We report the first observation of Raman optical activity (ROA) by coherent anti-Stokes Raman scattering. Thanks to the more freedom of polarization configurations in coherent anti-Stokes Raman scattering than in spontaneous Raman spectroscopy, the contrast ratio of the chiral signal to the achiral background has been improved markedly. For (-)-$\beta$-pinene, it is 2 orders of magnitude better than that in the reported spontaneous ROA measurement. This is also the first measurement of ROA signal using a pulsed laser source.

Boolean networks, widely used to model gene regulation, exhibit a phase transition between regimes in which small perturbations either die out or grow exponentially. We show and numerically verify that this phase transition in the dynamics can be mapped onto a static percolation problem which predicts the long-time average Hamming distance between perturbed and unperturbed orbits.

The fluctuational propagation of solitons (magnetic fluxons) in long Josephson junctions is studied both numerically and analytically. It is demonstrated that operation in conditions where solitons are subjected to Lorentz contraction for a significant part of the junctions length leads to drastic suppression of thermal jitter at the output junction end. Specifically, for large-to-critical damping and small values of bias current, the physically obvious dependence of the jitter versus length $\sigma \sim \sqrt{L}$ is confirmed, while for small damping starting from the experimentally relevant $\alpha =0.1$ and below, strong deviation from $\sigma \sim \sqrt{L}$ is observed, up to nearly complete independence of the jitter versus length, which is supported by the obtained theory.

We report on high-resolution differential conductance experiments on nanoscale superconductor-ferromagnet tunnel junctions with ultrathin oxide tunnel barriers. We observe subgap conductance features that are symmetric with respect to bias and shift according to the Zeeman energy with an applied magnetic field. These features can be explained by resonant transport via Andreev bound states induced by spin-active scattering at the interface. From the energy and Zeeman shift of the bound states, both the magnitude and sign of the spin-dependent interfacial phase shifts between spin-up and spin-down electrons can be determined. These results contribute to the microscopic insight into the triplet proximity effect at spin-active interfaces.

The temporal and spatial properties of terahertz magnons excited at ferromagnetic fcc Co(100) and bcc Fe(110) surfaces are investigated experimentally. The magnon lifetime is found to be a few tens of femtoseconds at low wave vectors, which reduces significantly as the wave vector approaches the Brillouin zone boundary. Surprisingly, the lifetime is very similar in both systems, in spite of the fact that the excitation energy in the Co(100) film is by a factor of two larger than in the Fe(110) film. The magnon wave packets propagate only a few nanometers within their lifetime. In addition to the fact that our results describe the damping mechanism in ultrafast time scales, they may provide a way to predict the ultimate time scale of magnetic switching in nanostructures.

We propose nonlinear resonant laser manipulation, a technique that drastically enhances the number of degrees of freedom when manipulating nano-objects. Considering the high laser intensity required to trap single molecules, we calculate the radiation force exerted on a molecule in a focused laser beam by solving the density matrix equations using the nonperturbative method. The results coherently elucidate certain recently reported puzzling phenomena that contradict the conventional understanding of laser trapping. Further, we demonstrate unconventional forms of laser manipulations using “stimulated recoil force” and “subwavelength laser manipulation.”

Lamellar copolymers confined into a film of thickness $D$ by two stripe-patterned surfaces, which are rotated against each other by a twist angle $\alpha$, form lamellar domains that register and align with the respective chemical surface patterns. The two domains of thickness $x$ and $D-x$ are separated by an interface that resembles a twist grain boundary. At small twist angles $\alpha$ or strong selectivity of the surface patterns, this interface fluctuates around the middle of the film, $x\approx D/2$, while the interface is localized at one of the surfaces, $x\approx 0$ or $x\approx D$, in the opposite limit. These two morphologies are separated by an interface localization-delocalization transition (ILDT) that can be controlled by the twist angle $\alpha$. For thin films, we find a second-order ILDT while the ILDT is first-order for large $D$ values. A phenomenological interface Hamiltonian is used to relate the findings to the ILDT of symmetric mixtures, and the predictions are confirmed by molecular simulation.

