We consider the growth of primordial dark matter halos seeded by three crossed initial sine waves of various amplitudes. Using a Lagrangian treatment of cosmological gravitational dynamics, we examine the convergence properties of a high-order perturbative expansion in the vicinity of shell crossing by comparing the analytical results with state-of-the-art high resolution Vlasov-Poisson simulations. Based on a quantitative exploration of parameter space, we study explicitly for the first time the convergence speed of the perturbative series and find, in agreement with intuition, that it slows down when going from quasi-one-dimensional initial conditions (one sine wave dominating) to quasitriaxial symmetry (three sine waves with same amplitude). In most cases, the system structure at collapse time is, as expected, very similar to what is obtained with simple one-dimensional dynamics, except in the quasitriaxial regime, where the phase-space sheet presents a velocity spike. In all cases, the perturbative series exhibits a generic convergence behavior as fast as an exponential of a power law of the order of the expansion, allowing one to numerically extrapolate it to infinite order. The results of such an extrapolation agree remarkably well with the simulations, even at shell crossing.

We analyze the universal radiative correction ${\mathrm{\Delta }}_R^V$ to neutron and superallowed nuclear $\beta$ decay by expressing the hadronic $\gamma W$-box contribution in terms of a dispersion relation, which we identify as an integral over the first Nachtmann moment of the $\gamma W$ interference structure function $F_3^{(0)}$. By connecting the needed input to existing data on neutrino and antineutrino scattering, we obtain an updated value of ${\mathrm{\Delta }}_R^V=0.02467(22)$, wherein the hadronic uncertainty is reduced. Assuming other standard model theoretical calculations and experimental measurements remain unchanged, we obtain an updated value of $|V_{ud}|=0.97370(14)$, raising tension with the first row Cabibbo-Kobayashi-Maskawa unitarity constraint. We comment on ways current and future experiments can provide input to our dispersive analysis.

We report a measurement of electron antineutrino oscillation from the Daya Bay Reactor Neutrino Experiment with nearly 4 million reactor ${\overline{\nu }}_e$ inverse $\beta$ decay candidates observed over 1958 days of data collection. The installation of a flash analog-to-digital converter readout system and a special calibration campaign using different source enclosures reduce uncertainties in the absolute energy calibration to less than 0.5% for visible energies larger than 2 MeV. The uncertainty in the cosmogenic ${}^9\mathrm{Li}$ and ${}^8\mathrm{He}$ background is reduced from 45% to 30% in the near detectors. A detailed investigation of the spent nuclear fuel history improves its uncertainty from 100% to 30%. Analysis of the relative ${\overline{\nu }}_e$ rates and energy spectra among detectors yields ${\sin }^{2}2{\theta }_{13}=0.0856\pm 0.0029$ and $\mathrm{\Delta }{m}_{32}^2=({2.471}_{-0.070}^{+0.068})\times {10}^{-3}{\mathrm{eV}}^2$ assuming the normal hierarchy, and $\mathrm{\Delta }{m}_{32}^2=-({2.575}_{-0.070}^{+0.068})\times {10}^{-3}{\mathrm{eV}}^2$ assuming the inverted hierarchy.

We present a state-of-the-art calculation of the isovector quark-helicity Bjorken-$x$ distribution in the proton using lattice-QCD ensembles at the physical pion mass. We compute quasidistributions at proton momenta $P_z\in \{2.2,2.6,3.0\}\mathrm{GeV}$ on the lattice and match them systematically to the physical parton distribution using the large-momentum effective theory. We reach an unprecedented precision through high statistics in simulations, large-momentum proton matrix elements, and control of excited-state contamination. The resulting distribution with combined statistical and systematic errors is in agreement with the latest phenomenological analysis of the spin-dependent experimental data, in particular, $\mathrm{\Delta }\overline{u}(x)>\mathrm{\Delta }\overline{d}(x)$.

Measurements of fragmentation functions for jets associated with an isolated photon are presented for the first time in $pp$ and Pb-Pb collisions. The analysis uses data collected with the CMS detector at the CERN LHC at a nucleon-nucleon center-of-mass energy of 5.02 TeV. Fragmentation functions are obtained for jets with $p_T^{\text{jet}}>30\mathrm{GeV}/c$ in events containing an isolated photon with $p_T^{\gamma }>60\mathrm{GeV}/c$, using charged tracks with transverse momentum $p_T^{\mathrm{trk}}>1\mathrm{GeV}/c$ in a cone around the jet axis. The association with an isolated photon constrains the initial $p_T$ and azimuthal angle of the parton whose shower produced the jet. For central Pb-Pb collisions, modifications of the jet fragmentation functions are observed when compared to those measured in $pp$ collisions, while no significant differences are found in the 50% most peripheral collisions. Jets in central Pb-Pb events show an excess (depletion) of low (high) $p_T$ particles, with a transition around $3\mathrm{GeV}/c$. This measurement shows for the first time the in-medium shower modifications of partons (quark dominated) with well-defined initial kinematics. It constitutes a new well-controlled reference for testing theoretical models of the parton passage through the quark-gluon plasma.

