Continuous spin excitations are widely recognized as one of the hallmarks of novel spin states in quantum magnets, such as quantum spin liquids (QSLs). Here, we report the observation of such kind of excitations in ${\mathrm{K}}_2{\mathrm{Ni}}_2({\mathrm{SO}}_4{)}_3$, which consists of two sets of intersected spin-1 (${\mathrm{Ni}}^{2+}$) trillium lattices. Our inelastic neutron scattering measurement on single crystals clearly shows a dominant excitation continuum, which exhibits a distinct temperature-dependent behavior from that of spin waves, and is rooted in strong quantum spin fluctuations. Further using the self-consistent-Gaussian-approximation method, we determine that the fourth- and fifth-nearest-neighbor exchange interactions are dominant. These two bonds together form a unique three-dimensional network of corner-sharing tetrahedra, which we name as a “hypertrillium” lattice. Our results provide direct evidence for the existence of QSL features in ${\mathrm{K}}_2{\mathrm{Ni}}_2({\mathrm{SO}}_4{)}_3$ and highlight the potential for the hypertrillium lattice to host frustrated quantum magnetism.

The observation of traveling breathers (TBs) with large-amplitude oscillatory tails realizes an almost 50-year-old theoretical prediction [E. A. Kuznetsov and A. V. Mikhailov, Stability of stationary waves in nonlinear weakly dispersive media, Zh. Eksp. Teor. Fiz. 67, 1717 (1974) [E. A. Kuznetsov and A. V. MikhailovSov. Phys. JETP 40, 855 (1975)] ] and generalizes the notion of a breather. Two strongly nonlinear TB families are created in a core-annular flow by interacting a soliton and a nonlinear periodic (cnoidal) carrier. Bright and dark TBs are observed to move faster or slower, respectively, than the carrier while imparting a phase shift. Agreement with model equations is achieved. Scattering of the TBs is observed to be physically elastic. The observed TBs generalize to many continuum and discrete systems.

We show that the second-order, two-time correlation functions for phonons and photons emitted from a vibronic molecule in a thermal bath result in bunching and antibunching (a purely quantum effect), respectively. Signatures relating to phonon exchange with the environment are revealed in photon-photon correlations. We demonstrate that cross-correlation functions have a strong dependence on the order of detection giving insight into how phonon dynamics influences the emission of light. This work offers new opportunities to investigate quantum effects in condensed-phase molecular systems.

Near-field thermal emission largely exceeds blackbody radiation, owing to spectrally sharp emission in surface polaritons. We turn the Casimir-Polder interaction between $\mathrm{Cs}(7P_{1/2})$ and a sapphire interface into a sensor sharply filtering, at 24.687 THz, the near-field sapphire emission at $\sim 24.5\mathrm{THz}$. The temperature evolution of the sapphire mode is demonstrated. The Cs sensor, sensitive to both dispersion and dissipation, suggests the polariton to be redshifted and sharper, as compared, up to 1100 K, to predictions from far-field sapphire emission, affected by birefringence and multiple resonances.

We report the observation of a set of coherent high frequency electromagnetic fluctuations that leads to a turbulence induced self-regulating phenomenon in the DIII-D high bootstrap current fraction plasma. The fluctuations have frequency of $130–220\mathrm{kHz}$, the poloidal wavelength and phase velocity are $16–30{\mathrm{m}}^{-1}$ and $\sim 30\mathrm{km}/\mathrm{s}$, respectively, in the outboard midplane with the estimated toroidal mode number $n\sim 5-9$. The fluctuations are located in the internal transport barrier (ITB) region at large radius and are experimentally validated to be kinetic ballooning modes (KBM). Quasilinear estimation predicts the KBM to be able to drive experimental particle flux and non-negligible thermal flux, suggesting its significant role in regulating the ITB saturation.

The interplay of the nonequivalent corners in the Brillouin zone of transition metal dichalcogenides (TMDCs) has been investigated extensively. While experimental and theoretical works contributed to a detailed understanding of the relaxation of selective optical excitations and the related relaxation rates, only limited microscopic descriptions of stationary experiments are available so far. Here we present microscopic calculations for the nonequilibrium steady state properties of excitons during continuous wave pumping exemplary for monolayer ${\mathrm{MoSe}}_2$. We find sharp features in photoluminescence excitation spectra and degree of polarization which result from phonon assisted excitonic transitions dominating over exciton recombination and intervalley exchange coupling.

Relating thermodynamic and kinetic properties is a conceptual challenge with many practical benefits. Here, based on first principles, we derive a rigorous inequality relating the entropy and the dynamic propagator of particle configurations. It is universal and applicable to steady states arbitrarily far from thermodynamic equilibrium. Applying the general relation to diffusive dynamics yields a relation between the entropy and the (normal or anomalous) diffusion coefficient. The relation can be used to obtain useful bounds for the late-time diffusion coefficient from the calculated steady-state entropy or, conversely, to estimate the entropy based on measured diffusion coefficients. We demonstrate the validity and usefulness of the relation through several examples and discuss its broad range of applications, in particular, for systems far from equilibrium.

The pervasive phenomenon of friction has been studied at the nanoscale via a controlled manipulation of single atoms and molecules with a metallic tip, which enabled a precise determination of the static friction force necessary to initiate motion. However, little is known about the atomic dynamics during manipulation. Here, we reveal the complete manipulation process of a CO molecule on a Cu(110) surface at low temperatures using a combination of noncontact atomic force microscopy and density functional theory simulations. We found that an intermediate state, inaccessible for the far-tip position, is enabled in the reaction pathway for the close-tip position, which is crucial to understanding the manipulation process, including dynamic friction. Our results show how friction forces can be controlled and optimized, facilitating new fundamental insights for tribology.

