We report diffusion quantum Monte Carlo calculations of the interlayer binding energy of bilayer graphene. We find the binding energies of the $AA$-and $AB$-stacked structures at the equilibrium separation to be 11.5(9) and $17.7(9)\mathrm{meV}/\mathrm{atom}$, respectively. The out-of-plane zone-center optical phonon frequency predicted by our binding-energy curve is consistent with available experimental results. As well as assisting the modeling of interactions between graphene layers, our results will facilitate the development of van der Waals exchange-correlation functionals for density functional theory calculations.

Andreev reflection spectroscopy of ferromagnet-superconductor (FS) junctions is an important probe of spin polarization. We theoretically investigate spin-polarized transport in FS junctions in the presence of Rashba and Dresselhaus interfacial spin-orbit fields and show that Andreev reflection can be controlled by changing the magnetization orientation. We predict a giant in- and out-of-plane magnetoanisotropy of the junction conductance. If the ferromagnet is highly spin polarized—in the half-metal limit—the magnetoanisotropic Andreev reflection depends universally on the spin-orbit fields only. Our results show that Andreev reflection spectroscopy can be used for sensitive probing of interfacial spin-orbit fields in a FS junction.

In two dimensions strongly interacting bosons in a magnetic field can realize a bosonic integer quantum Hall state, the simplest two-dimensional example of a symmetry-protected topological phase. We propose a realistic implementation of this phase using an optical flux lattice. Through exact diagonalization calculations, we show that the system exhibits a clear bulk gap and the topological signature of the bosonic integer quantum Hall state. In particular, the calculation of the many-body Chern number leads to a quantized Hall conductance in agreement with the analytical predictions. We also study the stability of the phase with respect to some of the experimentally relevant parameters.

We study a bosonic model with correlated hopping on a honeycomb lattice, and show that its ground state is a bosonic integer quantum Hall (BIQH) phase, a prominent example of a symmetry-protected topological (SPT) phase. By using the infinite density matrix renormalization group method, we establish the existence of the BIQH phase by providing clear numerical evidence: (i) a quantized Hall conductance with $|{\sigma }_{xy}|=2$, (ii) two counterpropagating gapless edge modes. Our simple model is an example of a novel class of systems that can stabilize SPT phases protected by a continuous symmetry on lattices and opens up new possibilities for the experimental realization of these exotic phases.

We investigate the influence of itinerant carriers on the dynamics and fluctuation of local moments in Fe-based superconductors, via linear spin-wave analysis of a spin-fermion model containing both itinerant and local degrees of freedom. Surprisingly, against the common lore, instead of enhancing the $(\pi ,0)$ order, itinerant carriers with well-nested Fermi surfaces are found to induce a significant amount of spatial and temporal quantum fluctuation that leads to the observed small ordered moment. Interestingly, the underlying mechanism is shown to be an intrapocket nesting-associated long-range coupling rather than the previously believed ferromagnetic double-exchange effect. This challenges the validity of ferromagnetically compensated first-neighbor coupling reported from short-range fitting to the experimental dispersion, which turns out to result instead from the ferro-orbital order that is also found instrumental in stabilizing the magnetic order.

Anharmonic thermal effects on the electron momentum distribution of a lithium fluoride single crystal are experimentally measured through high-resolution Compton scattering and theoretically modeled with ab initio simulations, beyond the harmonic approximation to the lattice potential, explicitly accounting for thermal expansion. Directional Compton profiles are measured at two different temperatures, 10 and 300 K, with a high momentum space resolution (0.10 a.u. in full width at half maximum), using synchrotron radiation. The effect of temperature on measured directional Compton profiles is clearly revealed by oscillations extending almost up to $|p|=4\mathrm{a}.\mathrm{u}.$, which perfectly match those predicted from quantum-mechanical simulations. The wave-function-based Hartree-Fock method and three classes of the Kohn-Sham density functional theory (local-density, generalized-gradient, and hybrid approximations) are adopted. The lattice thermal expansion, as described with the quasiharmonic approach, is found to entirely account for the effect of temperature on the electron momentum density within the experimental accuracy.