We suggest that low-energy electrons, released by resonant decay processes, experience substantial scattering on the electron density of excited electrons, which remain a spectator during the decay. As a result, the angular emission distribution is altered significantly. This effect is expected to be a common feature of low-energy secondary electron emission. In this Letter, we exemplify our idea by examining the spectator resonant interatomic Coulombic decay of Ne dimers. Our theoretical predictions are confirmed by a corresponding coincidence experiment.

We present the quantum master equation describing the coherent and incoherent dynamics of a rapidly rotating molecule in the presence of a thermal background gas. The master equation relates the rate of rotational alignment decay and decoherence to the microscopic scattering amplitudes, which we calculate for anisotropic van der Waals scattering. For large rotational energies, we find quantitative agreement of the resulting alignment decay rate with recent superrotor experiments.

Under a strong quantum measurement, the motion of an oscillator is disturbed by the measurement backaction, as required by the Heisenberg uncertainty principle. When a mechanical oscillator is continuously monitored via an electromagnetic cavity, as in a cavity optomechanical measurement, the backaction is manifest by the shot noise of incoming photons that becomes imprinted onto the motion of the oscillator. Following the photons leaving the cavity, the correlations appear as squeezing of quantum noise in the emitted field. Here we observe such “ponderomotive” squeezing in the microwave domain using an electromechanical device made out of a superconducting resonator and a drumhead mechanical oscillator. Under a strong measurement, the emitted field develops complex-valued quantum correlations, which in general are not completely accessible by standard homodyne measurements. We recover these hidden correlations, using a phase-sensitive measurement scheme employing two local oscillators. The utilization of hidden correlations presents a step forward in the detection of weak forces, as it allows us to fully utilize the quantum noise reduction under the conditions of strong force sensitivity.

We demonstrate nonlinear emission from molecular layers strongly coupled to extended light fields in arrays of plasmonic nanoparticles in the presence of structural imperfections. Hybrid light-matter states, known as plasmon-exciton polaritons (PEPs), are formed by the strong coupling of Frenkel excitons in molecules to surface lattice resonances. These resonances result from the radiative coupling of localized surface plasmon polaritons in silver nanoparticles enhanced by diffraction on the array. By designing arrays with different lattice constants, we show that the nonlinear emission frequency is solely determined by the relaxation of exciton polaritons through vibrational quanta in the molecules. We also observe long-range spatial coherence in the samples, which supports the explanation in terms of a nonlinear collective emission of strongly coupled PEPs. In contrast to recent observations of exciton-polariton lasing and condensation in organic systems, photonic modes play a minor role at the emission frequency in our system, and this emission has an undefined momentum because of the structural imperfections. This remarkable result reveals the rich and distinct physics of strongly coupled organic molecules to photonic cavities.

Although the conservation of momentum is a fundamental law in physics, its constraints are not fulfilled for wave propagation at material boundaries, where incident waves give rise to evanescent field distributions. While nonlinear susceptibility tensor terms can provide solutions in the optical regime, this framework cannot be applied directly to acoustic waves. Now, by considering a complete representation of wave interactions and scattering at boundaries, we are able to show a generic formalism of sum-frequency mixing for the whole scattering field including all evanescent waves. This general case was studied analytically and verified both numerically and experimentally for ultrasonic waves, showing that considering evanescent waves leads to an anomalous nonlinear interaction which enhances sum-frequency generation. This new interpretation not only provides a deeper understanding of the momentum conservation laws in acoustics but also promises translation of this new understanding into optics and photonics, to enhance nonlinear interactions.

We demonstrate a novel response of a nonlinear micromechanical resonator when operated in a region of strong, nonlinear mode coupling. The system is excited with a single drive signal and its response is characterized by periodic amplitude modulations that occur at timescales based on system parameters. The periodic amplitude modulations of the resonator are a consequence of nonlinear mode coupling and are responsible for the emergence of a “frequency-comb” regime in the spectral response. By considering a generic model for a 1∶3 internal resonance, we demonstrate that the novel behavior results from a saddle node on an invariant circle (SNIC) bifurcation. The ability to control the operating parameters of the micromechanical structures reported here makes the simple micromechanical resonator an ideal test bed to study the dynamic response of SNIC behavior demonstrated in mechanical, optical, and biological systems.

We present results for the ionic structure in hydrocarbons (polystyrene, polyethylene) that were shock compressed to pressures of up to 190 GPa, inducing rapid melting of the samples. The structure of the resulting liquid is then probed using in situ diffraction by an x-ray free electron laser beam, demonstrating the capability to obtain reliable diffraction data in a single shot, even for low-$Z$ samples without long range order. The data agree well with ab initio simulations, validating the ability of such approaches to model mixed samples in states where complex interparticle bonds remain, and showing that simpler models are not necessarily valid. While the results clearly exclude the possibility of complete carbon-hydrogen demixing at the conditions probed, they also, in contrast to previous predictions, indicate that diffraction is not always a sufficient diagnostic for this phenomenon.

