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Spontaneous fission instability of the neutron-deficient No and Rf isotopes: The new isotope No249

J. Khuyagbaatar1,2,*, H. Brand2, R. A. Cantemir2, Ch. E. Düllmann1,2,3, F. P. Heßberger1,2, E. Jäger2, B. Kindler2, J. Krier2, N. Kurz2 et al.

B. Lommel2, B. Schausten2, and A. Yakushev2

  • 1Helmholtz Institute Mainz, 55099 Mainz, Germany
  • 2GSI Helmholtzzentrum für Schwerionenforschung, 64291 Darmstadt, Germany
  • 3Johannes Gutenberg-Universität Mainz, 55099 Mainz, Germany

  • *J.Khuyagbaatar@gsi.de

Phys. Rev. C 104, L031303 – Published 10 September, 2021

DOI: https://doi.org/10.1103/PhysRevC.104.L031303

Abstract

In the heaviest elements, the instability of atomic nuclei against spontaneous fission leads to ever shorter nuclear half-lives. Upon falling below a timescale of 10−14 s, the border of existence of isotopes is crossed because this is the timescale on which the formation of atomic shells occurs. Analysis of the experimental data on the spontaneous fission half-lives of Rf isotopes in relation with their expected single-particle orbitals hint at a potentially abrupt decrease in half-lives of unknown neutron-deficient Rf isotopes with neutron numbers <149, which suggests that the isotopic border is already almost reached. However, this conjecture, which cannot be explained within the current knowledge, was directly related to uncertainty in the experimental data on Rf253. We revisited the decay of Rf253 and identified two fission activities, which are attributed to decays of the two different states with half-lives of 12.8−3.4+7.0 ms and 44−10+17μs. In addition, hitherto unknown α decay in Rf253, which is followed by α decay of the new isotope No249 with a half-life of 15−7+74 ms, was observed. Based on our new data, no abrupt decreases in half-lives of the neutron-deficient No and Rf isotopes are expected, which is in line with theoretical predictions. Fission half-lives of the two different states in Rf253 are benchmark cases for the theoretical description of the single-particle orbital influence on the fission process.

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