We develop an action formalism to calculate probabilities of rare events in cluster-cluster aggregation for arbitrary collision kernels and establish a pathwise large deviation principle with total mass being the rate. As an application, the rate function for the number of surviving particles as well as the optimal evolution trajectory are calculated exactly for the constant, sum, and product kernels. For the product kernel, we argue that the second derivative of the rate function has a discontinuity. The theoretical results agree with simulations tailored to the calculation of rare events.

The limit of energy saving in the control of small systems has recently attracted much interest due to the concept refinement of the Maxwell demon. Inspired by a newly proposed set of fluctuation theorems, we report the first experimental verification of these equalities and inequalities in an ultracold ${}^{40}{\mathrm{Ca}}^{+}$ ion system, confirming the intrinsic nonequilibrium in the system due to involvement of the demon. Based on elaborately designed demon-involved control protocols, such as the Szilard engine protocol, we provide experimentally quantitative evidence of the dissipative information and observe tighter bounds of both the extracted work and the demon’s efficacy than the limits predicted by the Sagawa-Ueda theorem. Our results substantiate a close connection between the physical nature of information and nonequilibrium processes at the microscale, which help to further understand the thermodynamic characteristics of information and the optimal design of nanoscale and smaller systems.

We derive necessary and sufficient conditions under which a large class of relativistic generalizations of Braginskii’s magnetohydrodynamics with shear, bulk, and heat diffusion effects is causal and strongly hyperbolic in the fully nonlinear regime in curved spacetime. We find that causality severely constrains the size of nonideal effects and the onset of kinetic instabilities. Our results are crucial for assessing the regime of validity of fluid dynamical simulations of plasmas near supermassive black holes.

In classical fluids, the Weber number is a dimensionless parameter that characterizes the flow of a multiphase fluid. The superfluid analogy of a classical multiphase fluid can be realized in a system of two or more immiscible Bose-Einstein condensates. These superfluid mixtures have been shown to display a wider variety of exotic dynamics than their single component counterparts. Here we systematically study the dynamics of a binary immiscible Bose-Einstein condensate in two dimensions, where a small bubble of the second component is used to “stir” the first component. We begin by rigorously mapping out the critical velocity for vortex shedding as a function of the size of the bubble, in analogy to the critical velocity of a laser spoon. Observing that the dynamics of the system depend on the initial size and velocity of the bubble, we then show that a dimensionless parameter with the same form as the Weber number accurately predicts the resulting bubble fragmentation.

Photon-pair correlations in spontaneous parametric down-conversion are ubiquitous in quantum photonics. The ability to engineer their properties for optimizing a specific task is essential, but often challenging in practice. We demonstrate the shaping of spatial correlations between entangled photons in the form of arbitrary amplitude and phase objects. By doing this, we encode image information within the pair correlations, making it undetectable by conventional intensity measurements. It enables the transmission of complex, high-dimensional information using quantum correlations of photons, which can be useful for developing quantum communication and imaging protocols.

We unveil a new scenario for the formation of dissipative localized structures in nonlinear systems. Commonly, the formation of such structures arises from the connection of a homogeneous steady state with either another homogeneous solution or a pattern. Both scenarios, typically found in cavities with normal and anomalous dispersion, respectively, exhibit unique fingerprints and particular features that characterize their behavior. However, we show that the introduction of a periodic non-Hermitian modulation in Kerr cavities hybridizes the two established soliton formation mechanisms, embodying the particular fingerprints of both. In the resulting novel scenario, the stationary states acquire a dual behavior, playing the role that was unambiguously attributed to either homogeneous states or patterns. These fundamental findings have profound practical implications for frequency comb generation, introducing unprecedented reversible mechanisms for real-time manipulation.

The skyrmion crystal (SkX) and helix (HL) phases, present in typical chiral magnets, can each be considered as forms of density waves but with distinct topologies. The SkX exhibits gyrodynamics analogous to electrons under a magnetic field, while the HL state resembles topological trivial spin density waves. However, unlike the charge density waves, the theoretical analysis of the sliding motion of SkX and HL remains unclear, especially regarding the similarities and differences in sliding dynamics between these two spin density waves. In this Letter, we systematically explore the sliding dynamics of SkX and HL in chiral magnets in the limit of large current density. We demonstrate that the sliding dynamics of both SkX and HL can be unified within the same theoretical framework as density waves, despite their distinct microscopic orders. Furthermore, we highlight the significant role of gyrotropic sliding induced by impurity effects in the SkX state, underscoring the impact of nontrivial topology on the sliding motion of density waves. Our theoretical analysis shows that the effect of impurity pinning is much stronger in HL compared with SkX, i.e., ${\chi }^{\mathrm{SkX}}/{\chi }^{\mathrm{HL}}\sim {\alpha }^2$ (${\chi }^{\mathrm{SkX}}$, ${\chi }^{\mathrm{HL}}$: susceptibility to the impurity potential, $\alpha$ ($\ll 1$) is the Gilbert damping). Moreover, the velocity correction is mostly in the transverse direction to the current in SkX. These results are further substantiated by realistic Landau-Lifshitz-Gilbert simulations.

The extraordinary properties of the Kitaev model have motivated an intense search for new physics in materials that combine geometrical and bond frustration. In this Letter, we employ inelastic neutron scattering, spin wave theory, and exact diagonalization to study the spin dynamics in the perfect triangular-lattice antiferromagnet (TLAF) ${\mathrm{CsCeSe}}_2$. This material orders into a stripe phase, which is demonstrated to arise as a consequence of the off-diagonal bond-dependent terms in the spin Hamiltonian. By studying the spin dynamics at intermediate fields, we identify an interaction between the single-magnon state and the two-magnon continuum that causes decay of coherent magnon excitations, level repulsion, and transfer of spectral weight to the continuum that are controlled by the strength of the magnetic field. Our results provide a microscopic mechanism for the stabilization of the stripe phase in TLAF and show how complex many-body physics can be present in the spin dynamics in a magnet with strong Kitaev coupling even in an ordered ground state.