The curvature dependence of the surface tension is central to the nucleation of liquids, but remains difficult to access experimentally and predict theoretically. This curvature dependence arises from the curvature-dependent molecular structure, which, for small nuclei, can deviate significantly from that of the planar liquid interface. Simulations and density functional theory have been used to predict this curvature dependence, however with contradicting results. Here, we provide the first direct measurement of the curvature-dependent surface tension in nucleating colloidal liquids. We employ critical Casimir forces to finely adjust colloidal particle interactions and induce liquid nucleation, and image individual nuclei at the particle scale to measure their curvature-dependent surface tension directly from thermally excited surface distortions. Using continuum models, we elucidate the interplay between nucleus structure, particle pair potential, and surface tension. Our results reveal a 20% lower surface tension for nuclei of critical size compared to bulk liquids, leading to 3 orders of magnitude higher nucleation rates, thus highlighting the importance of surface tension curvature corrections for accurate prediction of nucleation rates.

Transitions between topologically distinct electronic states have been predicted in different classes of materials and observed in some. A major goal is the identification of measurable properties that directly expose the topological nature of such transitions. Here, we focus on the giant Rashba material bismuth tellurium iodine which exhibits a pressure-driven phase transition between topological and trivial insulators in three dimensions. We demonstrate that this transition, which proceeds through an intermediate Weyl semimetallic state, is accompanied by a giant enhancement of the Berry curvature dipole which can be probed in transport and optoelectronic experiments. From first-principles calculations, we show that the Berry dipole—a vector along the polar axis of this material—has opposite orientations in the trivial and topological insulating phases and peaks at the insulator-to-Weyl critical points, at which the nonlinear Hall conductivity can increase by over 2 orders of magnitude.

We demonstrate strain-induced coupling between a hole spin in a quantum dot and mechanical motion of a cantilever. The optical transitions of quantum dots integrated into GaAs mechanical resonators are measured synchronously with the motion of the driven resonators. In a Voigt magnetic field, both electron and hole spin splittings are measured, showing negligible change for the electron spin but a large change for the hole spin of up to 36%. This large effect is attributed to the stronger spin orbit interaction of holes compared to electrons.

The concept of resonances and modes for the description of particle plasmons has recently received great interest, both in the context of efficient simulations as well as for an intuitive interpretation in physical terms. While resonance modes have been successfully employed for geometries whose optical response is governed by a few modes only, the resonance mode description exhibits considerable difficulties for larger nanoparticles with their richer mode spectra. We analyze the problem using a boundary element method approach together with a Mie solution for spherical particles, and identify the fixed link between the electric and magnetic components of the resonance modes as the main source for this shortcoming. We suggest a novel modal approximation scheme that allows us in principle to overcome this problem.

Motivated by recent reports of ${\mathrm{H}}_3{\mathrm{LiIr}}_2{\mathrm{O}}_6$ as a spin-orbital-entangled quantum liquid, we investigate via a combination of density functional theory and nonperturbative exact diagonalization the microscopic nature of its magnetic interactions. We find that while the interlayer $\mathrm{O}─\mathrm{H}─\mathrm{O}$ bond geometry strongly affects the local magnetic couplings, these bonds are likely to remain symmetrical due to large zero-point fluctuations of the H positions. In this case, the estimated magnetic model lies close to the classical tricritical point between ferromagnetic, zigzag, and incommensurate spiral orders, what may contribute to the lack of magnetic ordering. However, we also find that substitution of H by D (deuterium) as well as disorder-induced inhomogeneities destabilizes the $\mathrm{O}─\mathrm{H}$ or $\mathrm{D}─\mathrm{O}$ bonds, modifying strongly the local magnetic couplings. These results suggest that the magnetic response in ${\mathrm{H}}_3{\mathrm{LiIr}}_2{\mathrm{O}}_6$ is likely sensitive to both the stoichiometry and the microstructure of the samples and emphasize the importance of a careful treatment of hydrogen for similar systems.

Inspired by recent feats in exchange coupling antiferromagnets to an adjacent material, we demonstrate the possibility of employing them for inducing spin splitting in a superconductor, thereby avoiding the detrimental, parasitic effects of ferromagnets employed to this end. We derive the Gor’kov equation for the matrix Green’s function in the superconducting layer, considering a microscopic model for its disordered interface with a two-sublattice magnetic insulator. We find that an antiferromagnetic insulator with effectively uncompensated interface induces a large, disorder-resistant spin splitting in the adjacent superconductor. In addition, we find contributions to the self-energy stemming from the interfacial disorder. Within our model, these mimic impurity and spin-flip scattering, while another breaks the symmetries in particle-hole and spin spaces. The latter contribution, however, drops out in the quasiclassical approximation and thus, does not significantly affect the superconducting state.

The sensitivity of shot noise to the interplay between Kondo correlations and superconductivity is investigated in a carbon nanotube quantum dot connected to superconducting electrodes. Depending on the gate voltage, the SU(2) and SU(4) Kondo unitary regimes can be clearly identified. We observe enhancement of the shot noise via the Fano factor in the superconducting state. Its divergence at low bias voltage, which is more pronounced in the SU(4) regime than in the SU(2) one, is larger than what is expected from proliferation of multiple Andreev reflections predicted by the existing theories. Our result suggests that the Kondo effect is responsible for this strong enhancement.