Pulsar timing arrays are a prime tool to study unexplored astrophysical regimes with gravitational waves. Here, we show that the detection of gravitational radiation from individually resolvable supermassive black hole binary systems can yield direct information about the masses and spins of the black holes, provided that the gravitational-wave-induced timing fluctuations both at the pulsar and at Earth are detected. This in turn provides a map of the nonlinear dynamics of the gravitational field and a new avenue to tackle open problems in astrophysics connected to the formation and evolution of supermassive black holes. We discuss the potential, the challenges, and the limitations of these observations.

We suggest and verify experimentally the concept of functional metamaterials whose properties are remotely controlled by illuminating the metamaterial with a pattern of visible light. In such metamaterials arbitrary gradients of the effective material parameters can be achieved simply by adjusting the profile of illumination. We fabricate such light-tunable microwave metamaterials and demonstrate their unique functionalities for reflection, shaping, and focusing of electromagnetic waves.

Self-assembled Ge wires with a height of only 3 unit cells and a length of up to 2 micrometers were grown on Si(001) by means of a catalyst-free method based on molecular beam epitaxy. The wires grow horizontally along either the [100] or the [010] direction. On atomically flat surfaces, they exhibit a highly uniform, triangular cross section. A simple thermodynamic model accounts for the existence of a preferential base width for longitudinal expansion, in quantitative agreement with the experimental findings. Despite the absence of intentional doping, the first transistor-type devices made from single wires show low-resistive electrical contacts and single-hole transport at sub-Kelvin temperatures. In view of their exceptionally small and self-defined cross section, these Ge wires hold promise for the realization of hole systems with exotic properties and provide a new development route for silicon-based nanoelectronics.

We theoretically investigate the properties of a double-well bosonic Josephson junction coupled to a single trapped ion. We find that the coupling between the wells can be controlled by the internal state of the ion, which can be used for studying mesoscopic entanglement between the two systems and to measure their interaction with high precision. As a particular example we consider a single ${}^{87}\mathrm{Rb}$ atom and a small Bose-Einstein condensate controlled by a single ${}^{171}\mathrm{Yb}^{+}$ ion. We calculate interwell coupling rates reaching hundreds of Hz, while the state dependence amounts to tens of Hz for plausible values of the currently unknown $s$-wave scattering length between the atom and the ion. The analysis shows that it is possible to induce either the self-trapping or the tunneling regime, depending on the internal state of the ion. This enables the generation of large scale ion-atomic wave packet entanglement within current technology.

We study the evolution of a massive scalar field surrounding a Schwarzschild black hole and find configurations that can survive for arbitrarily long times, provided the black hole or the scalar field mass is small enough. In particular, both ultralight scalar field dark matter around supermassive black holes and axionlike scalar fields around primordial black holes can survive for cosmological times. Moreover, these results are quite generic in the sense that fairly arbitrary initial data evolve, at late times, as a combination of those long-lived configurations.

Neutron stars may harbor the true ground state of matter in the form of strange quark matter. If present, this type of matter is expected to be a color superconductor, a consequence of quark pairing with respect to the color and flavor degrees of freedom. The stellar magnetic field threading the quark core becomes a color-magnetic admixture and, in the event that superconductivity is of type II, leads to the formation of color-magnetic vortices. In this Letter, we show that the volume-averaged color-magnetic vortex tension force should naturally lead to a significant degree of nonaxisymmetry in systems such as radio pulsars. We show that gravitational radiation from such color-magnetic “mountains” in young pulsars, such as the Crab and Vela, could be observable by the future Einstein Telescope, thus, becoming a probe of paired quark matter in neutron stars. The detectability threshold can be pushed up toward the sensitivity level of Advanced LIGO if we invoke an interior magnetic field about a factor ten stronger than the surface polar field.

A mode converter for electron vortex beams is described. Numerical simulations, confirmed by experiment, show that the converter transforms a vortex beam with a topological charge $m=\pm 1$ into beams closely resembling Hermite-Gaussian ${\mathrm{HG}}_{10}$ and ${\mathrm{HG}}_{01}$ modes. The converter can be used as a mode discriminator or filter for electron vortex beams. Combining the converter with a phase plate turns a plane wave into modes with topological charge $m=\pm 1$. This combination serves as a generator of electron vortex beams of high brilliance.

