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    New experimental data on excitation functions of He3-induced nuclear reactions on Ta up to 27 MeV

    B. M. Ali1,*, Gehan Y. Mohamed1, F. Ditrói2, S. Takács2, and M. Al-Abyad1

    • 1Cyclotron Facility, Experimental Nuclear Physics Department, Nuclear Research Centre, Egyptian Atomic Energy Authority, Cairo 13759, Egypt
    • 2Institute for Nuclear Research (ATOMKI), Debrecen H4026, Hungary

    • *b.moh.ali@sci.asu.edu.eg

    Phys. Rev. C 102, 064608 – Published 9 December, 2020

    DOI: https://doi.org/10.1103/PhysRevC.102.064608

    Abstract

    Excitation functions of He3-induced nuclear reactions on Tanat were measured utilizing the MGC-20E cyclotron, stacked-foils activation technique, and high-resolution gamma-ray spectrometry. From their threshold energies up to 27 MeV, cross sections for Tanat(He3,xn)Rem182, Reg182, Re181, and Tanat(He3,αxn)TaA178, Tag180 reactions were measured. The half-life of the radionuclide Re181 was checked experimentally. The intensity of the energy line 360.7 keV, in the radionuclide Re181 decay scheme, was revised experimentally. The new experimental intensity represents about half the reported value in the different nuclear structure databases. The nuclear reaction codes TALYS-1.9 and EMPIRE-3.2.3 were used to predict the formation of these products. The isomeric cross-section ratio for the Rem,g182 was also calculated. The ratio indicates that the pre-equilibrium mechanism is dominant at energies over 19 MeV. Various combinations of the models’ parameters implemented in EMPIRE such as nuclear level density models, optical model, and pre-equilibrium parameters were used to reproduce the experimental excitation functions. For TALYS calculations, the TENDL-2019 nuclear data library based on TALYS-1.9 was used. The present data were compared to theoretical results and the available experimental data. Integral yields for the produced radioisotopes were determined.

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