We propose a simple theory for the dynamics of model glass-forming fluids, which should be solvable using a mean-field-like approach. The theory is based on transparent physical assumptions, which can be tested in computer simulations. The theory predicts an ergodicity-breaking transition that is identical to the so-called dynamic transition predicted within the replica approach. Thus, it can provide the missing dynamic component of the random first order transition framework. In the large-dimensional limit the theory reproduces the result of a recent exact calculation of Maimbourg et al. [Phys. Rev. Lett. 116, 015902 (2016)]. Our approach provides an alternative, physically motivated derivation of this result.

We investigate the time evolution of the Kondo resonance in response to a quench by applying the time-dependent numerical renormalization group (TDNRG) approach to the Anderson impurity model in the strong correlation limit. For this purpose, we derive within the TDNRG approach a numerically tractable expression for the retarded two-time nonequilibrium Green function $G(t+t^{\prime },t)$, and its associated time-dependent spectral function, $A(\omega ,t)$, for times $t$ both before and after the quench. Quenches from both mixed valence and Kondo correlated initial states to Kondo correlated final states are considered. For both cases, we find that the Kondo resonance in the zero temperature spectral function, a preformed version of which is evident at very short times $t\to 0^{+}$, only fully develops at very long times $t\gtrsim 1/T_K$, where $T_K$ is the Kondo temperature of the final state. In contrast, the final state satellite peaks develop on a fast time scale $1/\mathrm{\Gamma }$ during the time interval $-1/\mathrm{\Gamma }\lesssim t\lesssim +1/\mathrm{\Gamma }$, where $\mathrm{\Gamma }$ is the hybridization strength. Initial and final state spectral functions are recovered in the limits $t\to -\infty$ and $t\to +\infty$, respectively. Our formulation of two-time nonequilibrium Green functions within the TDNRG approach provides a first step towards using this method as an impurity solver within nonequilibrium dynamical mean field theory.

The interplays between different quasiparticles in solids lay the foundation for a wide spectrum of intriguing quantum effects, yet how the collective plasmon excitations affect the quantum transport of electrons remains largely unexplored. Here we provide the first demonstration that when the electron-plasmon coupling is introduced, the quantum coherence of electrons in graphene is substantially enhanced with the quantum coherence length almost tripled. We further develop a microscopic model to interpret the striking observations, emphasizing the vital role of the graphene plasmons in suppressing electron-electron dephasing. The novel and transformative concept of plasmon-enhanced quantum coherence sheds new insight into interquasiparticle interactions, and further extends a new dimension to exploit nontrivial quantum phenomena and devices in solid systems.

High-temperature superconductivity is closely adjacent to a long-range antiferromagnet, which is called a parent compound. In cuprates, all parent compounds are alike and carrier doping leads to superconductivity, so a unified phase diagram can be drawn. However, the properties of parent compounds for iron-based superconductors show significant diversity and both carrier and isovalent dopings can cause superconductivity, which casts doubt on the idea that there exists a unified phase diagram for them. Here we show that the ordered moments in a variety of iron pnictides are inversely proportional to the effective Curie constants of their nematic susceptibility. This unexpected scaling behavior suggests that the magnetic ground states of iron pnictides can be achieved by tuning the strength of nematic fluctuations. Therefore, a unified phase diagram can be established where superconductivity emerges from a hypothetical parent compound with a large ordered moment but weak nematic fluctuations, which suggests that iron-based superconductors are strongly correlated electron systems.

Using computer simulations, we investigate the phase behavior of a system of particles interacting with a remarkably simple repulsive square-shoulder pair potential and report the formation of a novel (and stable) pyrochlorelike crystal phase. The lattice structure of the pyrochlorelike phase formed in our simulations possesses two inherent length scales corresponding to the inter- and intratetrahedral neighbors. We show that it can be used to fabricate a photonic crystal which displays complete photonic band gaps in both the direct and inverted dielectric structures.

Entanglement in quantum mechanics contradicts local realism and is a manifestation of quantum nonlocality. Its presence can be detected through the violation of Bell, or Clauser-Horne-Shimony-Holt (CHSH) inequalities. Paradigmatic quantum systems provide examples of both, nonentangled and entangled states. Here, we consider a minimal complexity setup consisting of six Majorana zero modes. We find that any allowed state in the degenerate Majorana space is nonlocally entangled. We show how to measure (with available techniques) the CHSH-violating correlations using either intermediate strength or weak measurement protocols.

