We present neutron spin echo experiments that address the much debated topic of dynamic phenomena in polymer melts that are induced by interacting with a confining surface. We find an anchored surface layer that internally is highly mobile and not glassy as heavily promoted in the literature. The polymer dynamics in confinement is, rather, determined by two phases, one fully equal to the bulk polymer and another that is partly anchored at the surface. By strong topological interaction, this phase confines further chains with no direct contact to the surface. These form the often invoked interphase, where the full chain relaxation is impeded through the interaction with the anchored chains.

Most studies on susceptible-infected-susceptible epidemics in networks implicitly assume Markovian behavior: the time to infect a direct neighbor is exponentially distributed. Much effort so far has been devoted to characterize and precisely compute the epidemic threshold in susceptible-infected-susceptible Markovian epidemics on networks. Here, we report the rather dramatic effect of a nonexponential infection time (while still assuming an exponential curing time) on the epidemic threshold by considering Weibullean infection times with the same mean, but different power exponent $\alpha$. For three basic classes of graphs, the Erdős-Rényi random graph, scale-free graphs and lattices, the average steady-state fraction of infected nodes is simulated from which the epidemic threshold is deduced. For all graph classes, the epidemic threshold significantly increases with the power exponents $\alpha$. Hence, real epidemics that violate the exponential or Markovian assumption can behave seriously differently than anticipated based on Markov theory.

The main goal of quantum metrology is to obtain accurate values of physical parameters using quantum probes. In this context, we show that abstention, i.e., the possibility of getting an inconclusive answer at readout, can drastically improve the measurement precision and even lead to a change in its asymptotic behavior, from the shot-noise to the Heisenberg scaling. We focus on phase estimation and quantify the required amount of abstention for a given precision. We also develop analytical tools to obtain the asymptotic behavior of the precision and required rate of abstention for arbitrary pure states.

We investigate the properties of a strongly interacting superfluid gas of ${}^6\mathrm{Li}_2$ Feshbach molecules forming a thin film confined in a quasi-two-dimensional channel with a tunable random potential, creating a microscopic disorder. We measure the atomic current, extract the resistance of the film in a two-terminal configuration, and identify a superfluid state at low disorder strength, which evolves into a normal poorly conducting state for strong disorder. The transition takes place when the chemical potential reaches the percolation threshold of the disorder. The evolution of the conduction properties contrasts with the smooth behavior of the density and compressibility across the transition, measured in situ at equilibrium. These features suggest the emergence of a glasslike phase at strong disorder.

We use a microwave field to control the quantum state of optical photons stored in a cold atomic cloud. The photons are stored in highly excited collective states (Rydberg polaritons) enabling both fast qubit rotations and control of photon-photon interactions. Through the collective read-out of these pseudospin rotations it is shown that the microwave field modifies the long-range interactions between polaritons. This technique provides a powerful interface between the microwave and optical domains, with applications in quantum simulations of spin liquids, quantum metrology and quantum networks.

We demonstrate an inverse energy cascade in a minimal model of forced 2D quantum vortex turbulence. We simulate the Gross-Pitaevskii equation for a moving superfluid subject to forcing by a stationary grid of obstacle potentials, and damping by a stationary thermal cloud. The forcing injects large amounts of vortex energy into the system at the scale of a few healing lengths. A regime of forcing and damping is identified where vortex energy is efficiently transported to large length scales via an inverse energy cascade associated with the growth of clusters of same-circulation vortices, a Kolmogorov scaling law in the kinetic energy spectrum over a substantial inertial range, and spectral condensation of kinetic energy at the scale of the system size. Our results provide clear evidence that the inverse energy cascade phenomenon, previously observed in a diverse range of classical systems, can also occur in quantum fluids.

Lithium wall conditioning has lowered hydrogenic recycling and dramatically improved plasma performance in many magnetic-fusion devices. In this Letter, we report quantum-classical atomistic simulations and laboratory experiments that elucidate the roles of lithium and oxygen in the uptake of hydrogen in amorphous carbon. Surprisingly, we show that lithium creates a high oxygen concentration on a carbon surface when bombarded by deuterium. Furthermore, surface oxygen, rather than lithium, plays the key role in trapping hydrogen.

