We experimentally investigate the channel-resolved above-threshold double ionization (ATDI) of acetylene in the multiphoton regime using an ultraviolet femtosecond laser pulse centered at 395 nm by measuring all the ejected electrons and ions in coincidence. As compared to the sequential process, diagonal lines in the electron-electron joint energy spectrum are observed for the nonsequential ATDI owing to the correlative sharing of the absorbed multiphoton energies. We demonstrate that the distinct channel-resolved sequential and nonsequential ATDI spectra can clearly reveal the photon-induced acetylene-vinylidene isomerization via proton migration on the cation or dication states.

We report the results of flow experiments in which two chambers containing solid ${}^4\mathrm{He}$ are connected by a superfluid Vycor channel. At low temperatures and pressures, mechanically squeezing the solid in one chamber produced a pressure increase in the second chamber, a measure of mass transport through our solid-superfluid-solid junction. This pressure response is very similar to the flow seen in recent experiments at the University of Massachusetts: it began around 600 mK, increased as the temperature was reduced, then decreased dramatically at a temperature, $T_d$, which depended on the ${}^3\mathrm{He}$ impurity concentration. Our experiments indicate that the flow is limited by mass transfer across the solid-liquid interface near the Vycor ends, where the ${}^3\mathrm{He}$ collects at low temperature, rather than by flow paths within the solid ${}^4\mathrm{He}$.

The electrical and optical properties of the Mott insulator ${\mathrm{Sr}}_2{\mathrm{VO}}_4$ are investigated under high pressure on a phase pure polycrystalline sample. The system undergoes a pressure-driven insulator to metal transition (IMT) with a crossover between 20 and 24 GPa. The effect of pressure on the thermally driven electronic changes resulting from spin-orbital ordering transitions is studied. A multiorbital analysis of the low frequency optical conductivity spectra suggests a bandwidth-controlled and orbital selective nature of the Mott IMT transition. Dramatic enhancement of the low energy spectral weight in the high pressure correlated metallic phase is explained in terms of the formation of a quasiparticle peak in the spectral function of the narrow and degenerate $d_{yz,zx}$ orbitals. Our results overall establish a novel electronic phase diagram of tetragonal ${\mathrm{Sr}}_2{\mathrm{VO}}_4$.

The microscopic mechanism of the metal-insulator transition is studied by orbital-resolved ${}^{51}\mathrm{V}$ NMR spectroscopy in a prototype of the quasi-one-dimensional system ${\mathrm{V}}_6{\mathrm{O}}_{13}$. We uncover that the transition involves a site-selective $d$ orbital order lifting twofold orbital degeneracy in one of the two ${\mathrm{VO}}_6$ chains. The other chain leaves paramagnetic moments on the singly occupied $d_{xy}$ orbital across the transition. The two chains respectively stabilize an orbital-assisted spin-Peierls state and an antiferromagnetic long-range order in the ground state. The site-selective Mott transition may be a source of the anomalous metal and the Mott-Peierls duality.

We have investigated temperature-dependent behaviors of electronic structure and resistivity in a mixed-valent golden phase of SmS, based on the dynamical mean-field-theory band-structure calculations. Upon cooling, the coherent Sm $4f$ bands are formed to produce the hybridization-induced pseudogap near the Fermi level, and accordingly the topology of the Fermi surface is changed to exhibit a Lifshitz-like transition. The surface states emerging in the bulk gap region are found to be not topologically protected states but just typical Rashba spin-polarized states, indicating that SmS is not a topological Kondo semimetal. From the analysis of anomalous resistivity behavior in SmS, we have identified universal energy scales, which characterize the Kondo–mixed-valent semimetallic systems.

