The polarization of a material and its response to applied electric and magnetic fields are key solid-state properties with a long history in insulators, although a satisfactory theory required new concepts such as Berry-phase gauge fields. In metals, quantities such as static polarization and the magnetoelectric $\theta$ term cease to be well defined. In polar metals, there can be analogous dynamical current responses, which we study in a common theoretical framework. We find that current responses to dynamical strain in polar metals depend on both the first and second Chern forms, related to polarization and magnetoelectricity in insulators as well as the orbital magnetization on the Fermi surface. We provide realistic estimates that predict that the latter contribution will dominate, and we investigate the feasibility of experimental detection of this effect.

We extend covert communication to the quantum regime by showing that covert quantum communication is possible over optical channels with noise arising either from the environment or from the sender’s lab. In particular, we show that sequences of qubits can be transmitted covertly by using both a single photon and a coherent state encoding. We study the possibility of performing covert quantum key distribution (QKD) and show that positive key rates and covertness can be achieved simultaneously. Covert communication requires a secret key between the sender and receiver, which raises the problem of how this key can be regenerated covertly. We show that covert QKD consumes more secret bits than it can generate and propose instead a hybrid protocol for covert key regeneration that uses pseudorandom number generators (PRNGs) together with covert QKD to regenerate secret keys. The security of the new key is guaranteed by QKD while the security of the covert communication is at least as strong as the security of the PRNG.

We obtain a low optical inhomogeneous linewidth of 25 MHz in the stoichiometric rare-earth crystal ${\mathrm{EuCl}}_3·6{\mathrm{H}}_2\mathrm{O}$ by isotopically purifying the crystal in ${}^{35}\mathrm{Cl}$. With this linewidth, an important limit for stoichiometric rare-earth crystals is surpassed: the hyperfine structure of ${}^{153}\mathrm{Eu}$ is spectrally resolved, allowing the whole population of ${{}^{153}\mathrm{Eu}}^{3+}$ ions to be prepared in the same hyperfine state using hole-burning techniques. This material also has a very high optical density, and can have long coherence times when deuterated. This combination of properties offers new prospects for quantum information applications. We consider two of these: quantum memories and quantum many-body studies. We detail the improvements in the performance of current memory protocols possible in these high optical depth crystals, and describe how certain memory protocols, such as off-resonant Raman memories, can be implemented for the first time in a solid-state system. We explain how the strong excitation-induced interactions observed in this material resemble those seen in Rydberg systems, and describe how these interactions can lead to quantum many-body states that could be observed using standard optical spectroscopy techniques.

Bunched-beam collinear laser spectroscopy is performed on neutron deficient ${}^{52,53}\mathrm{Fe}$ prepared through in-flight separation followed by a gas stopping. This novel scheme is a major step to reach nuclides far from the stability line in laser spectroscopy. Differential mean-square charge radii $\delta ⟨r^2⟩$ of ${}^{52,53}\mathrm{Fe}$ are determined relative to stable ${}^{56}\mathrm{Fe}$ as $\delta ⟨r^2{⟩}^{56,52}=-0.034(13){\mathrm{fm}}^2$ and $\delta ⟨r^2{⟩}^{56,53}=-0.218(13){\mathrm{fm}}^2$, respectively, from the isotope shift of atomic hyperfine structures. The multiconfiguration Dirac-Fock method is used to calculate atomic factors to deduce $\delta ⟨r^2⟩$. The values of $\delta ⟨r^2⟩$ exhibit a minimum at the $N=28$ neutron shell closure. The nuclear density functional theory with Fayans and Skyrme energy density functionals is used to interpret the data. The trend of $\delta ⟨r^2⟩$ along the Fe isotopic chain results from an interplay between single-particle shell structure, pairing, and polarization effects and provides important data for understanding the intricate trend in the $\delta ⟨r^2⟩$ of closed-shell Ca isotopes.

We propose to use multiphoton interferences of photons emitted from statistically independent thermal light sources in combination with linear optical detection techniques to reconstruct, i.e., image, arbitrary source geometries in one dimension with subclassical resolution. The scheme is an extension of earlier work [S. Oppel et al., Phys. Rev. Lett. 109, 233603 (2012)], where $N$ regularly spaced sources in one dimension were imaged by use of the $N$th-order intensity correlation function. Here, we generalize the scheme to reconstruct any number of independent thermal light sources at arbitrary separations in one dimension, exploiting intensity correlation functions of order $m\ge 3$. We present experimental results confirming the imaging protocol and provide a rigorous mathematical proof for the obtained subclassical resolution.