In the supramolecular chemistry field, intuitive concepts such as molecular complementarity and molecular recognition are used to explain the mechanism of lock-key associations. However, these concepts lack a precise definition, and consequently this mechanism is not well defined and understood. Here we address the physical basis of this mechanism, based on formal statistical mechanics, through Monte Carlo simulation and compare our results with recent experimental data for charged or uncharged lock-key colloids. We find that, given the size range of the molecules involved in these associations, the entropy contribution, driven by the solvent, rules the interaction, over that of the enthalpy. A universal behavior for the uncharged lock-key association is found. Based on our results, we propose a supramolecular chemistry definition.

We demonstrate a superconducting resonator with variable coupling to a measurement transmission line. The resonator coupling can be adjusted through zero to a photon emission rate 1000 times the intrinsic resonator decay rate. We demonstrate the catch and release of photons in the resonator, as well as control of nonclassical Fock states. We also demonstrate the dynamical control of the release waveform of photons from the resonator, a key functionality that will enable high-fidelity quantum state transfer between distant resonators or qubits.

We argue that the entanglement entropy for a very small subsystem obeys a property which is analogous to the first law of thermodynamics when we excite the system. In relativistic setups, its effective temperature is proportional to the inverse of the subsystem size. This provides a universal relationship between the energy and the amount of quantum information. We derive the results using holography and confirm them in two-dimensional field theories. We will also comment on an example with negative specific heat and suggest a connection between the second law of thermodynamics and the strong subadditivity of entanglement entropy.

A measurement of the $\alpha \mathrm{\text{−}}\beta \mathrm{\text{−}}\overline{\nu }$ angular correlation in the Gamow-Teller decay ${}^8\mathrm{Li}\to {}^8\mathrm{Be}^{*}+\overline{\nu }+\beta$, ${}^8\mathrm{Be}^{*}\to \alpha +\alpha$ has been performed using ions confined in a linear Paul trap surrounded by silicon detectors. The energy difference spectrum of the $\alpha$ particles emitted along and opposite the direction of the $\beta$ particle is consistent with the standard model prediction and places a limit of 3.1% (95.5% confidence level) on any tensor contribution to the decay. From this result, the amplitude of any tensor component $C_T$ relative to that of the dominant axial-vector component $C_A$ of the electroweak interaction is limited to $|C_T/C_A|<0.18$ (95.5% confidence level). This experimental approach is facilitated by several favorable features of the ${}^8\mathrm{Li}$ $\beta$ decay and has different systematic effects than the previous $\beta \mathrm{\text{−}}\overline{\nu }$ correlation results for a pure Gamow-Teller transition obtained from studying ${}^6\mathrm{He}$ $\beta$ decay.

We show that a 450 fs nonresonant, moderately intense, linearly polarized laser pulse can induce field-free molecular axis alignment of methyliodide (${\mathrm{CH}}_3\mathrm{I}$) molecules dissolved in a helium nanodroplet. Time-resolved measurements reveal rotational dynamics much slower than that of isolated molecules and absence of the sharp transient alignment recurrences characteristic of gas phase molecules. Our results presage a range of new opportunities for exploring both molecular dynamics in a dissipative environment and the properties of He nanodroplets.

Do parametrically driven systems distinguish periodic excitations that are time mirrors of each other? Faraday waves in a Newtonian fluid are studied under excitation with superimposed harmonic wave forms. We demonstrate that the threshold parameters for the stability of the ground state are insensitive to a time inversion of the driving function. This is a peculiarity of some dynamic systems. The Faraday system shares this property with standard electroconvection in nematic liquid crystals [J. Heuer et al., Phys. Rev. E 78, 036218 (2008)]. In general, time inversion of the excitation affects the asymptotic stability of a parametrically driven system, even when it is described by linear ordinary differential equations. Obviously, the observed symmetry has to be attributed to the particular structure of the underlying differential equation system. The pattern selection of the Faraday waves above threshold, on the other hand, discriminates between time-mirrored excitation functions.