The absorption of light to create Wannier-Mott excitons is a fundamental feature dictating the optical and photovoltaic properties of low band gap, high permittivity semiconductors. Such excitons, with an electron-hole separation an order of magnitude greater than lattice dimensions, are largely limited to these semiconductors but here we find evidence of Wannier-Mott exciton formation in solid carbon monoxide (CO) with a band gap of $>8\mathrm{eV}$ and a low electrical permittivity. This is established through the observation that a change of a few degrees K in deposition temperature can shift the electronic absorption spectra of solid CO by several hundred wave numbers, coupled with the recent discovery that deposition of CO leads to the spontaneous formation of electric fields within the film. These so-called spontelectric fields, here approaching $4\times {10}^7\mathrm{V}{\mathrm{m}}^{-1}$, are strongly temperature dependent. We find that a simple electrostatic model reproduces the observed temperature dependent spectral shifts based on the Stark effect on a hole and electron residing several nm apart, identifying the presence of Wannier-Mott excitons. The spontelectric effect in CO simultaneously explains the long-standing enigma of the sensitivity of vacuum ultraviolet spectra to the deposition temperature.

A strong nonlinear coupling between harmonic oscillators is highly desirable for quantum information processing and quantum simulation, but is difficult to achieve in many physical systems. Here, we exploit the Coulomb interaction between two trapped ions to achieve strong nonlinear coupling between normal modes of motion at the single-phonon level. We experimentally demonstrate phonon up- and down-conversion and apply this coupling to directly measure the parity and Wigner functions of the ions’ motional states. Our results represent the fully quantum operation of a degenerate parametric oscillator and hold promise for quantum computation schemes that involve continuous variables.

It is a challenging task to explain, in terms of a simple and compelling new physics scenario, the intriguing discrepancies between the standard model expectations and the data for the neutral-current observables $R_K$ and $R_{K^{*}}$, as well as the charged-current observables $R(D)$ and $R(D^{*})$. We show that this can be achieved in an effective theory with only two unknown parameters. In addition, this class of models predicts some interesting signatures in the context of both $B$ decays as well as high-energy collisions.

Using two-dimensional hybrid-kinetic simulations, we explore the nonlinear “interruption” of standing and traveling shear-Alfvén waves in collisionless plasmas. Interruption involves a self-generated pressure anisotropy removing the restoring force of a linearly polarized Alfvénic perturbation, and occurs for wave amplitudes $\delta B_{\perp }/B_0\gtrsim {\beta }^{-1/2}$ (where $\beta$ is the ratio of thermal to magnetic pressure). We use highly elongated domains to obtain maximal scale separation between the wave and the ion gyroscale. For standing waves above the amplitude limit, we find that the large-scale magnetic field of the wave decays rapidly. The dynamics are strongly affected by the excitation of oblique firehose modes, which transition into long-lived parallel fluctuations at the ion gyroscale and cause significant particle scattering. Traveling waves are damped more slowly, but are also influenced by small-scale parallel fluctuations created by the decay of firehose modes. Our results demonstrate that collisionless plasmas cannot support linearly polarized Alfvén waves above $\delta B_{\perp }/B_0\sim {\beta }^{-1/2}$. They also provide a vivid illustration of two key aspects of low-collisionality plasma dynamics: (i) the importance of velocity-space instabilities in regulating plasma dynamics at high $\beta$, and (ii) how nonlinear collisionless processes can transfer mechanical energy directly from the largest scales into thermal energy and microscale fluctuations, without the need for a scale-by-scale turbulent cascade.

We report a new phase called clinohexagonal prism (CHP) that accounts for all the ground states of dipolar hard spheres prepared at any density. This phase merely consists of an oblique prismatic lattice with a hexagonal base. Our calculations show that at intermediate densities, a special close packed body-centered orthorhombic phase coincides with the CHP phase in the ground state for a wide density window. In the high packing regime, i.e., in the vicinity of the density of the hexagonal close packed phase, it is a limiting case of the CHP phase with vanishing obliquity that emerges. These findings provide a unified and clarified view of the solid-solid transitions occurring at zero temperature in dipolar systems and should be relevant in other related molecular or soft matter systems governed by anisotropic (and possibly isotropic) soft potentials.

Polarized neutron scattering has been used to obtain the magnetic moment at specific crystallographic sites of the austenitic and martensitic phases of two nonstoichiometric Ni-Mn-Ga single crystals with close composition. These alloys have been chosen because they exhibit different structures in the paramagnetic state and inverse positions of the respective martensitic transformation and Curie temperature. The diffraction analysis revealed a remarkable result: Despite the similar alloy composition, the magnetic moments of Mn are quite different for the two alloys at the same crystallographic position. Furthermore, such a difference enabled us to assess that the exchange coupling between Mn atoms switches from ferro- to antiferromagnetic at a distance between 2.92 and 3.32 Å in the martensite. These results are of great importance to guide first principles calculations that, up to now, have not been contrasted with experiments at the atomic level.

