Reuse & Permissions

It is not necessary to obtain permission to reuse this article or its components as it is available under the terms of the Creative Commons Attribution 4.0 International license. This license permits unrestricted use, distribution, and reproduction in any medium, provided attribution to the author(s) and the published article's title, journal citation, and DOI are maintained. Please note that some figures may have been included with permission from other third parties. It is your responsibility to obtain the proper permission from the rights holder directly for these figures.

Export citation

Export citation

Choose format for download:

Download Citation
  • Open Access

Conditional Entanglement Amplification via Non-Hermitian Superradiant Dynamics

Christoph Hotter1,2,*, Arkadiusz Kosior1, Helmut Ritsch1, and Karol Gietka1,†

  • *Contact author: christoph.hotter@nbi.ku.dk
  • †Contact author: karol.gietka@uibk.ac.at

Phys. Rev. Lett. 134, 233601 – Published 11 June, 2025

DOI: https://doi.org/10.1103/w377-f9mx

Abstract

Because of the inherently probabilistic nature of quantum mechanics, each experimental realization of a dynamical quantum system can produce distinct measurement outcomes, particularly when coupled to a dissipative environment. Although quantum trajectories that lead to exotic, highly entangled states are possible in principle, their observation is typically hindered by extremely low probabilities. In this Letter, we present a method to significantly enhance the probability of generating highly entangled states in an ensemble of atoms undergoing collective superradiant decay on timescales much shorter than the individual atomic spontaneous emission rate. By analyzing an effective non-Hermitian Hamiltonian governing the dynamics between photon emission events, we identify the conditions necessary for these rare no-click trajectories to occur with higher likelihood. Crucially, our method relies on initializing the system in a nonclassical state, whose entanglement is amplified via the non-Hermitian superradiant dynamics. This approach provides a new route to creating highly entangled macroscopic states such as atomic Schrödinger cat states, paving the way for advancements in quantum metrology and other quantum technologies.

View figure in article

Physics Subject Headings (PhySH)

Article Text

Supplemental Material

References (88)