Backward Raman compression in plasma enables pulse compression to intensities not available using material gratings. Mediating the compression with higher density plasma generally produces shorter and therefore more intense output pulses. However, very high density plasma, even if sufficiently tenuous to be transparent to the laser, also produces group velocity dispersion of the amplified pulse, deleteriously affecting the interaction. What is shown here is that, by chirping the seed pulse, the group velocity dispersion may in fact be used advantageously, achieving the maximum intensities over the shortest distances while minimizing unwanted effects.

Unconventional quantum criticality in heavy-fermion systems has been extensively analyzed in terms of a critical destruction of the Kondo effect. Motivated by a recent demonstration of quantum criticality in a mixed-valent heavy-fermion system, $\beta \mathrm{\text{−}}{\mathrm{YbAlB}}_4$, we study a particle-hole-asymmetric Anderson impurity model with a pseudogapped density of states. We demonstrate Kondo destruction at a mixed-valent quantum critical point, where a collapsing Kondo energy scale is accompanied by a singular charge-fluctuation spectrum. Both spin and charge responses scale with energy over temperature ($\omega /T$) and magnetic field over temperature ($H/T$). Implications for unconventional quantum criticality in mixed-valence heavy fermions are discussed.

The Kondo effect caused by the adsorption of iron phthalocyanine (FePc) on Au(111) was investigated by the combination of density functional theory and a numerical renormalization group calculation with scanning tunneling microscopy. We found that a novel Kondo effect is realized for a single FePc molecule on Au(111) by tuning the symmetry of the ligand field through the local coordination to the substrate. For FePc in the on top configuration where fourfold symmetry around the ${\mathrm{Fe}}^{2+}$ ion is held, the orbital degrees of freedom survive, resulting in the spin+orbital SU(4) Kondo effect. In contrast, the reduced symmetry in the bridge configuration freezes the orbital degrees of freedom, leading to the spin SU(2) Kondo effect. These results provide a novel example to manipulate the many-body phenomena by tuning the local symmetry.

We report on laser-assisted attosecond photoemission from single-crystalline magnesium. In strong contrast to the previously investigated transition metal tungsten, photoelectron wave packets originating from the localized core level and delocalized valence-band states are launched simultaneously from the solid within the experimental uncertainty of 20 as. This phenomenon is shown to be compatible with a heuristic model based on free-particle-like propagation of the electron wave packets generated inside the crystal by the attosecond excitation pulse and their subsequent interaction with the assisting laser field at the metal-vacuum interface.

One of the many bizarre features of entanglement is that Alice, by sending a qubit to Bob in a separable state, can generate some entanglement between herself and Bob. This protocol is stripped down to the bare essentials to better elucidate the key properties of the initial resource state that enable this entanglement distribution. The necessary and sufficient conditions under which the correlations of a Bell-diagonal state serve as a useful resource are proven, giving upper and lower bounds on the entanglement that can be distributed when those conditions are met.

We report tests of local position invariance based on measurements of the ratio of the ground state hyperfine frequencies of ${}^{133}\mathrm{Cs}$ and ${}^{87}\mathrm{Rb}$ in laser-cooled atomic fountain clocks. Measurements extending over 14 years set a stringent limit to a possible variation with time of this ratio: $d\ln ({\nu }_{\mathrm{Rb}}/{\nu }_{\mathrm{Cs}})/dt=(-1.39\pm 0.91)\times {10}^{-16}{\mathrm{yr}}^{-1}$. This improves by a factor of 7.7 over our previous report [H. Marion et al., Phys. Rev. Lett. 90, 150801 (2003)]. Our measurements also set the first limit to a fractional variation of the Rb/Cs frequency ratio with gravitational potential at the level of $c^{2}d\ln ({\nu }_{\mathrm{Rb}}/{\nu }_{\mathrm{Cs}})/dU=(0.11\pm 1.04)\times {10}^{-6}$, providing a new stringent differential redshift test. The above limits equivalently apply to the fractional variation of the quantity ${\alpha }^{-0.49}(g_{\mathrm{Rb}}/g_{\mathrm{Cs}})$, which involves the fine-structure constant $\alpha$ and the ratio of the nuclear $g$-factors of the two alkalis. The link with variations of the light quark mass is also presented together with a global analysis combining other available highly accurate clock comparisons.