Charge-to-spin conversion induced by the Rashba-Edelstein effect was directly observed for the first time in samples with no magnetic layer. A spin-polarized positron beam was used to probe the spin polarization of the outermost surface electrons of $\mathrm{Bi}/\mathrm{Ag}/{\mathrm{Al}}_2{\mathrm{O}}_3$ and $\mathrm{Ag}/\mathrm{Bi}/{\mathrm{Al}}_2{\mathrm{O}}_3$ when charge currents were only associated with the Ag layers. An opposite surface spin polarization was found between $\mathrm{Bi}/\mathrm{Ag}/{\mathrm{Al}}_2{\mathrm{O}}_3$ and $\mathrm{Ag}/\mathrm{Bi}/{\mathrm{Al}}_2{\mathrm{O}}_3$ samples with the application of a charge current in the same direction. The surface spin polarizations of both systems decreased exponentially with the outermost layer thickness, suggesting the occurrence of spin diffusion from the Bi/Ag interface to the outermost surfaces. This work provides a new technique to measure spin diffusion length.

Heavy metal surface alloys represent model systems to study the correlation between electron scattering, spin-orbit interaction, and atomic structure. Here, we investigate the electron scattering from the atomic steps of monolayer ${\mathrm{BiAg}}_2$ on Ag(111) using quasiparticle interference measurements and density functional theory. We find that intraband transitions between states of opposite spin projection can occur via a spin-flip backward scattering mechanism driven by the spin-orbit interaction. The spin-flip scattering amplitude depends on the chemical composition of the steps, leading to total confinement for pure Bi step edges, and considerable leakage for mixed Bi-Ag step edges. Additionally, the different localization of the occupied and unoccupied surface bands at Ag and Bi sites leads to a spatial shift of the scattering potential barrier at pure Bi step edges.

We address the enhancement of electron transport in semiconductor superlattices that occurs in combined electric and magnetic fields when cyclotron rotation becomes resonant with Bloch oscillations. We show that the phenomenon is regular in origin, contrary to the widespread belief that it arises through chaotic diffusion. The theory verified by simulations provides an accurate description of earlier numerical results and suggests new ways of controlling resonant transport.

Synaptic democracy concerns the general problem of how regions of an axon or dendrite far from the cell body (soma) of a neuron can play an effective role in neuronal function. For example, stimulated synapses far from the soma are unlikely to influence the firing of a neuron unless some sort of active dendritic processing occurs. Analogously, the motor-driven transport of newly synthesized proteins from the soma to presynaptic targets along the axon tends to favor the delivery of resources to proximal synapses. Both of these phenomena reflect fundamental limitations of transport processes based on a localized source. In this Letter, we show that a more democratic distribution of proteins along an axon can be achieved by making the transport process less efficient. This involves two components: bidirectional or “stop-and-go” motor transport (which can be modeled in terms of advection-diffusion), and reversible interactions between motor-cargo complexes and synaptic targets. Both of these features have recently been observed experimentally. Our model suggests that, just as in human societies, there needs to be a balance between “efficiency” and “equality”.

Rough or patterned surfaces infused with a lubricating liquid display many of the same useful properties as conventional gas-cushioned superhydrophobic surfaces. However, liquid-infused surfaces exhibit a new failure mode: the infused liquid film may drain due to an external shear flow, causing the surface to lose its advantageous properties. We examine shear-driven drainage of liquid-infused surfaces with the goal of understanding and thereby mitigating this failure mode. On patterned surfaces exposed to a known shear stress, we find that a finite length of the surface remains wetted indefinitely, despite the fact that no physical barriers prevent drainage. We develop an analytical model to explain our experimental results, and find that the steady-state retention results from the ability of patterned surfaces to wick wetting liquids, and is thus analogous to capillary rise. We establish the geometric surface parameters governing fluid retention and show how these parameters can describe even random substrate patterns.

We show a powerful method to compute entanglement measures based on convex roof constructions. In particular, our method is applicable to measures that, for pure states, can be written as low order polynomials of operator expectation values. We show how to compute the linear entropy of entanglement, the linear entanglement of assistance, and a bound on the dimension of the entanglement for bipartite systems. We discuss how to obtain the convex roof of the three-tangle for three-qubit states. We also show how to calculate the linear entropy of entanglement and the quantum Fisher information based on partial information or device independent information. We demonstrate the usefulness of our method by concrete examples.

