- Open Access
Nonlinear Faraday Rotation of Light Polarization in Time-Reversal-Invariant Materials
Phys. Rev. Lett. 136, 056901 – Published 6 February, 2026
DOI: https://doi.org/10.1103/grjy-22gq
Abstract
We investigate the propagation of electromagnetic waves through materials displaying a nonlinear Hall effect. The coupled Maxwell-Boltzmann equations for traveling waves can be mapped onto ordinary differential equations that resemble those for the motion of a pendulum. In the weakly nonlinear regime relevant for most experiments, we find that the polarization of light displays a Faraday-like rotation when it propagates inside a metal above its plasma frequency. In contrast to the conventional Faraday effect, however, the polarization direction swings back and forth around the direction of Berry dipole vector as the light beam traverses the material. This occurs concomitantly with an oscillation of its degree of polarization, with a characteristic frequency that increases linearly with the intensity of the traveling wave. These effects could be observed by measuring thickness-dependent Faraday rotations in materials displaying the nonlinear Hall effect.
Physics Subject Headings (PhySH)
Article Text
Supplemental Material
References (34)
- V. I. Belinicher and B. I. Sturman, Sov. Phys. Usp. 23, 199 (1980).
- V. Belinicher, E. Ivchenko, and B. Sturman, Zh. Eksp. Teor. Fiz. 83, 649 (1982).
- R. von Baltz and W. Kraut, Phys. Rev. B 23, 5590 (1981).
- C. Aversa and J. E. Sipe, Phys. Rev. B 52, 14636 (1995).
- S. M. Young and A. M. Rappe, Phys. Rev. Lett. 109, 116601 (2012).
- T. Morimoto and N. Nagaosa, Sci. Adv. 2, e1501524 (2016).
- T. Rangel, B. M. Fregoso, B. S. Mendoza, T. Morimoto, J. E. Moore, and J. B. Neaton, Phys. Rev. Lett. 119, 067402 (2017).
- A. M. Cook, B. M. Fregoso, F. De Juan, S. Coh, and J. E. Moore, Nat. Commun. 8, 14176 (2017).
- T. Morimoto, M. Nakamura, M. Kawasaki, and N. Nagaosa, Phys. Rev. Lett. 121, 267401 (2018).
- D. Kumar, C.-H. Hsu, R. Sharma, T.-R. Chang, P. Yu, J. Wang, G. Eda, G. Liang, and H. Yang, Nat. Nanotechnol. 16, 421 (2021).
- L. K. Shi, O. Matsyshyn, Justin C. Song, and I. S. Villadiego, Phys. Rev. B 107, 125151 (2023).
- Y. Onishi and L. Fu, Phys. Rev. B 110, 075122 (2024).
- T. G. Rappoport, T. A. Morgado, S. Lannebère, and M. G. Silveirinha, Phys. Rev. Lett. 130, 076901 (2023).
- P. Makushko, S. Kovalev, Y. Zabila, I. Ilyakov, A. Ponomaryov, A. Arshad, G. L. Prajapati, T. V. de Oliveira, J.-C. Deinert, P. Chekhonin et al., Natl. Electron. Rev. 7, 207 (2024).
- E. Deyo, L. Golub, E. Ivchenko, and B. Spivak, arXiv:0904.1917.
- J. E. Moore and J. Orenstein, Phys. Rev. Lett. 105, 026805 (2010).
- I. Sodemann and L. Fu, Phys. Rev. Lett. 115, 216806 (2015).
- C. Ortix, Adv. Quantum Technol. 4, 2100056 (2021).
- A. Bandyopadhyay, N. B. Joseph, and A. Narayan, Mater. Today Electron. 8, 100101 (2024).
- L. Vorob’ev, JETP Lett. 29, 441 (1979).
- V. Shalygin, A. Sofronov, L. Vorob’ev, and Farbshtein, Phys. Solid State 54, 2362 (2012).
- S. S. Tsirkin, P. A. Puente, and I. Souza, Phys. Rev. B 97, 035158 (2018).
- E. J. König, M. Dzero, A. Levchenko, and D. A. Pesin, Phys. Rev. B 99, 155404 (2019).
- C. X. Yu and J. Liu, Phys. Rev. A 90, 043834 (2014).
- K. Kang, T. Li, E. Sohn, J. Shan, and K. F. Mak, Nat. Mater. 18, 324 (2019).
- Q. Ma, S.-Y. Xu, H. Shen, D. MacNeill, V. Fatemi, T.-R. Chang, A. M. Mier Valdivia, S. Wu, Z. Du, C.-H. Hsu et al., Nature (London) 565, 337 (2019).
- T. Ma, H. Chen, K. Yananose, X. Zhou, L. Wang, R. Li, Z. Zhu, Z. Wu, Q.-H. Xu, J. Yu et al., Nat. Commun. 13, 5465 (2022).
Notice that in this geometry the magnetic field produces an out-of-plane Lorentz force along and, therefore, does not affect the dynamics.
- O. Matsyshyn and I. Sodemann, Phys. Rev. Lett. 123, 246602 (2019).
- See Supplemental Material at http://link.aps.org/supplemental/10.1103/grjy-22gq for details of the derivations for traveling and transmitted stationary waves, and for a comparison with the ordinary Faraday effect.
- D. M. Fradkin, Prog. Theor. Phys. 37, 798 (1967).
- L. Zhou, K. Xu, A. Zubair, A. D. Liao, W. Fang, F. Ouyang, Y.-H. Lee, K. Ueno, R. Saito, T. Palacios et al., J. Am. Chem. Soc. 137, 11892 (2015).
- Y. Sun, J. Zhang, Z. Ma, C. Chen, J. Han, F. Chen, X. Luo, Y. Sun, and Z. Sheng, Appl. Phys. Lett. 110, 102102 (2017).
- A. Kapitulnik, J. Xia, E. Schemm, and A. Palevski, New J. Phys. 11, 055060 (2009).