We study classical two-dimensional frustrated Heisenberg models with generically incommensurate ground states. A new theory for the lattice-nematic “order by disorder” transition is developed based on the self-consistent determination of the effective exchange coupling bonds. In our approach, fluctuations of the constraint field imposing conservation of the local magnetic moment drive nematicity at low temperatures. The critical temperature is found to be highly sensitive to the peak helimagnetic wave vector, and vanishes continuously when approaching rotation symmetric Lifshitz points. Transitions between symmetry distinct nematic orders may occur by tuning the exchange parameters, leading to lines of bicritical points.

We introduce a matrix-product state based method to efficiently obtain dynamical response functions for two-dimensional microscopic Hamiltonians. We apply this method to different phases of the Kitaev-Heisenberg model and identify characteristic dynamical features. In the ordered phases proximate to the spin liquid, we find significant broad high-energy features beyond spin-wave theory, which resemble those of the Kitaev model. This establishes the concept of a proximate spin liquid, which was recently invoked in the context of inelastic neutron scattering experiments on $\alpha \text{−}{\mathrm{RuCl}}_3$. Our results provide an example of a natural path for proximate spin liquid features to arise at high energies above a conventionally ordered state, as the diffuse remnants of spin-wave bands intersect to yield a broad peak at the Brillouin zone center.

We measure x-ray magnetic circular dichroism (XMCD) spectra at the Pu $M_{4,5}$ absorption edges from a newly prepared high-quality single crystal of the heavy-fermion superconductor ${}^{242}\mathrm{Pu}{\mathrm{CoGa}}_5$, exhibiting a critical temperature $T_c=18.7\mathrm{K}$. The experiment probes the vortex phase below $T_c$ and shows that an external magnetic field induces a Pu $5f$ magnetic moment at 2 K equal to the temperature-independent moment measured in the normal phase up to 300 K by a superconducting quantum interference device. This observation is in agreement with theoretical models claiming that the Pu atoms in ${\mathrm{PuCoGa}}_5$ have a nonmagnetic singlet ground state resulting from the hybridization of the conduction electrons with the intermediate-valence $5f$ electronic shell. Unexpectedly, XMCD spectra show that the orbital component of the $5f$ magnetic moment increases significantly between 30 and 2 K; the antiparallel spin component increases as well, leaving the total moment practically constant. We suggest that this indicates a low-temperature breakdown of the complete Kondo-like screening of the local $5f$ moment.

We study the statistics, in stationary conditions, of the work $W_{\tau }$ done by the active force in different systems of self-propelled particles in a time $\tau$. We show the existence of a critical value $W_{\tau }^{†}$ such that fluctuations with $W_{\tau }>W_{\tau }^{†}$ correspond to configurations where interaction between particles plays a minor role whereas those with $W_{\tau }<W_{\tau }^{†}$ represent states with single particles dragged by clusters. This twofold behavior is fully mirrored by the probability distribution $P(W_{\tau })$ of the work, which does not obey the large-deviation principle for $W_{\tau }<W_{\tau }^{†}$. This pattern of behavior can be interpreted as due to a phase transition occurring at the level of fluctuating quantities and an order parameter is correspondingly identified.

We use extremely bright and ultrashort pulses from an x-ray free-electron laser (XFEL) to measure correlations in x rays scattered from individual bioparticles. This allows us to go beyond the traditional crystallography and single-particle imaging approaches for structure investigations. We employ angular correlations to recover the three-dimensional (3D) structure of nanoscale viruses from x-ray diffraction data measured at the Linac Coherent Light Source. Correlations provide us with a comprehensive structural fingerprint of a 3D virus, which we use both for model-based and ab initio structure recovery. The analyses reveal a clear indication that the structure of the viruses deviates from the expected perfect icosahedral symmetry. Our results anticipate exciting opportunities for XFEL studies of the structure and dynamics of nanoscale objects by means of angular correlations.

We study an ensemble of strongly coupled electrons under continuous microwave irradiation interacting with a dissipative environment, a problem of relevance to the creation of highly polarized nonequilibrium states in nuclear magnetic resonance. We analyze the stationary states of the dynamics, described within a Lindblad master equation framework, at the mean-field approximation level. This approach allows us to identify steady-state phase transitions between phases of high and low polarization controlled by the distribution of disordered electronic interactions. We compare the mean-field predictions to numerically exact simulations of small systems and find good agreement. Our study highlights the possibility of observing collective phenomena, such as metastable states, phase transitions, and critical behavior, in appropriately designed paramagnetic systems. These phenomena occur in a low-temperature regime which is not theoretically tractable by conventional methods, e.g., the spin-temperature approach.