Reuse & Permissions

It is not necessary to obtain permission to reuse this article or its components as it is available under the terms of the Creative Commons Attribution 4.0 International license. This license permits unrestricted use, distribution, and reproduction in any medium, provided attribution to the author(s) and the published article's title, journal citation, and DOI are maintained. Please note that some figures may have been included with permission from other third parties. It is your responsibility to obtain the proper permission from the rights holder directly for these figures.

Export citation

Export citation

Choose format for download:

Download Citation
  • Open Access

Search for a heavy neutral lepton with the MAGNETO-ν experiment using Pu241β− decays

C. Lee1,*, X. Zhang1, A. Kavner1,†, T. Parsons-Davis1, D. Lee1, N. Hines1, S. T. P. Boyd2, M. Loidl3, X. Mougeot3 et al.

M. Rodrigues3, M. K. Lee4, J. W. Song4, R. Wood5,‡, I. Jovanovic5,‡, and G. B. Kim1,§

  • *Contact author: lee1118@llnl.gov
  • †Present address: University of Zurich, Rämistrasse 71, 8006 Zürich, Switzerland.
  • ‡Present address: University of California, Berkeley; 4163 Etcheverry Hall, Berkeley, CA 94720.
  • §Contact author: kim90@llnl.gov

Phys. Rev. C 113, 024620 – Published 26 February, 2026

DOI: https://doi.org/10.1103/4xt7-mdyv

Abstract

The MAGNETO-ν experiment searches for keV-scale heavy neutral leptons (HNLs) through precise measurements of the β−-decay spectrum of Pu241. We present spectra comprising a total of 194 million β− decays recorded using decay energy spectrometry with metallic magnetic calorimeters, representing the most statistically precise measurement of Pu241β− decay to date. The β-endpoint energy was determined using γ rays and x-rays from an external Ba133 calibration source, yielding Qβ=22.273(33)keV. The measured spectrum shows no statistically significant deviation from the allowed β-decay model. From a subset of the high-statistics data, we set an upper limit on the mixing of an 11.5-keV HNL with the electron neutrino, |Ue4|2<1.31×10−3 at the 95% confidence level.

View figure in article

Physics Subject Headings (PhySH)

Article Text

References (71)