Animals of all sizes form groups, as acting together can convey advantages over acting alone; thus, collective animal behavior has been identified as a promising template for designing engineered systems. However, models and observations have focused predominantly on characterizing the overall group morphology, and often focus on highly ordered groups such as bird flocks. We instead study a disorganized aggregation (an insect mating swarm), and compare its natural fluctuations with the group-level response to an external stimulus. We quantify the swarm’s frequency-dependent linear response and its spectrum of intrinsic fluctuations, and show that the ratio of these two quantities has a simple scaling with frequency. Our results provide a new way of comparing models of collective behavior with experimental data.

Dissolved ions can alter the local permittivity of water; nevertheless most theories and simulations ignore this fact. We present a novel algorithm for treating spatial and temporal variations in the permittivity and use it to measure the equivalent conductivity of a salt-free polyelectrolyte solution. Our new approach quantitatively reproduces experimental results unlike simulations with a constant permittivity that even qualitatively fail to describe the data. We can relate this success to a change in the ion distribution close to the polymer due to the buildup of a permittivity gradient.

A classical formulation of the quantum multichromophoric theory of resonance energy transfer is developed on the basis of classical electrodynamics. The theory allows for the identification of a variety of processes of different order in the interactions that contribute to the energy transfer in molecular aggregates with intracoupling in donors and acceptor chromophores. Enhanced rates in multichromophoric resonance energy transfer are shown to be well described by this theory. Specifically, in a coupling configuration between $N_A$ acceptors and $N_D$ donors, the theory correctly predicts an enhancement of the energy transfer rate dependent on the total number of donor-acceptor pairs. As an example, the theory, applied to the transfer rate in light harvesting II, gives results in excellent agreement with experiment. Finally, it is explicitly shown that as long as linear response theory holds, the classical multichromophoric theory formally coincides with the quantum formulation.

The Kochen-Specker theorem demonstrates that it is not possible to reproduce the predictions of quantum theory in terms of a hidden variable model where the hidden variables assign a value to every projector deterministically and noncontextually. A noncontextual value assignment to a projector is one that does not depend on which other projectors—the context—are measured together with it. Using a generalization of the notion of noncontextuality that applies to both measurements and preparations, we propose a scheme for deriving inequalities that test whether a given set of experimental statistics is consistent with a noncontextual model. Unlike previous inequalities inspired by the Kochen-Specker theorem, we do not assume that the value assignments are deterministic and therefore in the face of a violation of our inequality, the possibility of salvaging noncontextuality by abandoning determinism is no longer an option. Our approach is operational in the sense that it does not presume quantum theory: a violation of our inequality implies the impossibility of a noncontextual model for any operational theory that can account for the experimental observations, including any successor to quantum theory.

Searches for dark matter imprints are one of the most active areas of current research. We focus here on light fields with mass $m_B$, such as axions and axionlike candidates. Using perturbative techniques and full-blown nonlinear numerical relativity methods, we show the following. (i) Dark matter can pile up in the center of stars, leading to configurations and geometries oscillating with a frequency that is a multiple of $f=2.5\times 10^{14}(m_B{c}^2/\mathrm{eV})\mathrm{Hz}$. These configurations are stable throughout most of the parameter space, and arise out of credible mechanisms for dark-matter capture. Stars with bosonic cores may also develop in other theories with effective mass couplings, such as (massless) scalar-tensor theories. We also show that (ii) collapse of the host star to a black hole is avoided by efficient gravitational cooling mechanisms.

Low-energy spectra of $4n$ nuclei are described with high accuracy in terms of four-body correlated structures (“quartets”). The states of all $N\ge Z$ nuclei belonging to the $A=24$ isobaric chain are represented as a superposition of two-quartet states, with quartets being characterized by isospin $T$ and angular momentum $J$. These quartets are assumed to be those describing the lowest states in ${}^{20}\mathrm{Ne}$ ($T_z=0$), ${}^{20}\mathrm{F}$ ($T_z=1$), and ${}^{20}\mathrm{O}$ ($T_z=2$). We find that the spectrum of the self-conjugate nucleus ${}^{24}\mathrm{Mg}$ can be well reproduced in terms of $T=0$ quartets only and that, among these, the $J=0$ quartet plays by far the leading role in the structure of the ground state. The same conclusion is drawn in the case of the three-quartet $N=Z$ nucleus ${}^{28}\mathrm{Si}$. As an application of the quartet formalism to nuclei not confined to the $sd$ shell, we provide a description of the low-lying spectrum of the proton-rich ${}^{92}\mathrm{Pd}$. The results achieved indicate that, in $4n$ nuclei, four-body degrees of freedom are more important and more general than usually expected.