With the advent of coherent x rays provided by the x-ray free-electron laser (FEL), strong interest has been kindled in sophisticated diffraction imaging techniques. In this Letter, we exploit such techniques for the diagnosis of the density distribution of the intense electron beams typically utilized in an x-ray FEL itself. We have implemented this method by analyzing the far-field coherent transition radiation emitted by an inverse-FEL microbunched electron beam. This analysis utilizes an oversampling phase retrieval method on the transition radiation angular spectrum to reconstruct the transverse spatial distribution of the electron beam. This application of diffraction imaging represents a significant advance in electron beam physics, having critical applications to the diagnosis of high-brightness beams, as well as the collective microbunching instabilities afflicting these systems.

We revisit the normal-state electronic structure of ${\mathrm{Sr}}_2{\mathrm{RuO}}_4$ by angle-resolved photoemission spectroscopy with improved data quality, as well as ab initio band structure calculations in the local-density approximation with the inclusion of spin-orbit coupling. We find that the current model of a single surface layer $(\sqrt{2}\times \sqrt{2})R45°$ reconstruction does not explain all detected features. The observed depth-dependent signal degradation, together with the close quantitative agreement with the slab calculations based on the surface crystal structure as determined by low-energy electron diffraction, reveal that—at a minimum—the subsurface layer also undergoes a similar although weaker reconstruction. This model accounts for all features—a key step in understanding the electronic structure—and indicates a surface-to-bulk progression of the electronic states driven by structural instabilities. Finally, we find no evidence for other phases stemming from either topological bulk properties or, alternatively, the interplay between spin-orbit coupling and the broken symmetry of the surface.

We report on a novel nonlinear optical phenomenon, coined as ciliary white light, during laser ablation of transparent dielectrics. It is observed in 14 different transparent materials including glasses, crystals, and polymers. This phenomenon is also universal with respect to laser polarization, pulse duration, and focusing geometry. We interpret its formation in terms of the nonlinear diffraction of the laser generated white light by the ablation crater covered by nanostructures. It carries rich information on the damage profile and morphology dynamics of the ablated surface, providing a real time in situ observation of the laser ablation process.

We show exactly with an $SU(N)$ interacting model that even if the ambiguity associated with the placement of the chemical potential, $\mu$, for a $T=0$ gapped system is removed by using the unique value $\mu (T\to 0)$, Luttinger’s sum rule is violated even if the ground-state degeneracy is lifted by an infinitesimal hopping. The failure stems from the nonexistence of the Luttinger-Ward functional for a system in which the self-energy diverges. Since it is the existence of the Luttinger-Ward functional that is the basis for Luttinger’s theorem which relates the charge density to sign changes of the single-particle Green function, no such theorem exists. Experimental data on the cuprates are presented which show a systematic deviation from the Luttinger count, implying a breakdown of the electron quasiparticle picture in strongly correlated electron matter.

We consider a quantum quench in which two initially independent condensates are suddenly coupled and study the subsequent “rephasing” dynamics. For weak tunneling couplings, the time evolution of physical observables is predicted to follow universal scaling laws, connecting the short-time dynamics to the long-time nonperturbative regime. We first present a two-mode model valid in two and three dimensions and then move to one dimension, where the problem is described by a gapped sine-Gordon theory. Combining analytical and numerical methods, we compute universal time-dependent expectation values, allowing a quantitative comparison with future experiments.

We study the nonequilibrium dynamics of a coherently split one-dimensional Bose gas by measuring the full probability distribution functions of matter-wave interference. Observing the system on different length scales allows us to probe the dynamics of excitations on different energy scales, revealing two distinct length-scale-dependent regimes of relaxation. We measure the crossover length scale separating these two regimes and identify it with the prethermalized phase-correlation length of the system. Our approach enables a direct observation of the multimode dynamics characterizing one-dimensional quantum systems.

We study the robustness of quantum information stored in the degenerate ground space of a local, frustration-free Hamiltonian with commuting terms on a 2D spin lattice. On one hand, a macroscopic energy barrier separating the distinct ground states under local transformations would protect the information from thermal fluctuations. On the other hand, local topological order would shield the ground space from static perturbations. Here we demonstrate that local topological order implies a constant energy barrier, thus inhibiting thermal stability.