  1. M. Aker et al. (KATRIN Collaboration), Direct neutrino-mass measurement with sub-electronvolt sensitivity, Nat. Phys. 18, 160 (2022).
  2. C. Velte et al., High-resolution and low-background Ho163 spectrum: interpretation of the resonance tails, Eur. Phys. J. C 79, 1026 (2019).
  3. M. De Gerone et al., Status of the HOLMES experiment, J. Low Temp. Phys. 209, 980 (2022).
  4. D. M. Asner et al. (Project 8 Collaboration), Single-electron detection and spectroscopy via relativistic cyclotron radiation, Phys. Rev. Lett. 114, 162501 (2015).
  5. E. Cosulich, G. Gallinaro, F. Gatti, and S. Vitale, Detection of Re187 beta decay with a cryogenic microcalorimeter. Preliminary results, Phys. Lett. B 295, 143 (1992).
  6. D. Deptuck, L. Erhardt, and J. Harrison, Achievable neutrino mass limits from calorimetric beta spectroscopy, Nucl. Instrum. Methods Phys. Res., Sect. A 444, 80 (2000).
  7. N. de Groot, Plutonium-241 as a possible isotope for neutrino mass measurement and capture, J. Phys. G 50, 055106 (2023).
  8. L. Pagnanini et al., Simultaneous measurement of the half-life and spectral shape of In115β decay with an indium iodide cryogenic calorimeter, Phys. Rev. Lett. 133, 122501 (2024).
  9. M. Paulsen, P. C.-O. Ranitzsch, M. Loidl, M. Rodrigues, K. Kossert, X. Mougeot, A. Singh, S. Leblond, J. Beyer, L. Bockhorn, C. Enss, M. Wegner, S. Kempf, and O. Nähle, High precision measurement of the Tc99β spectrum, Phys. Rev. C 110, 055503 (2024).
  10. L. Hayen, J. Kostensalo, N. Severijns, and J. Suhonen, First-forbidden transitions in the reactor anomaly, Phys. Rev. C 100, 054323 (2019).
  11. M. Betti et al., Neutrino physics with the PTOLEMY project: Active neutrino properties and the light sterile case, J. Cosmol. Astropart. Phys. 2019, 047 (2019).
  12. V. Brdar, R. Plestid, and N. Rocco, Empirical capture cross sections for cosmic neutrino detection with Sm151 and Tm171, Phys. Rev. C 105, 045501 (2022).
  13. M. Aker et al. (KATRIN Collaboration), Improved eV-scale sterile-neutrino constraints from the second KATRIN measurement campaign, Phys. Rev. D 105, 072004 (2022).
  14. E. Holzschuh, W. Kündig, L. Palermo, H. Stüssi, and P. Wenk, Search for heavy neutrinos in the β-spectrum of Ni63, Phys. Lett. B 451, 247 (1999).
  15. K. H. Hiddemann, H. Daniel, and O. Schwentker, Limits on neutrino masses from the tritium beta spectrum, J. Phys. G 21, 639 (1995).
  16. J. N. Abdurashitov, A. I. Belesev, V. G. Chernov, E. V. Geraskin, A. A. Golubev, P. V. Grigorieva, G. A. Koroteev, N. A. Likhovid, A. A. Nozik, V. S. Pantuev, V. I. Parfenov, A. K. Skasyrskaya, I. I. Tkachev, and S. V. Zadorozhny, First measurements in search for keV sterile neutrino in tritium beta-decay in the Troitsk nu-mass experiment, JETP Lett. 105, 753 (2017).
  17. O. Dragoun, A. Spalek, M. Rysavý, A. Kovalík, E. A. Yakushev, V. Brabec, A. F. Novgorodov, N. Dragounová, and J. Rízek, Search for an admixture of heavy neutrinos in the β− decay of Pu241, J. Phys. G 25, 1839 (1999).
  18. S. Friedrich, G. Kim, C. Bray, R. Cantor, J. Dilling, S. Fretwell, J. Hall, A. Lennarz, V. Lordi, P. Machule, et al., Limits on the existence of sub-MeV sterile neutrinos from the decay of Be7 in superconducting quantum sensors, Phys. Rev. Lett. 126, 021803 (2021).
  19. C. Martoff, F. Granato, V. Palmaccio, X. Yu, P. Smith, E. Hudson, P. Hamilton, C. Schneider, E. Chang, A. Renshaw, et al., HUNTER: Precision massive-neutrino search based on a laser cooled atomic source, Quantum Sci. Technol. 6, 024008 (2021).
  20. M. González-Alonso and O. Naviliat-Cuncic, Kinematic sensitivity to the Fierz term of β-decay differential spectra, Phys. Rev. C 94, 035503 (2016).
  21. H. Saul, C. Roick, H. Abele, H. Mest, M. Klopf, A. K. Petukhov, T. Soldner, X. Wang, D. Werder, and B. Märkisch, Limit on the Fierz interference term b from a measurement of the beta asymmetry in neutron decay, Phys. Rev. Lett. 125, 112501 (2020).
  22. A. Rudakovskyi and D. Iakubovskyi, Dark matter model favoured by reionization data: 7 keV sterile neutrino versus cold dark matter, Mon. Not. R. Astron. Soc. 483, 4080 (2019).
  23. R. Adhikari et al., A white paper on keV sterile neutrino dark matter, J. Cosmol. Astropart. Phys. 2017, 025 (2017).
  24. M. Loidl, E. Leblanc, M. Rodrigues, T. Branger, D. Lacour, J. Bouchard, and B. Censier, Validation study of a new technique for absolute activity measurement with 4π solid angle metallic magnetic calorimeters, Appl. Radiat. Isot. 66, 872 (2008).
