- Open Access
Beta-Delayed Neutron Emission of
Phys. Rev. Lett. 136, 232504 – Published 11 June, 2026
DOI: https://doi.org/10.1103/z93q-9g6y
Abstract
Using the time-of-flight technique, we measured the beta-delayed neutron emission of . From our large-scale shell model (LSSM) calculation using the interaction [, Phys. Rev. Lett. 131, 022501 (2023)], we suggest the decay is dominated by the transformation of a neutron in the orbital, deep below the Fermi surface, into a proton in the orbital. We compare the beta-decay half-lives and neutron branching ratios of nuclei with and obtained with our LSSM with those of leading “global” models such as finite-range droplet model (FRDM). Our calculations match known half-lives and neutron branching ratios well and suggest that current leading models overestimate the yet-to-be-measured half-lives. Our model, backed by the decay data presented here, offers robust predictive power for nuclei of astrophysical interest such as -process waiting points.
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References (41)
- M. R. Mumpower, R. Surman, G. C. McLaughlin, and A. Aprahamian, The impact of individual nuclear properties on -process nucleosynthesis, Prog. Part. Nucl. Phys. 86, 86 (2016).
- M. R. Mumpower, T. M. Sprouse, J. M. Miller, K. A. Lund, J. C. Garcia, N. Vassh, G. C. McLaughlin, and R. Surman, Nuclear uncertainties associated with the nucleosynthesis in ejecta of a black hole accretion disk, Astrophys. J. 970, 173 (2024).
- K. L. Jones et al., The magic nature of explored through the single-particle states of , Nature (London) 465, 454 (2010).
- F. Nowacki, A. Obertelli, and A. Poves, The neutron-rich edge of the nuclear landscape: Experiment and theory, Prog. Part. Nucl. Phys. 120, 86 (2021).
- H. Watanabe et al., Isomers in and : Evidence for a robust shell closure at the neutron magic number 82 in exotic palladium isotopes, Phys. Rev. Lett. 111, 152501 (2013).
- V. H. Phong et al., Observation of a isomer in : Proton-neutron coupling “southeast” of , Phys. Rev. C 100, 011302 (2019).
- J. M. Allmond et al., Electromagnetic moments of radioactive and the emergence of collectivity outside of double-magic , Phys. Rev. Lett. 118, 092503 (2017).
- T. J. Gray et al., Early signal of emerging nuclear collectivity in neutron-rich , Phys. Rev. Lett. 124, 032502 (2020).
- P. Möller, M. R. Mumpower, T. Kawano, and W. D. Myers, Nuclear properties for astrophysical and radioactive-ion-beam applications (II), At. Data Nucl. Data Tables 125, 1 (2019).
- I. N. Borzov, Self-consistent approach to beta decay and delayed neutron emission, Phys. At. Nucl. 79, 910 (2017).
- G. Lorusso et al., -decay half-lives of 110 neutron-rich nuclei across the shell gap: Implications for the mechanism and universality of the astrophysical Process, Phys. Rev. Lett. 114, 192501 (2015).
- P. Möller, B. Pfeiffer, and K.-L. Kratz, New calculations of gross -decay properties for astrophysical applications: Speeding-up the classical r process, Phys. Rev. C 67, 055802 (2003).
- O. Hall et al., -delayed neutron emission of -process nuclei at the , Phys. Lett. B 816, 136266 (2021).
- V. H. Phong et al., -delayed one and two neutron emission probabilities southeast of and the odd-even systematics in -process nuclide abundances, Phys. Rev. Lett. 129, 172701 (2022).
- Z. Y. Xu et al., : A rosetta stone for decays of -process nuclei, Phys. Rev. Lett. 131, 022501 (2023).
- P. Hoff et al. (ISOLDE Collaboration), Single-Neutron States in , Phys. Rev. Lett. 77, 1020 (1996).
- M. Piersa et al. (IDS Collaboration), decay of : emission from neutron-unbound states in , Phys. Rev. C 99, 024304 (2019).
- M. Piersa-Siłkowska et al. (IDS Collaboration), First -decay spectroscopy of and new -decay branches of , Phys. Rev. C 104, 044328 (2021).
- J. Taprogge et al., proton-hole state in and the shell structure along PY-2014/04/01, Phys. Rev. Lett. 112, 132501 (2014).
- A. Jungclaus et al., First observation of rays emitted from excited states south-east of : The multiplet of , Phys. Rev. C 93, 041301 (2016).
- T. Kautzsch, W. B. Walters, M. Hannawald, K. L. Kratz, V. I. Mishin, V. N. Fedoseyev, W. Böhmer, Y. Jading, P. Van Duppen, B. Pfeiffer, A. Wöhr, P. Möller, I. Klöckl, V. Sebastian, U. Köster, M. Koizumi, J. Lettry, and H. L. Ravn (ISOLDE Collaboration), New states in heavy Cd isotopes and evidence for weakening of the shell structure, Eur. Phys. J. A 9, 201 (2000).
