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Examining evidence for a shorter Sm146−Nd142 chronology in the early solar system

Shuling Tang, Yibin Qian2,*, and Wei Liu2

Zhongzhou Ren†

  • *Contact author: qyibin@njust.edu.cn
  • †Contact author: zren@tongji.edu.cn

Phys. Rev. C 111, L052801 – Published 13 May, 2025

DOI: https://doi.org/10.1103/PhysRevC.111.L052801

Abstract

Sm146, as an extinct p-process isotope, plays an irreplaceable role in the timeline construction of the early solar system (ESS) via the geochemical tracing of its α decay to Nd142. There have been persistent discrepancies among both measured and theoretical half-lives of Sm146, which result in a large uncertainty in the initial Sm146 abundance in the ESS and subsequent dating of planetary events after the birth of the Sun. In this study, a newly proposed technique was used to analyze the α decay process within the widely employed α-core nuclear potentials, namely, three different Woods-Saxon shapes and the double-folding potential. The half-life is obtained through large-scale random sampling of parameters for each potential, with the robust results subjected to statistical analysis. Additionally, a well-founded extrapolation for α decay energy of Sm146, based on the systematic behavior of the neighboring decay chain, is in perfect agreement with the adopted experimental value, further supporting the present evaluation on this crucial half-life. As a result, the half-life of Sm146 was determined to be 71.74±7.39 million years (Ma) with a 95% confidence interval. The initial Sm146/Sm144 ratio of 0.0092±0.0014 at 4568(±10) Ma, corresponding to the formation of the solar system, is then determined, further leading to a reduced timescale for various planetary silicate mantle differentiation events of the ESS. It is expected that this study paves the way for a theoretically calibrated Sm146−Nd142 chronometer in future studies of nucleosynthesis and in earth and planetary astrophysics.

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