  25. Y. S. Jang, S. J. Lee, G. B. Kim, I. H. Kim, M. S. Kim, H. J. Lee, J. S. Lee, K. B. Lee, M. K. Lee, H. C. Ri, W. S. Yoon, and Y. H. Kim, Development of decay energy spectroscopy for radionuclide analysis using cryogenic 4π measurements, J. Low Temp. Phys. 167, 967 (2012).
  26. K. E. Koehler, Low temperature microcalorimeters for decay energy spectroscopy, Appl. Sci. 11, 4044 (2021).
  27. A. Fleischmann, C. Enss, and G. Seidel, Metallic magnetic calorimeters, in Cryogenic Particle Detection, edited by C. Enss (Springer, Berlin, Heidelberg, 2005), pp. 151–216.
  28. S. Kempf, A. Fleischmann, L. Gastaldo, and C. Enss, Physics and applications of metallic magnetic calorimeters, J. Low Temp. Phys. 193, 365 (2018).
  29. T. Sikorsky, J. Geist, D. Hengstler, S. Kempf, L. Gastaldo, C. Enss, C. Mokry, J. Runke, C. E. Düllmann, P. Wobrauschek, K. Beeks, V. Rosecker, J. H. Sterba, G. Kazakov, T. Schumm, and A. Fleischmann, Measurement of the Th229 isomer energy with a magnetic microcalorimeter, Phys. Rev. Lett. 125, 142503 (2020).
  30. F. L. Wilson, Fermi’s theory of beta decay, Am. J. Phys. 36, 1150 (1968).
  31. Particle Data Group, Review of particle physics, Prog. Theor. Exp. Phys. 2020, 083C01 (2020).
  32. E. Fermi, Versuch einer theorie der β-strahlen. I, Eur. Phys. J. A 88, 161 (1934).
  33. L. Hayen, N. Severijns, K. Bodek, D. Rozpedzik, and X. Mougeot, High precision analytical description of the allowed β spectrum shape, Rev. Mod. Phys. 90, 015008 (2018).
  34. J. Řízek, M. Ryšavý, and V. Brabec, Effect of nuclear structure on the single particle β−transitions in deformed nuclei, Czech. J. Phys. B 45, 477 (1995).
  35. M. Chadwick et al., ENDF/B-VII.0: Next generation evaluated nuclear data library for nuclear science and technology, Nucl. Data Sheets 107, 2931 (2006).
  36. M. Wang, W. Huang, F. Kondev, G. Audi, and S. Naimi, The AME 2020 atomic mass evaluation (II). Tables, graphs and references, Chin. Phys. C 45, 030003 (2021).
  37. M. Basunia, Nuclear data sheets for A = 237, Nucl. Data Sheets 107, 2323 (2006).
  38. M. Bé, V. Chisté, C. Dulieu, E. Browne, V. Chechev, N. Kuzmenko, R. Helmer, A. Nichols, E. Schönfeld, and R. Dersch, Monographie BIPM-5—table of radionuclides, Vol. 4, Internet: http://www.nucleide.org (2004).
  39. F. L. Oetting, Average beta energy of Plutonium-241 by calorimetry, Phys. Rev. 168, 1398 (1968).
  40. M. Loidl, M. Rodrigues, B. Censier, S. Kowalski, X. Mougeot, P. Cassette, T. Branger, and D. Lacour, First measurement of the beta spectrum of Pu241 with a cryogenic detector, Appl. Radiat. Isot. 68, 1454 (2010).
  41. K. Kossert, O. J. Nähle, and A. G. Carles, Beta shape-factor function and activity determination of Pu241, Appl. Radiat. Isot. 69, 1246 (2011).
  42. X. Mougeot, Atomic exchange correction in forbidden unique beta transitions, Appl. Radiat. Isot. 201, 111018 (2023).
  43. K. Kossert, M. Loidl, X. Mougeot, M. Paulsen, P. Ranitzsch, and M. Rodrigues, High precision measurement of the Sm151 beta decay by means of a metallic magnetic calorimeter, Appl. Radiat. Isot. 185, 110237 (2022).
  44. F. G. A. Quarati, G. Bollen, P. Dorenbos, M. Eibach, K. Gulyuz, A. Hamaker, C. Izzo, D. K. Keblbeck, X. Mougeot, D. Puentes, M. Redshaw, R. Ringle, R. Sandler, J. Surbrook, and I. Yandow, Measurements and computational analysis of the natural decay of Lu176, Phys. Rev. C 107, 024313 (2023).
  45. B. Brown and W. Rae, The shell-model code NuShellX@MSU, Nucl. Data Sheets 120, 115 (2014).
  46. E. K. Warburton and B. A. Brown, Appraisal of the Kuo-Herling shell-model interaction and application to A = 210–212 nuclei, Phys. Rev. C 43, 602 (1991).
  47. C. R. Bates, C. Pies, S. Kempf, D. Hengstler, A. Fleischmann, L. Gastaldo, C. Enss, and S. Friedrich, Reproducibility and calibration of MMC-based high-resolution gamma detectors, Appl. Phys. Lett. 109, 023513 (2016).
  48. N. Kovač, F. Adam, S. Kempf, M.-C. Langer, M. Müller, R. Sack, M. Schlösser, M. Steidl, and K. Valerius, Comparison of the detector response and calibration function of metallic microcalorimeters for X-ray photons and external electrons, Nucl. Instrum. Methods Phys. Res., Sect. A 1080, 170662 (2025).
  49. G.-B. Kim, R. Hummatov, S. Kempf, C. Flynn, R. Cantor, A. Fleischmann, S. T. P. Boyd, C. Enss, and S. Friedrich, Consistent measurements of U233 gamma emissions using metallic magnetic calorimeters with ultra-high energy resolution, J. Radioanal. Nucl. Chem. 318, 803 (2018).