  1. R. P. Feynman, Simulating physics with computers, Int. J. Theor. Phys. 21, 467 (1982).
  2. T. D. Ladd, F. Jelezko, R. Laflamme, Y. Nakamura, C. Monroe, and J. L. O’Brien, Quantum computers, Nature (London) 464, 45 (2010).
  3. P. Hauke, F. M. Cucchietti, L. Tagliacozzo, I. Deutsch, and M. Lewenstein, Can one trust quantum simulators?, Rep. Prog. Phys. 75, 082401 (2012).
  4. I. Georgescu, S. Ashhab, and F. Nori, Quantum simulation, Rev. Mod. Phys. 86, 153 (2014).
  5. C. H. Bennett, G. Brassard, C. Crépeau, R. Jozsa, A. Peres, and W. K. Wootters, Teleporting an unknown quantum state via dual classical and Einstein-Podolsky-Rosen channels, Phys. Rev. Lett. 70, 1895 (1993).
  6. S. Pirandola, J. Eisert, C. Weedbrook, A. Furusawa, and S. L. Braunstein, Advances in quantum teleportation, Nat. Photonics 9, 641 (2015).
  7. D. Leibfried, M. D. Barrett, T. Schaetz, J. Britton, J. Chiaverini, W. M. Itano, J. D. Jost, C. Langer, and D. J. Wineland, Toward Heisenberg-limited spectroscopy with multiparticle entangled states, Science 304, 1476 (2004).
  8. S. Colombo, E. Pedrozo-Peñafiel, A. F. Adiyatullin, Z. Li, E. Mendez, C. Shu, and V. Vuletić, Time-reversal-based quantum metrology with many-body entangled states, Nat. Phys. 18, 925 (2022).
  9. Z. Li, S. Colombo, C. Shu, G. Velez, S. Pilatowsky-Cameo, R. Schmied, S. Choi, M. Lukin, E. Pedrozo-Peñafiel, and V. Vuletić, Improving metrology with quantum scrambling, Science 380, 1381 (2023).
  10. R. W. Hamming, Error detecting and error correcting codes, Bell Syst. Tech. J. 29, 147 (1950).
  11. T. K. Moon, Error Correction Coding: Mathematical Methods and Algorithms (John Wiley & Sons, New York, 2020).
  12. A. Ourjoumtsev, H. Jeong, R. Tualle-Brouri, and P. Grangier, Generation of optical “Schrödinger cats” from photon number states, Nature (London) 448, 784 (2007).
  13. S. T. Merkel and F. K. Wilhelm, Generation and detection of NOON states in superconducting circuits, New J. Phys. 12, 093036 (2010).
  14. J.-Q. Liao, J.-F. Huang, and L. Tian, Generation of macroscopic Schrödinger-cat states in qubit-oscillator systems, Phys. Rev. A 93, 033853 (2016).
  15. T. Serikawa, J.-i. Yoshikawa, S. Takeda, H. Yonezawa, T. C. Ralph, E. H. Huntington, and A. Furusawa, Generation of a cat state in an optical sideband, Phys. Rev. Lett. 121, 143602 (2018).
  16. A. A. Bychek, D. N. Maksimov, and A. R. Kolovsky, NOON state of Bose atoms in the double-well potential via an excited-state quantum phase transition, Phys. Rev. A 97, 063624 (2018).
  17. Y.-A. Chen, X.-H. Bao, Z.-S. Yuan, S. Chen, B. Zhao, and J.-W. Pan, Heralded generation of an atomic NOON state, Phys. Rev. Lett. 104, 043601 (2010).
  18. K. Takase, J.-i. Yoshikawa, W. Asavanant, M. Endo, and A. Furusawa, Generation of optical Schrödinger cat states by generalized photon subtraction, Phys. Rev. A 103, 013710 (2021).
  19. W. Qin, A. Miranowicz, H. Jing, and F. Nori, Generating long-lived macroscopically distinct superposition states in atomic ensembles, Phys. Rev. Lett. 127, 093602 (2021).
  20. Y. Zhao, R. Zhang, W. Chen, X.-B. Wang, and J. Hu, Creation of Greenberger-Horne-Zeilinger states with thousands of atoms by entanglement amplification, npj Quantum Inf. 7, 24 (2021).
  21. M. Kitagawa and M. Ueda, Squeezed spin states, Phys. Rev. A 47, 5138 (1993).
  22. D. J. Wineland, J. J. Bollinger, W. M. Itano, and D. J. Heinzen, Squeezed atomic states and projection noise in spectroscopy, Phys. Rev. A 50, 67 (1994).
  23. J. Ma, X. Wang, C. Sun, and F. Nori, Quantum spin squeezing, Phys. Rep. 509, 89 (2011).
  24. G. Liu, Y.-N. Wang, L.-F. Yan, N.-Q. Jiang, W. Xiong, and M.-F. Wang, Spin squeezing via one- and two-axis twisting induced by a single off-resonance stimulated Raman scattering in a cavity, Phys. Rev. A 99, 043840 (2019).