We describe a dynamical phase transition occurring within a shear band at high temperature and under extremely high shear rates. With increasing temperature, dislocation deformation and grain boundary sliding are supplanted by amorphization in a highly localized nanoscale band, which allows for massive strain and fracture. The mechanism is similar to shear melting and leads to liquid metal embrittlement at high temperature. From simulation, we find that the necessary conditions are lack of dislocation slip systems, low thermal conduction, and temperature near the melting point. The first two are exhibited by bcc titanium alloys, and we show that the final one can be achieved experimentally by adding low-melting-point elements: specifically, we use insoluble rare earth metals (REMs). Under high shear, the REM becomes mixed with the titanium, lowering the melting point within the shear band and triggering the shear-melting transition. This in turn generates heat which remains localized in the shear band due to poor heat conduction. The material fractures along the shear band. We show how to utilize this transition in the creation of new titanium-based alloys with improved machinability.

It is recognized that for a certain class of periodic photonic crystals, conical dispersion can be related to a zero-refractive index. It is not obvious whether such a notion can be extended to a noncrystalline system. We show that certain photonic quasicrystalline approximants have conical dispersions at the zone center with a triply degenerate state at the Dirac frequency, which is the necessary condition to qualify as a zero-refractive-index medium. The states in the conical dispersions are extended and have a nearly constant phase. Experimental characterizations of finite-sized samples show evidence that the photonic quasicrystals do behave as a near zero-refractive-index material around the Dirac frequency.

The dissociative chemisorption of water on rigid Ni(111) is investigated using a quasiclassical trajectory method on a nine-dimensional global potential energy surface based on a faithful permutation invariant fit of $\sim 25000$ density functional theory points. This full-dimensional model not only confirms the validity of our earlier reduced-dimensional model with 6 degrees of freedom, but also allows the examination of the influence of impact sites and incident angles. It is shown that the reactivity depends on the site of impact in a complex fashion controlled by the topography of the potential energy surface rather than the barrier height alone. In addition, the reaction is promoted by momenta both parallel and perpendicular to the surface, as predicted by the recently proposed sudden vector projection model.

A study of the temperature ($T$) and density ($n_s$) dependence of conductivity $\sigma (n_s,T)$ of a highly disordered, two-dimensional (2D) electron system in Si demonstrates scaling behavior consistent with the existence of a metal-insulator transition (MIT). The same critical exponents are found when the Coulomb interaction is screened by the metallic gate and when it is unscreened or long range. The results strongly suggest the existence of a disorder-dominated 2D MIT, which is not directly affected by the range of the Coulomb interactions.

Motivated by Weyl semimetals and weakly doped semiconductors, we study transport in a weakly disordered semiconductor with a power-law quasiparticle dispersion ${\xi }_{\mathbf{k}}\propto k^{\alpha }$. We show, that in $2\alpha$ dimensions short-correlated disorder experiences logarithmic renormalization from all energies in the band. We study the case of a general dimension $d$ using a renormalization group, controlled by an $ϵ=2\alpha -d$ expansion. Above the critical dimensions, conduction exhibits a localization-delocalization phase transition or a sharp crossover (depending on the symmetries of the Hamiltonian) as a function of disorder strength. We utilize this analysis to compute the low-temperature conductivity in Weyl semimetals and weakly doped semiconductors near and below the critical disorder point.

A new bursting $m=1/n=1$ instability ($m,n$: poloidal and toroidal mode numbers) with rapid frequency chirping down has been observed for the first time in a helical plasma with intense perpendicular neutral beam injection. This is destabilized in the plasma peripheral region by resonant interaction between helically trapped energetic ions and the resistive interchange mode. A large radial electric field is induced near the edge due to enhanced radial transport of the trapped energetic ions by the mode, and leads to clear change in toroidal plasma flow, suppression of microturbulence, and triggering an improvement of bulk plasma confinement.