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    High-precision direct decay energy measurements of the electron-capture decay of Tc97

    Zhuang Ge1,*, Tommi Eronen1,†, Vasile Alin Sevestrean2,3,4,‡, Marlom Ramalho1, Ovidiu Niţescu2,4, Stefan Ghinescu2,3,4, Sabin Stoica2, Jouni Suhonen1,2,§, Antoine de Roubin5,6,∥ et al.

    Dmitrii Nesterenko1, Anu Kankainen1, Pauline Ascher6, Samuel Ayet San Andres7, Olga Beliuskina1, Pierre Delahaye8, Mathieu Flayol6, Mathias Gerbaux6, Stéphane Grévy6, Marjut Hukkanen1,9, Arthur Jaries1, Ari Jokinen1, Audric Husson6, Daid Kahl10,¶, Joel Kostensalo11, Jenni Kotila12, Iain Moore1, Stylianos Nikas1, Jouni Ruotsalainen1, Marek Stryjczyk1, and Ville Virtanen1

    • *Contact author: zhuang.z.ge@jyu.fi
    • †Contact author: tommi.eronen@jyu.fi
    • ‡Contact author: sevestrean.alin@theory.nipne.ro
    • §Contact author: jouni.t.suhonen@jyu.fi
    • ∥Present address: Université de Caen Normandie, CNRS/IN2P3, LPC Caen UMR6534, F-14000 Caen, France.
    • Present address: Facility for Rare Isotope Beams, Michigan State University, 640 South Shaw Lane East Lansing, MI 48824, USA.

    Phys. Rev. C 112, 035501 – Published 17 September, 2025

    DOI: https://doi.org/10.1103/g393-xx1w

    Abstract

    A direct measurement of the ground-state-to-ground-state electron-capture decay Q (QEC) value of Tc97 has been conducted employing the high-resolving-power phase-imaging ion-cyclotron-resonance technique with the double Penning trap mass spectrometer JYFLTRAP. The resulting QEC value for Tc97 is 324.82(21) keV, exhibiting a precision approximately 19 times higher than the value adopted in the newest Atomic Mass Evaluation (AME2020) and differing by 1.2σ. Furthermore, by combining this refined Q value with nuclear energy-level data for the decay-daughter Mo97, a potential ultralow Q-value transition Tc97 (9/2+, ground state) →Mo*97 [320(1) keV] was detected. The ground-state-to-excited-state electron-capture decay Q value (QEC*) of this transition was determined to be 4.8(10) keV, confirming it to be energetically allowed with a confidence level of exceeding 4σ. The captures of electrons occupying the L and higher shells for this transition are energetically allowed, giving a value of 2.0(10) keV for the closest distance of QEC* to the allowed binding energy of the L1 shell. To predict partial half-lives and energy-release distributions for this transition, the atomic self-consistent many-electron Dirac-Hartree-Fock-Slater method and the nuclear shell model have been employed. Dominant correction terms such as exchange and overlap corrections, as well as shake-up and shake-off effects, were included in the final results. Moreover, in the case of a possible allowed transition, the normalized distribution of released energy in the electron-capture decay of Tc97 to the excited 320-keV state of Mo97, is compared with that of Ho163, which is being used for electron-neutrino-mass determination. A pseudoexperiment technique was introduced to calculate error propagation in half-life and the 68% confidence interval for normalized energy distributions.

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