  25. M. Płodzień, M. Kościelski, E. Witkowska, and A. Sinatra, Producing and storing spin-squeezed states and Greenberger-Horne-Zeilinger states in a one-dimensional optical lattice, Phys. Rev. A 102, 013328 (2020).
  26. K. Gietka, A. Usui, J. Deng, and T. Busch, Simulating the same physics with two distinct Hamiltonians, Phys. Rev. Lett. 126, 160402 (2021).
  27. M. Płodzień, M. Lewenstein, E. Witkowska, and J. Chwedeńczuk, One-axis twisting as a method of generating many-body Bell correlations, Phys. Rev. Lett. 129, 250402 (2022).
  28. T. Hernández Yanes, G. Žlabys, M. Płodzień, D. Burba, M. M. Sinkevičiené, E. Witkowska, and G. Juzeliūnas, Spin squeezing in open Heisenberg spin chains, Phys. Rev. B 108, 104301 (2023).
  29. G. Bornet, G. Emperauger, C. Chen, B. Ye, M. Block, M. Bintz, J. A. Boyd, D. Barredo, T. Comparin, F. Mezzacapo, T. Roscilde, T. Lahaye, N. Y. Yao, and A. Browaeys, Scalable spin squeezing in a dipolar Rydberg atom array, Nature (London) 621, 728 (2023).
  30. W. J. Eckner, N. Darkwah Oppong, A. Cao, A. W. Young, W. R. Milner, J. M. Robinson, J. Ye, and A. M. Kaufman, Realizing spin squeezing with Rydberg interactions in an optical clock, Nature (London) 621, 734 (2023).
  31. M. Dziurawiec, T. Hernández Yanes, M. Płodzień, M. Gajda, M. Lewenstein, and E. Witkowska, Accelerating many-body entanglement generation by dipolar interactions in the Bose-Hubbard model, Phys. Rev. A 107, 013311 (2023).
  32. A. Cao, W. J. Eckner, T. Lukin Yelin et al., Multi-qubit gates and Schrödinger cat states in an optical clock, Nature (London) 634, 315 (2024).
  33. M. Płodzień, T. Wasak, E. Witkowska, M. Lewenstein, and J. Chwedeńczuk, Generation of scalable many-body Bell correlations in spin chains with short-range two-body interactions, Phys. Rev. Res. 6, 023050 (2024).
  34. A. S. Sørensen and K. Mølmer, Entangling atoms in bad cavities, Phys. Rev. A 66, 022314 (2002).
  35. J. Borregaard, E. J. Davis, G. S. Bentsen, M. H. Schleier-Smith, and A. S. Sørensen, One- and two-axis squeezing of atomic ensembles in optical cavities, New J. Phys. 19, 093021 (2017).
  36. B. Braverman, A. Kawasaki, E. Pedrozo-Peñafiel, S. Colombo, C. Shu, Z. Li, E. Mendez, M. Yamoah, L. Salvi, D. Akamatsu, Y. Xiao, and V. Vuletić, Near-unitary spin squeezing in Yb171, Phys. Rev. Lett. 122, 223203 (2019).
  37. E. Pedrozo-Peñafiel, S. Colombo, C. Shu, A. F. Adiyatullin, Z. Li, E. Mendez, B. Braverman, A. Kawasaki, D. Akamatsu, Y. Xiao, and V. Vuletić, Entanglement on an optical atomic-clock transition, Nature (London) 588, 414 (2020).
  38. K. Mølmer and A. Sørensen, Multiparticle entanglement of hot trapped ions, Phys. Rev. Lett. 82, 1835 (1999).
  39. G. S. Agarwal, R. R. Puri, and R. P. Singh, Atomic Schrödinger cat states, Phys. Rev. A 56, 2249 (1997).
  40. D. M. Greenberger, GHZ (Greenberger-Horne-Zeilinger) theorem and GHZ states, in Compendium of Quantum Physics, edited by D. Greenberger, K. Hentschel, and F. Weinert (Springer, Berlin, Heidelberg, 2009), pp. 258–263.
  41. I. Afek, O. Ambar, and Y. Silberberg, High-NOON states by mixing quantum and classical light, Science 328, 879 (2010).
  42. C. Song, K. Xu, H. Li, Y.-R. Zhang, X. Zhang, W. Liu, Q. Guo, Z. Wang, W. Ren, J. Hao, H. Feng, H. Fan, D. Zheng, D.-W. Wang, H. Wang, and S.-Y. Zhu, Generation of multicomponent atomic Schrödinger cat states of up to 20 qubits, Science 365, 574 (2019).
  43. A. Omran, H. Levine, A. Keesling, G. Semeghini, T. T. Wang, S. Ebadi, H. Bernien, A. S. Zibrov, H. Pichler, S. Choi, J. Cui, M. Rossignolo, P. Rembold, S. Montangero, T. Calarco, M. Endres, M. Greiner, V. Vuletić, and M. D. Lukin, Generation and manipulation of Schrödinger cat states in Rydberg atom arrays, Science 365, 570 (2019).