Vortex crystals are commonly observed in ultrathin ferroelectrics. However, a clear physical picture of origin of this topological state is currently lacking. Here, we show that vortex crystallization in ultrathin $\mathrm{Pb}({\mathrm{Zr}}_{0.4},{\mathrm{Ti}}_{0.6}){\mathrm{O}}_3$ films stems from the softening of a phonon mode and can be described as a $Z_2\times \mathrm{SU}(1)$ symmetry-breaking transition. This result sheds light on the topology of the polar vortex patterns and bridges polar vortices with smectic phases, spin spirals, and other modulated states. Finally, we predict a resonant switching of the vortex tube orientation driven by midinfrared laser light which could enable new technologies.

The longitudinal nonreciprocal charge transport (NCT) in crystalline materials is a highly nontrivial phenomenon, motivating the design of next generation two-terminal rectification devices (e.g., semiconductor diodes beyond PN junctions). The practical application of such devices is built upon crystalline materials whose longitudinal NCT occurs at room temperature and under low magnetic field. However, materials of this type are rather rare and elusive, and theory guiding the discovery of these materials is lacking. Here, we develop such a theory within the framework of semiclassical Boltzmann transport theory. By symmetry analysis, we classify the complete 122 magnetic point groups with respect to the longitudinal NCT phenomenon. The symmetry-adapted Hamiltonian analysis further uncovers a previously overlooked mechanism for this phenomenon. Our theory guides the first-principles prediction of longitudinal NCT in multiferroic $ϵ\text{−}{\mathrm{Fe}}_2{\mathrm{O}}_3$ semiconductor that possibly occurs at room temperature, without the application of external magnetic field. These findings advance our fundamental understandings of longitudinal NCT in crystalline materials, and aid the corresponding materials discoveries.

The quantum coherent dynamics of a vibronic wave packet in a molecule passing through a conical intersection can be revealed using attosecond transient coherent Raman spectroscopy. In particular, the time evolution of the electronic coherence can be monitored in the presence of vibrational dynamics. So far, the technique has been investigated without including environmental quantum noise. Here, we employ the numerically exact hierarchy equation of motion approach to show that the transient coherent Raman signals are robust and accessible on times of up to a few hundred femtoseconds with respect to electonic and vibrational dephasing.

The detrimental impact of noise on sensing performance in quantum metrology has been widely recognized by researchers in the field. However, there are no explicit fundamental laws of physics stating that noise invariably weakens quantum metrology. We reveal that phase-covariant noise either degrades or remains neutral to sensing precision, whereas non-phase-covariant noise can potentially enhance parameter estimation, surpassing even the ultimate precision limit achievable in the absence of noise. This implies that a non-Hermitian quantum sensor may outperform its Hermitian counterpart in terms of sensing performance. To illustrate and validate our theory, we present several paradigmatic examples of magnetic field metrology.

We investigate the formation of high-redshift supermassive black holes (SMBHs) via the direct collapse of baryonic clouds, where the unwanted formation of molecular hydrogen is successfully suppressed by a Lyman-Werner (LW) photon background from relic particle decay. We improve on existing studies by dynamically simulating the collapse, accounting for the adiabatic contraction of the DM halo, as well as the in situ production of the LW photons within the cloud which reduce the impact of the cloud’s shielding. We find a viable parameter space where the decay of either some of the dark matter or all of a subdominant decaying species successfully allows direct collapse of the cloud to a SMBH.

The direct imaging of time-evolving molecular charge densities on atomistic scale and at femtosecond resolution has long been an elusive task. In this theoretical study, we propose a self-heterodyne electron diffraction technique based on single electron pulses. The electron is split into two beams, one passes through the sample and its interference with the second beam produces a heterodyne diffraction signal that images the charge density. Application to probing the ultrafast electronic dynamics in Mg-phthalocyanine demonstrates its potential for imaging chemical dynamics.

We propose and demonstrate a radio-frequency (rf) atomic magnetometer based on parametric resonances. Previously, most rf atomic magnetometers are based on magnetic resonances and their sensitivities are often limited by spin-exchange relaxation. Here, we introduce a novel scheme for an rf magnetometer where the rf magnetic field is measured by exciting the parametric resonances instead of magnetic resonances using parametric modulation fields. In this way, the spin-exchange relaxation is almost eliminated. Benefiting from the low spin relaxation rate, the parametric resonance scheme exhibits a narrower linewidth and stronger signal, which results in a higher sensitivity. With a $6\times 6\times 3{\mathrm{mm}}^3$ Rb atomic vapor cell, we developed an rf atomic magnetometer with a noise floor of $2\mathrm{fT}/{\mathrm{Hz}}^{1/2}$, which is about one order of magnitude higher than the sensitivity achieved in the magnetic-resonance-based scheme. The presented rf detection scheme holds promise in advancing rf atomic magnetometers and brings new insight into their various applications.

We analyze the transitions between established phases of the El Niño Southern Oscillation (ENSO) by surveying the daily data of the southern oscillation index from an entropic viewpoint using the framework of stochastic statistical physics. We evaluate the variation of entropy produced due to each recorded path of that index during each transition as well as taking only into consideration the beginning and the end of the change between phases and verified both integral fluctuation relations. The statistical results show that these entropy variations have not been extreme entropic events; only the transition between the strong 1999–2000 La Niña to the moderate 2002–2003 El Niño is at the edge of being so. With that, the present work opens a long and winding avenue of research over the application of stochastic statistical physics to climate dynamics.