A buckled sheet offers a reservoir of material that can be unfurled at a later time. For sufficiently thin yet stiff materials, this geometric process has a striking mechanical feature: when the slack runs out, the material locks to further extension. Here, we establish a simple route to a tunable locking material: a system with an interval where it is freely deformable under a given deformation mode, and where the endpoints of this interval can be changed continuously over a wide range. We demonstrate this type of mechanical response in a thin sheet formed into a cylindrical shell and subjected to axial twist and compression, and we rationalize our results with a simple geometric model.

Experiments over many decades are suggestive that the combination of cellular contractility and active phase separation in cell-matrix composites can enable spatiotemporal patterning in multicellular tissues across scales. To characterize these phenomena, we provide a general theory that incorporates active cellular contractility into the classical Cahn-Hilliard-Larché model for phase separation in passive viscoelastic solids. Within this framework, we show how a homogeneous cell-matrix mixture can be destabilized by activity via either a pitchfork or Hopf bifurcation, resulting in stable phase separation and/or traveling waves. Numerical simulations of the full equations allow us to track the evolution of the resulting self-organized patterns in periodic and mechanically constrained domains, and in different geometries. Altogether, our study underscores the importance of integrating both cellular activity and mechanical phase separation in understanding patterning in soft, active biosolids in both in vivo and in vitro settings.

We elucidate how the presence of higher-form symmetries affects the dynamics of thermalization in isolated quantum systems. Under reasonable assumptions, we analytically show that a $p$-form symmetry in a ($d+1$)-dimensional quantum field theory leads to the breakdown of the eigenstate thermalization hypothesis for many nontrivial ($d-p$)-dimensional observables. For discrete higher-form (i.e., $p\ge 1$) symmetry, this indicates the absence of thermalization for observables that are nonlocal but much smaller than the whole system size without any local conserved quantities. We numerically demonstrate this argument for the ($2+1$)-dimensional ${\mathbb{Z}}_2$ lattice gauge theory. While local observables such as the plaquette operator thermalize even for mixed symmetry sectors, the nonlocal observable exciting a magnetic dipole instead relaxes to the generalized Gibbs ensemble that takes account of the ${\mathbb{Z}}_2$ one-form symmetry.

We discuss recent lattice data for the $T_{cc}(3875{)}^{+}$ state to stress, for the first time, a potentially strong impact of left-hand cuts from the one-pion exchange on the pole extraction for near-threshold exotic states. In particular, if the left-hand cut is located close to the two-particle threshold, which happens naturally in the $D{D}^{*}$ system for the pion mass exceeding its physical value, the effective-range expansion is valid only in a very limited energy range up to the cut and as such is of little use to reliably extract the poles. Then, an accurate extraction of the pole locations requires the one-pion exchange to be implemented explicitly into the scattering amplitudes. Our findings are general and potentially relevant for a wide class of hadronic near-threshold states.

We present a general approach to excite robust dissipative three-dimensional and high-order solitons and breathers in passively driven nonlinear cavities. Our findings are illustrated in the paradigmatic example provided by an optical Kerr cavity with diffraction and anomalous dispersion, with the addition of an attractive three-dimensional parabolic potential. The potential breaks the translational symmetry along all directions, and impacts the system in a qualitatively unexpected manner: three-dimensional solitons, or light bullets, are the only existing and stable states for a given set of parameters. This property is extremely rare, if not unknown, in passive nonlinear systems. As a result, the excitation of the cavity with any input field leads to the deterministic formation of a target soliton or breather, with a spatiotemporal profile that unambiguously corresponds to the given cavity and pumping conditions. In addition, the tuning of the potential width along the temporal direction results in the existence of a plethora of stable asymmetric solitons. Our results may provide a solid route toward the observation of dissipative light bullets and three-dimensional breathers.

Understanding and achieving concurrent modulation of amplitude and frequency, particularly adjusting one quantity and simultaneously sustaining the other at an invariant level, are of paramount importance for complex biophysical systems, including the signal pathway where different frequency indicates different upstream signal yielding a certain downstream physiological function while different amplitude further determines different efficacy of a downstream output. However, such modulators with clearly described and universally valid mechanisms are still lacking. Here, we rigorously propose an easy-to-use control strategy containing only one or two steps, leveraging the nonlinearity in the modulated systems to decouple frequency and amplitude in a noncomputational manner. The strategy’s efficacy is demonstrated using representative biochemical systems and, thus, it could be potentially applicable to modulating rhythms in experiments of biochemistry and synthetic biology.

Intrinsic quantum randomness is produced when a projective measurement on a given basis is implemented on a pure state that is not an element of the basis. The prepared state and implemented measurement are perfectly known, yet the measured result cannot be deterministically predicted. In realistic situations, however, measurements and state preparation are always noisy, which introduces a component of stochasticity in the outputs that is not a consequence of the intrinsic randomness of quantum theory. Operationally, this stochasticity is modeled through classical or quantum correlations with an eavesdropper, Eve, whose goal is to make the best guess about the outcomes produced in the experiment. In this Letter, we study Eve’s maximum guessing probability when she is allowed to have correlations with both the state and the measurement. We show that, unlike the case of projective measurements (as it was already known) or pure states (as we prove), in the setting of generalized measurements and mixed states, Eve’s guessing probability differs depending on whether she can prepare classically or quantumly correlated strategies.