We discuss the use of inequalities of the Leggett-Garg type (LGtI) to witness quantum coherence and present the first experimental violation of this type of inequalities using a light-matter interfaced system. By separately benchmarking the Markovian character of the evolution and the translational invariance of the conditional probabilities, the observed violation of a LGtI is attributed to the quantum coherent character of the process. These results provide a general method to benchmark “quantumness” when the absence of memory effects can be independently certified and confirm the persistence of quantum coherent features within systems of increasing complexity.

Random spin-exchange collisions in warm alkali vapor cause rapid decoherence and act to equilibrate the spin state of the atoms in the vapor. In contrast, here we demonstrate experimentally and theoretically a coherent coupling of one alkali species to another species, mediated by these random collisions. We show that the minor species (potassium) inherits the magnetic properties of the dominant species (rubidium), including its lifetime ($T_1$), coherence time ($T_2$), gyromagnetic ratio, and spin-exchange relaxation-free magnetic-field threshold. We further show that this coupling can be completely controlled by varying the strength of the magnetic field. Finally, we explain these phenomena analytically by mode mixing of the two species via spin-exchange collisions.

The scaling behavior of the moments of two passive scalars that are excited by two different methods and simultaneously convected by the same isotropic steady turbulence at $R_{\lambda }=805$ and $\text{Sc}=0.72$ is studied by using direct numerical simulation with $N={4096}^3$ grid points. The passive scalar $\theta$ is excited by a random source that is Gaussian and white in time, and the passive scalar $q$ is excited by the mean uniform scalar gradient. In the inertial convective range, the $n$th-order moments of the scalar increment $\delta \theta (r)$ do not obey a simple power law, but have the local scaling exponents ${\xi }_n^{\theta }+{\beta }_n\log (r/r_{*})$ with ${\beta }_n>0$. In contrast, the local scaling exponents of $q$ have well-developed plateaus and saturate with increasing order. The power law of passive scalar moments is not trivial. The universality of passive scalars is found not in the moments, but in the normalized moments.

We present the first highly resolved measurements of the plasmon spectrum in an ultrafast heated solid. Multi-keV x-ray photons from the Linac Coherent Light Source have been focused to one micrometer diameter focal spots producing solid density aluminum plasmas with a known electron density of $n_{\mathrm{e}}=1.8\times {10}^{23}{\mathrm{cm}}^{-3}$. Detailed balance is observed through the intensity ratio of up- and down-shifted plasmons in x-ray forward scattering spectra measuring the electron temperature. The plasmon damping is treated by electron-ion collision models beyond the Born approximation to determine the electrical conductivity of warm dense aluminum.

We realize and study the ionic Hubbard model using an interacting two-component gas of fermionic atoms loaded into an optical lattice. The bipartite lattice has a honeycomb geometry with a staggered energy offset that explicitly breaks the inversion symmetry. Distinct density-ordered phases are identified using noise correlation measurements of the atomic momentum distribution. For weak interactions the geometry induces a charge density wave. For strong repulsive interactions we detect a strong suppression of doubly occupied sites, as expected for a Mott insulating state, and the externally broken inversion symmetry is not visible anymore in the density distribution. The local density distributions in different configurations are characterized by measuring the number of doubly occupied lattice sites as a function of interaction and energy offset. We further probe the excitations of the system using direction dependent modulation spectroscopy and discover a complex spectrum, which we compare with a theoretical model.

We compute the two-particle quantities relevant for superconducting correlations in the two-dimensional Hubbard model within the dynamical cluster approximation. In the normal state we identify the parameter regime in density, interaction, and second-nearest-neighbor hopping strength that maximizes the $d_{x^2-y^2}$ superconducting transition temperature. We find in all cases that the optimal transition temperature occurs at intermediate coupling strength, and is suppressed at strong and weak interaction strengths. Similarly, superconducting fluctuations are strongest at intermediate doping and suppressed towards large doping and half filling. We find a change in sign of the vertex contributions to $d_{xy}$ superconductivity from repulsive near half filling to attractive at large doping. $p$-wave superconductivity is not found at the parameters we study, and $s$-wave contributions are always repulsive. For negative second-nearest-neighbor hopping the optimal transition temperature shifts towards the electron-doped side in opposition to the van Hove singularity, which moves towards hole doping. We surmise that an increase of the local interaction of the electron-doped compounds would increase $T_c$.