\beta$ is 2, as is often the case in the high PKEs. Exceptionally, odd-order anisotropy parameters are increased by a factor of 20 by orientation, even for high PKEs.

We demonstrate that dissociative ionization of ${\mathrm{H}}_2$ can be fully manipulated in an angle-time-resolved fashion, employing a polarization-skewed (PS) laser pulse in which the polarization vector rotates. The leading and falling edges of the PS laser pulse, characterized by unfolded field polarization, trigger, sequentially, parallel and perpendicular transitions of stretching ${\mathrm{H}}_2$ molecules, respectively. These transitions result in counterintuitive proton ejections that deviate significantly from the laser polarization directions. Our findings demonstrate that the reaction pathways can be controlled through fine-tuning the time-dependent polarization of the PS laser pulse. The experimental results are well reproduced using an intuitive wave-packet surface propagation simulation method. This research highlights the potential of PS laser pulses as powerful tweezers to resolve and manipulate complex laser-molecule interactions.

The moiré lattice has recently attracted broad interest in both solid-state physics and photonics where exotic phenomena in manipulating the quantum states are explored. In this work, we study the one-dimensional (1D) analogs of “moiré” lattices in a synthetic frequency dimension constructed by coupling two resonantly modulated ring resonators with different lengths. Unique features associated with the flatband manipulation as well as the flexible control of localization position inside each unit cell in the frequency dimension have been found, which can be controlled via the choice of flatband. Our work therefore provides insight into simulating moiré physics in 1D synthetic frequency space, which holds important promise for potential applications toward optical information processing.

Unitary control changes the absorption and emission of an object by transforming the external light modes. It is widely used and underlies coherent perfect absorption. Yet two basic questions remain unanswered: For a given object under unitary control, what absorptivity $\alpha$, emissivity $e$, and their contrast $\delta =e-\alpha$ are attainable? How to obtain a given $\alpha$, $e$, or $\delta$? We answer both questions using the mathematics of majorization. We show that unitary control can achieve perfect violation or preservation of Kirchhoff’s law in nonreciprocal objects, and uniform absorption or emission for any object.