We demonstrate that a focused beam of high-energy electrons can be used to map the vibrational modes of a material with a spatial resolution of the order of one nanometer. Our demonstration is performed on boron nitride, a polar dielectric which gives rise to both localized and delocalized electron-vibrational scattering, either of which can be selected in our off-axial experimental geometry. Our experimental results are well supported by our calculations, and should reconcile current controversy regarding the spatial resolution achievable in vibrational mapping with focused electron beams.

X-ray reflectivity (XR) and atomistic molecular dynamics (MD) simulations, carried out to determine the structure of the oil-water interface, provide new insight into the simplest liquid-liquid interface. For several oils (hexane, dodecane, and hexadecane) the XR shows very good agreement with a monotonic interface-normal electron density profile (EDP) broadened only by capillary waves. Similar agreement is also found for an EDP including a sub-Å thick electron depletion layer separating the oil and the water. The XR and MD derived depletions are much smaller than reported for the interface between solid-supported hydrophobic monolayers and water.

In unconventional superconductors, understanding the form of the pairing interaction is the primary goal. In this regard, Raman spectroscopy is a very useful tool, as it identifies the ground state and also the subleading pairing channels by probing collective modes. Here, we propose a general theory for a multiband Raman response and identify new features in the spectrum that can provide a robust test for a pairing theory. We identify multiple Bardasis-Schrieffer type collective modes and connect the weights of these modes to the subleading gap structures within a microscopic pairing theory. While our conclusions are completely general, we apply our approach to interpret the specific case of $B_{1g}$ Raman scattering in hole-doped ${\mathrm{BaFe}}_2{\mathrm{As}}_2$.

We study the effects of disorder on unconventional superconductors in the presence of correlations, and explore a novel correlated disorder paradigm dominated by strong deviations from standard Abrikosov-Gor’kov theory due to generation of local bound states and cooperative impurity behavior driven by Coulomb interactions. Specifically we explain under which circumstances magnetic disorder acts as a strong poison destroying high-$T_c$ superconductivity at the sub-1% level, and when nonmagnetic disorder, counterintuitively, hardly affects the unconventional superconducting state while concomitantly inducing an inhomogeneous full-volume magnetic phase. Recent experimental studies of Fe-based superconductors have discovered that such unusual disorder behavior seems to be indeed present in those systems.

We study adatom-covered single layers of ${\mathrm{CrSiTe}}_3$ and ${\mathrm{CrGeTe}}_3$ using first-principles calculations based on hybrid functionals. We find that the insulating ground state of a monolayer of La (Lu) deposited on single-layer ${\mathrm{CrSiTe}}_3$ (${\mathrm{CrGeTe}}_3$) carries spontaneously generated current loops around the Cr sites. These “flux states” induce antiferromagnetically ordered orbital moments on the Cr sites and are also associated with nontrivial topological properties. The calculated Chern numbers for these systems are predicted to be $\pm 1$ even in the absence of spin-orbit coupling, with sizable gaps on the order of 100 meV. The flux states and the associated topological phases result from spontaneous time-reversal symmetry breaking due to the presence of nonlocal Coulomb interactions.

We study the properties of classical vortex solutions in a non-Abelian gauge theory. A system of two adjoint Higgs fields breaks the SU(2) gauge symmetry to $Z_2$, producing ’t Hooft–Polyakov monopoles trapped on cosmic strings, termed beads; there are two charges of monopole and two degenerate string solutions. The strings break an accidental discrete $Z_2$ symmetry of the theory, explaining the degeneracy of the ground state. Further symmetries of the model, not previously appreciated, emerge when the masses of the two adjoint Higgs fields are degenerate. The breaking of the enlarged discrete symmetry gives rise to additional string solutions and splits the monopoles into four types of “semipole”: kink solutions that interpolate between the string solutions, classified by a complex gauge-invariant magnetic flux and a $Z_4$ charge. At special values of the Higgs self-couplings, the accidental symmetry broken by the string is continuous, giving rise to supercurrents on the strings. The SU(2) theory can be embedded in a wide class of grand unified theories (GUTs), including SO(10). We argue that semipoles and supercurrents are generic on GUT strings.

Cilia and flagella exhibit regular bending waves that perform mechanical work on the surrounding fluid, to propel cellular swimmers and pump fluids inside organisms. Here, we quantify a force-velocity relationship of the beating flagellum, by exposing flagellated Chlamydomonas cells to controlled microfluidic flows. A simple theory of flagellar limit-cycle oscillations, calibrated by measurements in the absence of flow, reproduces this relationship quantitatively. We derive a link between the energy efficiency of the flagellar beat and its ability to synchronize to oscillatory flows.