- P. Hoff et al., Nuclear spectroscopy at 133Sn, Hyperfine Interact. 129, 141 (2000).
- J. Heideman et al. (IDS Collaboration), Evidence of nonstatistical neutron emission following decay near doubly magic , Phys. Rev. C 108, 024311 (2023).
- V. Mishin, V. Fedoseyev, H.-J. Kluge, V. Letokhov, H. Ravn, F. Scheerer, Y. Shirakabe, S. Sundell, and O. Tengblad, Chemically selective laser ion-source for the CERN-ISOLDE on-line mass separator facility, Nucl. Instrum. Methods Phys. Res., Sect. B 73, 550 (1993).
- W. A. Peters et al., Performance of the Versatile Array of Neutron Detectors at Low Energy (VANDLE), Nucl. Instrum. Methods Phys. Res., Sect. A 836, 122 (2016).
- M. Baginova, P. Vojtyla, and P. P. Povinec, Investigation of neutron interactions with Ge detectors, Nucl. Instrum. Methods Phys. Res., Sect. A 897, 22 (2018).
- B. Fogelberg, M. Hellström, D. Jerrestam, H. Mach, J. Blomqvist, A. Kerek, L. O. Norlin, and J. P. Omtvedt, Detailed Spectroscopy of the doubly closed shell nucleus first observation of octupole collectivity, Phys. Rev. Lett. 73, 2413 (1994).
- H. Ohm, W. Rudolph, and K.-L. Kratz, Beta-delayed neutron emission following the decay of 17N, Nucl. Phys. A274, 45 (1976).
- L. Carraz, P. Hansen, A. Huck, B. Jonson, G. Klotz, A. Knipper, K. Kratz, C. Miéhé, S. Mattsson, G. Nyman, H. Ohm, A. Poskanzer, A. Poves, H. Ravn, C. Richard-Serre, A. Schröder, G. Walter, and W. Ziegert, The 49 K beta decay, Phys. Lett. B 109, 419 (1982).
- M. Wang, W. Huang, F. Kondev, G. Audi, and S. Naimi, The AME 2020 atomic mass evaluation (II). Tables, graphs and references, Chin. Phys. C 45, 030003 (2021).
- D. R. Entem and R. Machleidt, Accurate charge-dependent nucleon-nucleon potential at fourth order of chiral perturbation theory, Phys. Rev. C 68, 041001(R) (2003).
- C. Izzo et al., Mass measurements of neutron-rich indium isotopes for -process studies, Phys. Rev. C 103, 025811 (2021).
- T. Marketin, L. Huther, and G. Martínez-Pinedo, Large-scale evaluation of -decay rates of -process nuclei with the inclusion of first-forbidden transitions, Phys. Rev. C 93, 025805 (2016).
- A. Ravlić, Y. Saito, and W. Nazarewicz, Large-scale calculations of -decay rates and implications for -process nucleosynthesis, Phys. Rev. C 113, 045802 (2026).
- E. M. Ney, J. Engel, T. Li, and N. Schunck, Global description of decay with the axially deformed Skyrme finite-amplitude method: Extension to odd-mass and odd-odd nuclei, Phys. Rev. C 102, 034326 (2020).
- N. Shimizu, T. Togashi, and Y. Utsuno, GamowTeller transitions of neutron-rich nuclei by shell-model calculations, Prog. Theor. Exp. Phys. 2021, 033D01 (2021).
- Q. Zhi, E. Caurier, J. J. Cuenca-García, K. Langanke, G. Martínez-Pinedo, and K. Sieja, Shell-model half-lives including first-forbidden contributions for -process waiting-point nuclei, Phys. Rev. C 87, 025803 (2013).
- National Nuclear Data Center, Information extracted from the NuDat database, https://www.nndc.bnl.gov/nudat/.
- I. N. Borzov,Beta-decay rates, Nucl. Phys. A777, 645 (2006).
- M. Hannawald, K.-L. Kratz, B. Pfeiffer, W. B. Walters, V. N. Fedoseyev, V. I. Mishin, W. F. Mueller, H. Schatz, J. Van Roosbroeck, U. Köster, V. Sebastian, and H. L. Ravn (ISOLDE Collaboration), Selective laser ionization of very neutron-rich cadmium isotopes: Decay properties of and , Phys. Rev. C 62, 054301 (2000).
- N. Shimizu, T. Mizusaki, Y. Utsuno, and Y. Tsunoda, Thick-restart block Lanczos method for large-scale shell-model calculations, Comput. Phys. Commun. 244, 372 (2019).