Femtosecond time-resolved x-ray diffraction is used to study a photoinduced phase transition between two charge density wave (CDW) states in $1T\text{−}{\mathrm{TaS}}_2$, namely the nearly commensurate (NC) and the incommensurate (I) CDW states. Structural modulations associated with the NC-CDW order are found to disappear within 400 fs. The photoinduced I-CDW phase then develops through a nucleation and growth process which ends 100 ps after laser excitation. We demonstrate that the newly formed I-CDW phase is fragmented into several nanometric domains that are growing through a coarsening process. The coarsening dynamics is found to follow the universal Lifshitz-Allen-Cahn growth law, which describes the ordering kinetics in systems exhibiting a nonconservative order parameter.

We experimentally explore the dynamical optical hysteresis of a semiconductor microcavity as a function of the sweep time. The hysteresis area exhibits a double power law decay due to the influence of fluctuations, which trigger switching between metastable states. Upon increasing the average photon number and approaching the thermodynamic limit, the double power law evolves into a single power law. This algebraic behavior characterizes a dissipative phase transition. Our findings are in good agreement with theoretical predictions for a single mode resonator influenced by quantum fluctuations, and the present experimental approach is promising for exploring critical phenomena in photonic lattices.

The photovoltaic reciprocity theory relates the electroluminescence spectrum of a solar cell under applied bias to the external photovoltaic quantum efficiency of the device as measured at short circuit conditions. Its derivation is based on detailed balance relations between local absorption and emission rates in optically isotropic media with nondegenerate quasiequilibrium carrier distributions. In many cases, the dependence of density and spatial variation of electronic and optical device states on the point of operation is modest and the reciprocity relation holds. In nanostructure-based photovoltaic devices exploiting confined modes, however, the underlying assumptions are no longer justifiable. In the case of ultrathin absorber solar cells, the modification of the electronic structure with applied bias is significant due to the large variation of the built-in field. Straightforward use of the external quantum efficiency as measured at short circuit conditions in the photovoltaic reciprocity theory thus fails to reproduce the electroluminescence spectrum at large forward bias voltage. This failure is demonstrated here by numerical simulation of both spectral quantities at normal incidence and emission for an ultrathin GaAs $p\text{−}i\text{−}n$ solar cell using an advanced quantum kinetic formalism based on nonequilibrium Green’s functions of coupled photons and charge carriers. While coinciding with the semiclassical relations under the conditions of their validity, the theory provides a consistent microscopic relationship between absorption, emission, and charge carrier transport in photovoltaic devices at arbitrary operating conditions and for any shape of optical and electronic density of states.

When a semiflexible chain is confined in a narrow cylindrical tube, the formation of a polymer hairpin is a geometrical conformation that accompanies an exponentially large local free energy and, hence, is a relatively rare event. Numerical solutions of the hairpin distribution functions for persistence-length-to-tube-radius ratios over a wide range are obtained in high precision, by using the Green’s function approach for the wormlike-chain model. The crossover region between the narrow and moderately narrow tubes is critically investigated in terms of the hairpin free energy, global persistence length, mean hairpin-tip distance from the tube axis, and hairpin-plane orientational properties. Accurate representations of the solutions by simple interpolation formulae are suggested.

Experimental measurements of the relaxation kinetics of copolymeric surfactant exchange for micellar systems unexpectedly show a peculiar logarithmic decay. Several authors use polydispersity as an explanation for this behavior. However, in coarse-grained simulations that preserve microscopic details of the surfactants, we find evidence of the same logarithmic behavior. Since we use a strictly monodisperse distribution of chain lengths such a relaxation process cannot be attributed to polydispersity, but has to be caused by an inherent physical process characteristic of this type of system. This is supported by the fact that the decay is specifically logarithmic and not a power law with an exponent inherited from the particular polydispersity distribution of the sample. We suggest that the degeneracy of the energy states of the hydrophobic block in the core, which is broken on leaving the micelle, can qualitatively explain the broad distribution of energy barriers, which gives rise to the observed nonexponential relaxation.

