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    Search for evidence of nuclear excitation by electron capture in Cs127

    C. J. Chiara1,*, J. J. Carroll1, A. D. Ayangeakaa2,3, M. P. Carpenter4, P. A. Copp4,†, C. Gautam1,5,6, M. Gott4,‡, J. P. Greene4, D. J. Hartley7 et al.

    A. B. Hayes8,9, G. J. Lane10, T. Lauritsen4, D. A. Matters11, A. J. Mitchell10, C. Müller-Gatermann4, M. Polasik12, W. Reviol4, J. Rzadkiewicz13, D. Seweryniak4, M. Siciliano4, K. Słabkowska12, Ł. Syrocki12,14, J. R. Vanhoy7, and S. Zhu8,§

    • *Contact author: christopher.j.chiara2.civ@army.mil
    • †Present address: Los Alamos National Laboratory, Los Alamos, New Mexico 87545, USA.
    • ‡Present address: Enrichment Science and Engineering Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37830, USA.
    • §Deceased.

    Phys. Rev. C 114, 024310 – Published 4 August, 2026

    DOI: https://doi.org/10.1103/18zr-mm2k

    Abstract

    Nuclear excitation by electron capture (NEEC) is a coupled nuclear-atomic process by which the capture of an electron by an ion into an atomic vacancy results in the excitation of the corresponding nucleus into a higher excited state. To date, there has been only one experimental result, for the nucleus Mo93, where a signal indicative of NEEC has been reported. Additional experimental data are vital to provide a testbed for developing theoretical NEEC models to aid in better understanding this phenomenon. In this work, a second NEEC candidate, Cs127, was explored using a methodology similar to that in the prior Mo93 study. Highly stripped ions of Cs127 in its 53.3-µs isomeric state were produced in Be9(Sb123,5n) reactions and implanted into target foils. NEEC-signature γ-ray coincidences were sought using the Digital Gammasphere spectrometer. Although a signature was not observed, upper limits on the NEEC probability were established: 0.17% for implantation into a layered Al27/Pb208 target and 0.27% for a single Pb208 foil. Theory predicts a yield well below these levels; while the results for Cs127 are thus consistent, they ultimately do not provide an explanation that helps resolve the underlying discrepancy between theory and experiment for Mo93.

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