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    White-line evolution in shocked solid Ta evidenced by synchrotron x-ray absorption spectroscopy

    C. M. Pépin1,2, R. Torchio3, F. Occelli1,2, E. Lescoute1,2, O. Mathon3, V. Recoules1,2, J. Bouchet1,2, L. Videau1,2, A. Benuzzi-Mounaix4 et al.

    T. Vinci4, R. Briggs3,*, S. Pascarelli3, R. Gaal5, P. Loubeyre1,2, and A. Sollier1,2,†

    • 1CEA, DAM, DIF, 91297 Arpajon, France
    • 2Université Paris-Saclay, CEA, Laboratoire Matière en Conditions Extrêmes, 91680 Bruyères-le-Châtel, France
    • 3ESRF, 6 Rue Jules Horowitz BP220, F-38043 Grenoble Cedex, France
    • 4Laboratoire d'Utilisation des Lasers Intenses - CNRS, Ecole Polytechnique, CEA, Université Paris-Saclay, F-91128 Palaiseau Cedex, France
    • 5Earth and Planetary Science Laboratory, Institute of Physics, Ecole Polytechnique Fédérale de Lausanne, CH-1015 Lausanne, Switzerland

    • *Present address: Lawrence Livermore National Laboratory, Livermore, CA 94550, USA.
    • †arnaud.sollier@cea.fr

    Phys. Rev. B 102, 144102 – Published 9 October, 2020

    DOI: https://doi.org/10.1103/PhysRevB.102.144102

    Abstract

    Time-resolved x-ray absorption experiments have been performed on shocked tantalum. Using a single 100 ps synchrotron x-ray pulse, nanosecond-lived equilibrium states of shocked solid Ta have been measured by L3-edge absorption spectroscopy. The energy shift and intensity change of the white line were measured up to 130 GPa and 2000 K. The experimental results are discussed in light of density functional theory calculations and FEFF simulations. The absence of occurrence of the hcp-ω phase is suggested from the analysis of the shape of the white line.

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