  50. C. Enss and S. Hunklinger, Low-Temperature Physics, SpringerLink: Springer e-Books (Springer, Berlin, Heidelberg, 2005).
  51. M. Krantz, F. Toschi, B. Maier, G. Heine, C. Enss, and S. Kempf, Magnetic microcalorimeter with paramagnetic temperature sensors and integrated dc-SQUID readout for high-resolution x-ray emission spectroscopy, Appl. Phys. Lett. 124, 032601 (2024).
  52. M. Wegner, N. Karcher, O. Krömer, D. Richter, F. Ahrens, O. Sander, S. Kempf, M. Weber, and C. Enss, Microwave SQUID multiplexing of metallic magnetic calorimeters: Status of multiplexer performance and room-temperature readout electronics development, J. Low Temp. Phys. 193, 462 (2018).
  53. S. Kempf, M. Wegner, A. Fleischmann, L. Gastaldo, F. Herrmann, M. Papst, D. Richter, and C. Enss, Demonstration of a scalable frequency-domain readout of metallic magnetic calorimeters by means of a microwave SQUID multiplexer, AIP Adv. 7, 015007 (2017).
  54. A. S. Hoover, E. M. Bond, M. P. Croce, T. G. Holesinger, G. J. Kunde, M. W. Rabin, L. E. Wolfsberg, D. A. Bennett, J. P. Hays-Wehle, D. R. Schmidt, et al., Measurement of the Pu240/Pu239 mass ratio using a transition-edge-sensor microcalorimeter for total decay energy spectroscopy, Anal. Chem. 87, 3996 (2015).
  55. G.-B. Kim, A. Kavner, T. Parsons-Davis, S. Friedrich, O. Drury, D. Lee, X. Zhang, N. Hines, S. Boyd, S. Weidenbenner, et al., Decay energy spectrometry for improved nuclear material analysis at the IAEA NML, arXiv:2406.05200.
  56. J. Song, S. Kim, H. Kim, H. Kim, and M. Lee, Modification of the metallic magnetic calorimeter fabrication process for high production yield, J. Low Temp. Phys. 216, 436 (2024).
  57. J. Song, Y. Cho, H. Kim, and M. Lee, Synthesis and characterization of an Ag: Er alloy for metallic magnetic calorimeters, J. Low Temp. Phys. 218, 110 (2025).
  58. S. Agostinelli et al., geant4—a simulation toolkit, Nucl. Instrum. Methods Phys. Res., Sect. A 506, 250 (2003).
  59. S. T. Perkins, D. E. Cullen, and S. M. Seltzer, Tables and graphs of electron-interaction cross sections from 10 eV to 100 GeV derived from the LLNL evaluated electron data library (EEDL), Z = 1–100, Technical Report (Lawrence Livermore National Laboratory, 1991).
  60. Stanford Research Systems (2024), https://www.thinksrs.com/products/sr560.html.
  61. National Instrument (2024), https://www.ni.com/en-us/shop/model/pxie-5172.html?srsltid=AfmBOoq1zTkV7A2chB330 NRnwc4GyKLPY8r1qYRh8FY5EvU-0k5JMy_6.
  62. V. T. Jordanov, G. F. Knoll, A. C. Huber, and J. A. Pantazis, Digital techniques for real-time pulse shaping in radiation measurements, Nucl. Instrum. Methods Phys. Res., Sect. A 353, 261 (1994).
  63. I. Kim et al. (BeEST Collaboration), Signal processing and spectral modeling for the BeEST experiment, Phys. Rev. D 111, 052010 (2025).
  64. M. Berger, J. Coursey, and M. Zucker, ESTAR, PSTAR, and ASTAR: Computer programs for calculating stopping-power and range tables for electrons, protons, and helium ions (version 1.21) (1999).
  65. R. D. Deslattes, E. G. Kessler, P. Indelicato, L. de Billy, E. Lindroth, and J. Anton, X-ray transition energies: New approach to a comprehensive evaluation, Rev. Mod. Phys. 75, 35 (2003).
  66. S. Friedrich, F. Ponce, J. A. Hall, and R. Cantor, Non-linearities in superconducting tunnel junction radiation detectors and their MCA readout, J. Low Temp. Phys. 200, 200 (2020).
  67. This approximation of the asymmetric response, similar to that used for α peaks, is justified because the expected energy loss due to self-absorption is two orders of magnitude smaller than the energy resolution at 20 keV.
  68. M. L. Zahir, M. Rodrigues, M. Loidl, and A. Kaur, Energy non-linearity study of a high-resolution metallic magnetic calorimeter, Radiat. Phys. Chem. 220, 111730 (2024).
  69. S. Friedrich, A. Marino, F. Ponce, M. F. Carpenter, G. B. Kim, O. B. Drury, J. Drake, C. R. Bray, S. Fretwell, K. G. Leach, J. Harris, W. K. Warburton, J. A. Hall, and R. Cantor, Characterization of non-uniformities in superconducting tunnel junction radiation detectors, J. Low Temp. Phys. 209, 1063 (2022).
  70. C. Bray et al., The data acquisition system for phase-III of the BeEST experiment, J. Low Temp. Phys. 218, 74 (2025).
  71. N. Abgrall et al., ADC nonlinearity correction for the Majorana demonstrator, IEEE Trans. Nucl. Sci. 68, 359 (2021).

Outline

Information

Sign In to Your Journals Account

Filter

Filter

Article Lookup

Enter a citation