Evolution of high-spin states in neutron-rich isotopes approaching the shell closure
Phys. Rev. C 114, 034313 – Published 10 September, 2026
DOI: https://doi.org/10.1103/nclr-tjv1
Abstract
Background: The nuclear structure in the region southwest of the doubly magic is important to benchmark theoretical models relevant for neutron-rich heavy element formation and for the origin of the peak in the mass abundance distribution. Although neutron-rich Pb, Tl, and Hg () isotopes are relatively well studied, experimental data for neutron-rich Au isotopes () remain largely limited due to experimental challenges.
Purpose: The purpose of this work is to investigate the evolution of the high-spin structure in neutron-rich Au isotopes near the shell closure and to characterize the underlying shell-model configurations, with a particular focus on the roles of the high- unique-parity and orbitals.
Methods: Neutron-rich isotopes were produced using multinucleon transfer reactions of at a beam energy of 7 MeV/nucleon. Prompt and delayed -ray spectroscopy of isotopically identified reaction products was performed with a unique experimental setup combining the large acceptance magnetic spectrometer, the AGATA high-purity germanium -ray tracking array, and the CATLIFE detection system.
Results: In even- isotopes, prompt -ray transitions built on the isomer have been observed for the first time. The odd- band built on the state vanishes for . In odd- isotopes, new prompt and delayed -ray transitions above the isomer were identified, confirming and extending the known level schemes. New isomeric states assigned to () have been established in and . The minima in the excitation energies of the bands as a function of built on the and isomers occur at (), showing a dip against an otherwise smooth evolution.
Conclusions: Large-scale shell-model calculations based on the Kuo-Herling hole effective interaction show an overall good agreement with experimental level schemes. However, the present calculations do not reproduce the minima in excitation energies at observed in both Au and Hg isotopes. A systematic analysis of and hole occupancies, together with spin contributions of protons and neutrons, sheds light on the role of these high- unique-parity orbitals in the generation of high-spin states. Part of the results of this work have been reported in another publication [Y. Cho et al., Phys. Lett. B 878, 140558 (2026)].