  44. I. Pogorelov, T. Feldker, C. D. Marciniak, L. Postler, G. Jacob, O. Krieglsteiner, V. Podlesnic, M. Meth, V. Negnevitsky, M. Stadler, B. Höfer, C. Wächter, K. Lakhmanskiy, R. Blatt, P. Schindler, and T. Monz, Compact ion-trap quantum computing demonstrator, PRX Quantum 2, 020343 (2021).
  45. S. A. Moses et al., A race-track trapped-ion quantum processor, Phys. Rev. X 13, 041052 (2023).
  46. A. K. Rajagopal and R. W. Rendell, Decoherence, correlation, and entanglement in a pair of coupled quantum dissipative oscillators, Phys. Rev. A 63, 022116 (2001).
  47. D. Braun, Creation of entanglement by interaction with a common heat bath, Phys. Rev. Lett. 89, 277901 (2002).
  48. M. S. Kim, J. Lee, D. Ahn, and P. L. Knight, Entanglement induced by a single-mode heat environment, Phys. Rev. A 65, 040101(R) (2002).
  49. S. Schneider and G. J. Milburn, Entanglement in the steady state of a collective-angular-momentum (Dicke) model, Phys. Rev. A 65, 042107 (2002).
  50. M. Hor-Meyll, A. Auyuanet, C. V. S. Borges, A. Aragão, J. A. O. Huguenin, A. Z. Khoury, and L. Davidovich, Environment-induced entanglement with a single photon, Phys. Rev. A 80, 042327 (2009).
  51. Y. Hama, E. Yukawa, W. J. Munro, and K. Nemoto, Negative-temperature-state relaxation and reservoir-assisted quantum entanglement in double-spin-domain systems, Phys. Rev. A 98, 052133 (2018).
  52. J. Dias, C. W. Wächtler, K. Nemoto, and W. J. Munro, Entanglement generation between distant spins via quasilocal reservoir engineering, Phys. Rev. Res. 5, 043295 (2023).
  53. J. Dalibard, Y. Castin, and K. Mølmer, Wave-function approach to dissipative processes in quantum optics, Phys. Rev. Lett. 68, 580 (1992).
  54. R. Dum, P. Zoller, and H. Ritsch, Monte Carlo simulation of the atomic master equation for spontaneous emission, Phys. Rev. A 45, 4879 (1992).
  55. K. Mølmer, Y. Castin, and J. Dalibard, Monte Carlo wave-function method in quantum optics, J. Opt. Soc. Am. B 10, 524 (1993).
  56. H.-P. Breuer and F. Petruccione, The Theory of Open Quantum Systems (Oxford University Press, USA, 2002).
  57. A. J. Daley, Quantum trajectories and open many-body quantum systems, Adv. Phys. 63, 77 (2014).
  58. B. P. Marsh, R. M. Kroeze, S. Ganguli, S. Gopalakrishnan, J. Keeling, and B. L. Lev, Entanglement and replica symmetry breaking in a driven-dissipative quantum spin glass, Phys. Rev. X 14, 011026 (2024).
  59. R. H. Dicke, Coherence in spontaneous radiation processes, Phys. Rev. 93, 99 (1954).
  60. M. A. Norcia, M. N. Winchester, J. R. K. Cline, and J. K. Thompson, Superradiance on the millihertz linewidth strontium clock transition, Sci. Adv. 2, e1601231 (2016).
  61. M. A. Norcia, J. R. K. Cline, J. A. Muniz, J. M. Robinson, R. B. Hutson, A. Goban, G. E. Marti, J. Ye, and J. K. Thompson, Frequency measurements of superradiance from the strontium clock transition, Phys. Rev. X 8, 021036 (2018).
  62. T. Laske, H. Winter, and A. Hemmerich, Pulse delay time statistics in a superradiant laser with calcium atoms, Phys. Rev. Lett. 123, 103601 (2019).
  63. C. Hotter, L. Ostermann, and H. Ritsch, Cavity sub- and superradiance for transversely driven atomic ensembles, Phys. Rev. Res. 5, 013056 (2023).
  64. E. A. Bohr, S. L. Kristensen, C. Hotter, S. A. Schäffer, J. Robinson-Tait, J. W. Thomsen, T. Zelevinsky, H. Ritsch, and J. H. Müller, Collectively enhanced Ramsey readout by cavity sub- to superradiant transition, Nat. Commun. 15, 1084 (2024).
  65. H. Ritsch, P. Domokos, F. Brennecke, and T. Esslinger, Cold atoms in cavity-generated dynamical optical potentials, Rev. Mod. Phys. 85, 553 (2013).
  66. A. Piñeiro Orioli, J. K. Thompson, and A. M. Rey, Emergent dark states from superradiant dynamics in multilevel atoms in a cavity, Phys. Rev. X 12, 011054 (2022).
  67. B. M. Garraway and P. L. Knight, Evolution of quantum superpositions in open environments: Quantum trajectories, jumps, and localization in phase space, Phys. Rev. A 50, 2548 (1994).
