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    Evolution of high-spin states in neutron-rich Au195–202 isotopes approaching the N=126 shell closure

    Y. Cho1,2,3, Y. H. Kim3,*, A. Navin4, M. Rejmund4, A. Lemasson4, D. Ramos4, E. Clément4, C. Yuan5, M. Liu5 et al.

    P. van Isacker4, A. N. Andreyev6, J. Dudouet7, S. Choi1,2, Y. Son1,2,3, A. Mukherjee3, D. Ackermann4, G. de Angelis8, S. Bae3, R. Banik9, S. Bhattacharya10, S. Bhattacharyya10, K. Chae11, F. Didierjean12, C. Fougéres4, G. de France4, G. Fremont4, J. Goupil4, G. M. Gu11, J. Ha13, K. I. Hahn3, Y. Hirayama14, S. Jeong14, D. T. Kattikat Melcom16, C. H. Kim11, M. J. Kim11, S. H. Kim11, W. Korten15, P. Marini16,4, H. Miyatake14, M. Mukai14,17, G. Mukherjee10, T. Niwase14, T. Otsuka18, J. Park19,3, R. M. Pérez-Vidal20, F. Recchia21, K. Rezynkina22, P. Schury17, J. C. Thomas4, I. Tsekhanovich16, A. Utepov4, and Y. X. Watanabe14

    • *Contact author: yunghee.kim@ibs.re.kr

    Phys. Rev. C 114, 034313 – Published 10 September, 2026

    DOI: https://doi.org/10.1103/nclr-tjv1

    Abstract

    Background: The nuclear structure in the region southwest of the doubly magic Pb208 is important to benchmark theoretical models relevant for neutron-rich heavy element formation and for the origin of the A≈195 peak in the mass abundance distribution. Although neutron-rich Pb, Tl, and Hg (Z=80–82) isotopes are relatively well studied, experimental data for neutron-rich Au isotopes (Z=79) remain largely limited due to experimental challenges.

    Purpose: The purpose of this work is to investigate the evolution of the high-spin structure in neutron-rich Au isotopes near the N=126 shell closure and to characterize the underlying shell-model configurations, with a particular focus on the roles of the high-j unique-parity πh11/2 and νi13/2 orbitals.

    Methods: Neutron-rich Au195–202 isotopes were produced using multinucleon transfer reactions of Pt198(Xe136, Ix)Auy at a beam energy of 7 MeV/nucleon. Prompt and delayed γ-ray spectroscopy of isotopically identified reaction products was performed with a unique experimental setup combining the VAMOS++ large acceptance magnetic spectrometer, the AGATA high-purity germanium γ-ray tracking array, and the CATLIFE detection system.

    Results: In even-A Au196,198,200,202 isotopes, prompt γ-ray transitions built on the 12− isomer have been observed for the first time. The odd-J band built on the 11− state vanishes for A≥196. In odd-A Au195,197,199,201 isotopes, new prompt and delayed γ-ray transitions above the 11/2− isomer were identified, confirming and extending the known level schemes. New isomeric states assigned to (25/2+) have been established in Au199 and Au201. The minima in the excitation energies of the bands as a function of N built on the 11/2− and 12− isomers occur at Au198 (N=119), showing a dip against an otherwise smooth evolution.

    Conclusions: Large-scale shell-model calculations based on the Kuo-Herling hole effective interaction show an overall good agreement with experimental level schemes. However, the present calculations do not reproduce the minima in excitation energies at N=119 observed in both Au and Hg isotopes. A systematic analysis of πh11/2 and νi13/2 hole occupancies, together with spin contributions of protons and neutrons, sheds light on the role of these high-j unique-parity orbitals in the generation of high-spin states. Part of the results of this work have been reported in another publication [Y. Cho et al., Phys. Lett. B 878, 140558 (2026)].

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