The $d$-dimensional long-range Ising model, defined by spin-spin interactions decaying with the distance as the power $1/r^{d+s}$, admits a second-order phase transition with continuously varying critical exponents. At $s=s_{*}$, the phase transition crosses over to the usual short-range universality class. The standard field-theoretic description of this family of models is strongly coupled at the crossover. We find a new description, which is instead weakly coupled near the crossover, and use it to compute critical exponents. The existence of two complementary UV descriptions of the same long-range fixed point provides a novel example of infrared duality.

Deep-inelastic scattering, in the laboratory and on the lattice, is most instructive for understanding how the nucleon is built from quarks and gluons. The long-term goal is to compute the associated structure functions from first principles. So far this has been limited to model calculations. In this Letter we propose a new method to compute the structure functions directly from the virtual, all-encompassing Compton amplitude, utilizing the operator product expansion. This overcomes issues of renormalization and operator mixing, which so far have hindered lattice calculations of power corrections and higher moments.

Classically, the tendency towards spontaneous synchronization is strongest if the natural frequencies of the self-oscillators are as close as possible. We show that this wisdom fails in the deep quantum regime, where the uncertainty of amplitude narrows down to the level of single quanta. Under these circumstances identical self-oscillators cannot synchronize and detuning their frequencies can actually help synchronization. The effect can be understood in a simple picture: Interaction requires an exchange of energy. In the quantum regime, the possible quanta of energy are discrete. If the extractable energy of one oscillator does not exactly match the amount the second oscillator may absorb, interaction, and thereby synchronization, is blocked. We demonstrate this effect, which we coin quantum synchronization blockade, in the minimal example of two Kerr-type self-oscillators and predict consequences for small oscillator networks, where synchronization between blocked oscillators can be mediated via a detuned oscillator. We also propose concrete implementations with superconducting circuits and trapped ions. This paves the way for investigations of new quantum synchronization phenomena in oscillator networks both theoretically and experimentally.

Design and synthesis of new carbon allotropes have always been important topics in condensed matter physics and materials science. Here we report a new carbon allotrope, formed from cold-compressed ${\mathrm{C}}_{70}$ peapods, which most likely can be identified with a fully $s{p}^3$-bonded monoclinic structure, here named $V$ carbon, predicted from our simulation. The simulated x-ray diffraction pattern, near $K$-edge spectroscopy, and phonon spectrum agree well with our experimental data. Theoretical calculations reveal that $V$ carbon has a Vickers hardness of 90 GPa and a bulk modulus $\sim 400\mathrm{GPa}$, which well explains the “ring crack” left on the diamond anvils by the transformed phase in our experiments. The $V$ carbon is thermodynamically stable over a wide pressure range up to 100 GPa, suggesting that once $V$ carbon forms, it is stable and can be recovered to ambient conditions. A transition pathway from peapod to $V$ carbon has also been suggested. These findings suggest a new strategy for creating new $s{p}^3$-hybridized carbon structures by using fullerene@nanotubes carbon precursor containing odd-numbered rings in the structures.

We study single- and multiquantum transitions of the nuclear spins of an ensemble of ionized arsenic donors in silicon and find quadrupolar effects on the coherence times, which we link to fluctuating electrical field gradients present after the application of light and bias voltage pulses. To determine the coherence times of superpositions of all orders in the 4-dimensional Hilbert space, we use a phase-cycling technique and find that, when electrical effects were allowed to decay, these times scale as expected for a fieldlike decoherence mechanism such as the interaction with surrounding ${}^{29}\mathrm{Si}$ nuclear spins.

We study the dynamics of screening in photodoped Mott insulators with long-ranged interactions using a nonequilibrium implementation of the $GW$ plus extended dynamical mean-field theory formalism. Our study demonstrates that the complex interplay of the injected carriers with bosonic degrees of freedom (charge fluctuations) can result in long-lived transient states with properties that are distinctly different from those of thermal equilibrium states. Systems with strong nonlocal interactions are found to exhibit a self-sustained population inversion of the doublons and holes. This population inversion leads to low-energy antiscreening which can be detected in time-resolved electron-energy-loss spectra.