  68. C. Zerba and A. Silva, Measurement phase transitions in the no-click limit as quantum phase transitions of a non-Hermitian vacuum, SciPost Phys. Core 6, 051 (2023).
  69. G. De Tomasi and I. M. Khaymovich, Stable many-body localization under random continuous measurements in the no-click limit, Phys. Rev. B 109, 174205 (2024).
  70. Y. Le Gal, X. Turkeshi, and M. Schirò, Entanglement dynamics in monitored systems and the role of quantum jumps, PRX Quantum 5, 030329 (2024).
  71. G. Di Fresco, B. Spagnolo, D. Valenti, and A. Carollo, Metrology and multipartite entanglement in measurement-induced phase transition, Quantum 8, 1326 (2024).
  72. L. K. Thomsen, S. Mancini, and H. M. Wiseman, Spin squeezing via quantum feedback, Phys. Rev. A 65, 061801(R) (2002).
  73. Z. Chen, J. G. Bohnet, S. R. Sankar, J. Dai, and J. K. Thompson, Conditional Spin squeezing of a large ensemble via the vacuum Rabi splitting, Phys. Rev. Lett. 106, 133601 (2011).
  74. J. G. Bohnet, K. C. Cox, M. A. Norcia, J. M. Weiner, Z. Chen, and J. K. Thompson, Reduced spin measurement back-action for a phase sensitivity ten times beyond the standard quantum limit, Nat. Photonics 8, 731 (2014).
  75. K. C. Cox, G. P. Greve, J. M. Weiner, and J. K. Thompson, Deterministic squeezed states with collective measurements and feedback, Phys. Rev. Lett. 116, 093602 (2016).
  76. Y. C. Liu, Z. F. Xu, G. R. Jin, and L. You, Spin squeezing: Transforming one-axis twisting into two-axis twisting, Phys. Rev. Lett. 107, 013601 (2011).
  77. D. Kajtoch and E. Witkowska, Quantum dynamics generated by the two-axis countertwisting Hamiltonian, Phys. Rev. A 92, 013623 (2015).
  78. T. Hernández Yanes, M. Płodzień, M. Mackoit Sinkevičienė, G. Žlabys, G. Juzeliūnas, and E. Witkowska, One- and two-axis squeezing via laser coupling in an atomic Fermi-Hubbard model, Phys. Rev. Lett. 129, 090403 (2022).
  79. I. D. Leroux, M. H. Schleier-Smith, and V. Vuletić, Implementation of cavity squeezing of a collective atomic spin, Phys. Rev. Lett. 104, 073602 (2010).
  80. S. C. Carrasco, M. H. Goerz, Z. Li, S. Colombo, V. Vuletić, and V. S. Malinovsky, Extreme spin squeezing via optimized one-axis twisting and rotations, Phys. Rev. Appl. 17, 064050 (2022).
  81. D. Barberena, A. Chu, J. K. Thompson, and A. M. Rey, Trade-offs between unitary and measurement induced spin squeezing in cavity QED, Phys. Rev. Res. 6, L032037 (2024).
  82. See Supplemental Material at http://link.aps.org/supplemental/10.1103/w377-f9mx for a more detailed analysis and discussion on cat state fidelity, as well as experimental considerations including imperfect measurements.
  83. K. Gietka, P. Szańkowski, T. Wasak, and J. Chwedeńczuk, Quantum-enhanced interferometry and the structure of twisted states, Phys. Rev. A 92, 043622 (2015).
  84. L. Pezzè, A. Smerzi, M. K. Oberthaler, R. Schmied, and P. Treutlein, Quantum metrology with nonclassical states of atomic ensembles, Rev. Mod. Phys. 90, 035005 (2018).
  85. H. Strobel, W. Muessel, D. Linnemann, T. Zibold, D. B. Hume, L. Pezzè, A. Smerzi, and M. K. Oberthaler, Fisher information and entanglement of non-Gaussian spin states, Science 345, 424 (2014).
  86. A state is called oversqueezed when it starts to wrap around the Bloch sphere and hence can no longer be approximated by a Gaussian state.

  87. S. Krämer, D. Plankensteiner, L. Ostermann, and H. Ritsch, quantumoptics.jl: A julia framework for simulating open quantum systems, Comput. Phys. Commun. 227, 109 (2018).
  88. C. Hotter, A. Kosior, H. Ritsch, and K. Gietka, Conditional entanglement amplification via non-Hermitian superradiant dynamics, Zenodo (2025), 10.5281/zenodo.15590880.

Outline

Information

Sign In to Your Journals Account

Filter

Filter

Article Lookup

Enter a citation