We employ time-resolved resonant x-ray diffraction to study the melting of charge order and the associated insulator-to-metal transition in the doped manganite ${\mathrm{Pr}}_{0.5}{\mathrm{Ca}}_{0.5}{\mathrm{MnO}}_3$ after resonant excitation of a high-frequency infrared-active lattice mode. We find that the charge order reduces promptly and highly nonlinearly as function of excitation fluence. Density-functional theory calculations suggest that direct anharmonic coupling between the excited lattice mode and the electronic structure drives these dynamics, highlighting a new avenue of nonlinear phonon control.

We report a study of the quantum Hall states (QHS) of holes in mono- and bilayer ${\mathrm{WSe}}_2$. The QHS sequence transitions between predominantly even and predominantly odd filling factors as the hole density is tuned in the range $1.6–12\times 10^{12}{\mathrm{cm}}^{-2}$. Measurements in tilted magnetic fields reveal an insensitivity of the QHS to the in-plane magnetic field, evincing that the hole spin is locked perpendicular to the ${\mathrm{WSe}}_2$ plane. Furthermore, the QHS sequence is insensitive to an applied electric field. These observations imply that the QHS sequence is controlled by the Zeeman-to-cyclotron energy ratio, which remains constant as a function of perpendicular magnetic field at a fixed carrier density, but changes as a function of density due to strong electron-electron interaction.

The Zeno and anti-Zeno effects are features of measurement-driven quantum evolution where frequent measurement inhibits or accelerates the decay of a quantum state. Either type of evolution can emerge depending on the system-environment interaction and measurement method. In this experiment, we use a superconducting qubit to map out both types of Zeno effect in the presence of structured noise baths and variable measurement rates. We observe both the suppression and acceleration of qubit decay as repeated measurements are used to modulate the qubit spectrum causing the qubit to sample different portions of the bath. We compare the Zeno effects arising from dispersive energy measurements and purely dephasing “quasimeasurements,” showing energy measurements are not necessary to accelerate or suppress the decay process.

We report on the first $\gamma$-ray spectroscopy of low-lying states in neutron-rich ${}^{98,100}\mathrm{Kr}$ isotopes obtained from ${}^{99,101}\mathrm{Rb}(p,2p)$ reactions at $\sim 220\mathrm{MeV}/\mathrm{nucleon}$. A reduction of the $2_1^{+}$ state energies beyond $N=60$ demonstrates a significant increase of deformation, shifted in neutron number compared to the sharper transition observed in strontium and zirconium isotopes. State-of-the-art beyond-mean-field calculations using the Gogny D1S interaction predict level energies in good agreement with experimental results. The identification of a low-lying ($0_2^{+}$, $2_2^{+}$) state in ${}^{98}\mathrm{Kr}$ provides the first experimental evidence of a competing configuration at low energy in neutron-rich krypton isotopes consistent with the oblate-prolate shape coexistence picture suggested by theory.

We present a multiaperture analyzer setup for performing x-ray phase contrast imaging in planar and three-dimensional modalities. The method is based on strongly structuring the x-ray beam with an amplitude modulator, before it reaches the sample, and on a multiaperture analyzing element before detection. A multislice representation of the sample is used to establish a quantitative relation between projection images and the corresponding three-dimensional distributions, leading to successful tomographic reconstruction. Sample absorption, phase, and scattering are retrieved from the measurement of five intensity projections. The method is tested on custom-built phantoms with synchrotron radiation: sample absorption and phase can be reliably retrieved also in combination with strong scatterers, simultaneously attaining high sensitivity and dynamic range.

Plasma-based acceleration is being considered as the basis for building a future linear collider. Nonlinear plasma wakefields have ideal properties for accelerating and focusing electron beams. Preservation of the emittance of nano-Coulomb beams with nanometer scale matched spot sizes in these wakefields remains a critical issue due to ion motion caused by their large space charge forces. We use fully resolved quasistatic particle-in-cell simulations of electron beams in hydrogen and lithium plasmas, including when the accelerated beam has different emittances in the two transverse planes. The projected emittance initially grows and rapidly saturates with a maximum emittance growth of less than 80% in hydrogen and 20% in lithium. The use of overfocused beams is found to dramatically reduce the emittance growth. The underlying physics that leads to the lower than expected emittance growth is elucidated.